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Homogeneous nucleation is formulated within the context of fluctuating hydrodynamics. It is shown that for a colloidal or macromolecular system in the strong damping limit the most likely path for nucleation can be determined by gradient…

Soft Condensed Matter · Physics 2011-10-27 James F. Lutsko

The microscopic mechanisms controlling heterogeneous ice nucleation are complex and remain poorly understood. Although good ice nucleators are generally believed to match ice lattice and to bind water, counter examples are often identified.…

Chemical Physics · Physics 2015-10-07 Yuanfei Bi , Raffaela Cabriolu , Tianshu Li

Orientational and positional ordering properties of liquid crystal monolayers are examined by means of Fundamental-Measure Density Functional Theory. Particles forming the monolayer are modeled as hard parallelepipeds of square section of…

Soft Condensed Matter · Physics 2015-06-19 Yuri Martinez-Raton , Szabolcs Varga y Enrique Velasco

We test the performance of a recently proposed fundamental measure density functional of aligned hard cylinders by calculating the phase diagram of a monodisperse fluid of these particles. We consider all possible liquid crystalline…

Soft Condensed Matter · Physics 2009-11-13 Jose A. Capitan , Yuri Martinez-Raton , Jose A. Cuesta

We present a phase field theory for binary crystal nucleation. In the one-component limit, quantitative agreement is achieved with computer simulations (Lennard-Jones system) and experiments (ice-water system) using model parameters…

Soft Condensed Matter · Physics 2009-11-07 Laszlo Granasy , Tamas Borzsonyi , Tamas Pusztai

The classical nucleation theory for homogeneous nucleation is formulated as a theory for a density fluctuation in a supersaturated gas at a given temperature. But Molecular Dynamics simulations reveal that it is small cold clusters which…

Other Condensed Matter · Physics 2015-10-28 Søren Toxvaerd

The atomic lensing model has been proposed as a promising method facilitating atom-counting in heterogeneous nanocrystals [KHW van den Bos et. al, Phys. Rev. Lett. 116 (2016) 246101] Here, image simulations will validate the model, which…

Materials Science · Physics 2019-02-18 K. H. W. van den Bos , L. Janssens , A. De Backer , P. D. Nellist , S. Van Aert

It is increasingly being realized that liquid-crystalline features can play an important role in the properties and dynamics of cell monolayers. Here, we present a cell-based model of cell layers, based on the phase-field formulation, that…

Soft Condensed Matter · Physics 2022-04-28 Aleksandra Ardaševa , Romain Mueller , Amin Doostmohammadi

Nucleation, commonly associated with discontinuous transformations between metastable and stable phases, is crucial in fields as diverse as atmospheric science and nanoscale electronics. Traditionally, it is considered a microscopic process…

Nucleation and growth of crystal in an oxide glass was studied in a Si B Al Zr Nd Ca Na O system. The nucleation and growth process was monitored by thermal analysis and isothermal experiments. For the Ca sample the crystallization is…

Materials Science · Physics 2007-10-10 D. De Ligny , Daniel Caurant , I. Bardez , J. -L. Dussossoy , P. Loiseau , D. R. Neuville

Homogeneous nucleation of the new phase of one transition near a second phase transition is considered. The system has two phase transitions, we study the nucleation of the new phase of one of these transitions under conditions such that we…

Statistical Mechanics · Physics 2009-11-07 Z. Tavassoli , R. P. Sear

Motivated by unexpected morphologies of the emerging liquid phase (channels, bulges, droplets) at the edge of thin, melting alkane terraces, we propose a new heterogeneous nucleation pathway. The competition between bulk and interfacial…

Chemical Physics · Physics 2015-06-04 Halim Kusumaatmaja , Reinhard Lipowsky , Chenyu Jin , Radu-Cristian Mutihac , Hans Riegler

This paper deals with the condensation of liquid droplets on hydrophobic and hydrophilic surfaces. A stochastic mesoscale model based on the theory of fluctuating hydrodynamics and the thermodynamics of a diffuse interface approach shows…

Soft Condensed Matter · Physics 2025-06-30 Matteo Teodori , Dario Abbondanza , Mirko Gallo , Carlo Massimo Casciola

Understanding the underlying mechanism of crystal nucleation during solidification is a fundamental aspect in the prediction and control of materials properties. Classical nucleation theory (CNT) assumes that homogeneous nucleation occurs…

Computational Physics · Physics 2018-12-14 Grisell Diaz Leines , Jutta Rogal

A continuum density-field formulation with particle-scale resolution is constructed to simultaneously incorporate the orientation dependence of interparticle interactions and the rotational invariance of the system, a fundamental but…

Materials Science · Physics 2018-05-28 Zi-Le Wang , Zhirong Liu , Zhi-Feng Huang

The nucleation of a droplet of stable cylinder phase from a metastable lamellar phase is examined within the single-mode approximation to the Brazovskii model for diblock copolymer melts. By employing a variational ansatz for the droplet…

Soft Condensed Matter · Physics 2009-11-10 Robert A. Wickham , An-Chang Shi , Zhen-Gang Wang

Systems with long-range interactions when quenced into a metastable state near the pseudo-spinodal exhibit nucleation processes that are quite different from the classical nucleation seen near the coexistence curve. In systems with…

Materials Science · Physics 2009-11-07 W. Klein , T. Lookman , A. Saxena , D. Hatch

$^4$He nanodroplets doped with an alkali ion feature a snowball of crystallized layers surrounded by superfluid helium. For large droplets, we predict that a transitional supersolid layer can form, bridging between the solid core and the…

Quantum Gases · Physics 2025-03-12 Juan Carlos Acosta Matos , Panos Giannakeas , Matteo Ciardi , Thomas Pohl , Jan M. Rost

Experiments have not only revealed the remarkably long lifetime of nanobubbles, but also demonstrated the diffusive instability of bubbles above micrometers, thus a full-scale physical understanding on the stability of bubbles is in urgent…

Soft Condensed Matter · Physics 2021-12-28 Binghai Wen , Yongcai Pan , Lijuan Zhang , Shuo Wang , Limin Zhou , Chunlei Wang , Jun Hu

Ice nucleation is greatly important in areas as diverse as climate change, cryobiology, geology or food industry. Predicting the ability of a substrate to induce the nucleation of ice from supercooled water is a difficult problem. Here, we…

Materials Science · Physics 2026-01-12 Miguel Camarillo , Javier Oller-Iscar , María M. Conde , Jorge Ramírez , Eduardo Sanz
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