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We study the influence of off-resonant two photon transitions on high precision measurements with atom interferometers based on stimulated Raman transitions. These resonances induce a two photon light shift on the resonant Raman condition.…

Optical sensing schemes that rely on two-photon interference provide a powerful platform for precision metrology, although they are inherently constrained by a trade-off between dynamic range and measurement precision. To overcome this…

We report a numerical calculation of the two-photon absorption coefficient of electrons in a binding potential using the real-time real-space higher-order difference method. By introducing random vector averaging for the intermediate state,…

Materials Science · Physics 2009-10-31 Yoshiyuki Kurokawa , Shintaro Nomura , Tadashi Takemori , Yoshinobu Aoyagi

Quantum spectroscopy seeks to probe chemical systems using nonclassical light, which has properties that are qualitatively and quantitatively different than conventional light sources. One promising technique uses intensity-correlated twin…

We closely replicated and extended a recent experiment ("Spatial properties of entangled two-photon absorption," Phys. Rev. Lett. 129, 183601, 2022) that reportedly observed enhancement of two-photon absorption rates in molecular samples by…

Quantum Physics · Physics 2024-04-26 Tiemo Landes , Brian J. Smith , Michael G. Raymer

We have found that the error-signal frequency corresponding to the coherent population trapping resonance can be displaced from that of "$0-0$" transition unperturbed by the optical field, although the frequency is not sensitive to changes…

Precise measurement of the angular deviation of an object is a common task in science and technology. Many methods use light for this purpose. Some of these exploit interference effects to achieve technological advantages, such as…

Quantum Physics · Physics 2020-08-19 G. H. Aguilar , R. S. Piera , P. L. Saldanha , R. L. de Matos Filho , S. P. Walborn

We demonstrate a technique to lock the frequency of a laser to a transition between two excited states in Rb vapor in the presence of a weak magnetic field. We use a ladder configuration from specific hyperfine sublevels of the 5S 1/2, 5P…

Optics · Physics 2015-05-13 F. E. Becerra , R. T. Willis , S. L. Rolston , L. A. Orozco

Recent theoretical and experimental studies have shown that squeezed states of light can be engineered to enhance the resolution of nonlinear optical measurements. Here, we analyze non-degenerate two-photon absorption signals obtained from…

Quantum Physics · Physics 2025-06-10 Gaurav Shukla , Shahram Panahiyan , Devendra Kumar Mishra , Frank Schlawin

We demonstrate and study the enhancement of intermediate-field two-photon absorption by shaped femtosecond pulses having spectral phases of antisymmetric nature. The intermediate-field regime corresponds to pulse intensities, where the…

Atomic Physics · Physics 2015-05-14 Lev Chuntonov , Leonid Rybak , Andrey Gandman , Zohar Amitay

Measurements monitoring the inductive coupling between oscillating radio-frequency magnetic fields and objects of interest create versatile platforms for non-destructive testing. The benefits of ultra low frequency measurements, i.e., below…

Applied Physics · Physics 2024-10-17 L. M. Rushton , L. M. Ellis , J. D. Zipfel , P. Bevington , W. Chalupczak

A two-photon transition in laser-cooled and trapped calcium atoms is proposed as the atomic reference in an optical frequency standard. An efficient scheme for interrogation of the frequency standard is described, and the sensitivity of the…

Atomic Physics · Physics 2015-01-09 Amar C. Vutha

Optical absorption measurements characterize a wide variety of systems from atomic gases to \emph{in-vivo} diagnostics of living organisms. Here we study the potential of non-classical techniques to reduce statistical noise below the…

The effect of quantum interference on the optical properties of a pumped-probe three-level V-type atomic system is investigated. The probe absorption, dispersion, group index and optical bistability beyond the two-photon resonance condition…

Quantum Physics · Physics 2015-06-04 S. M. Mousavi , L. Safari , M. Mahmoudi , M. Sahrai

By combining genetic algorithm and a spatial light modulator we theoretically analyse how to improve a two-photon cascade absorption in atomic ensembles, inspecting the impact of various configurations and parameters in the optimized phase…

Atomic Physics · Physics 2026-02-24 L. B. A. Mélo , Daniel Felinto , Marcio H. G. de Miranda

Dissipation of electromagnetic energy through absorption is a fundamental process that underpins phenomena ranging from photovoltaics to photography, analytical spectroscopy, photosynthesis, and human vision. Absorption is also a dynamic…

Optics · Physics 2022-09-13 Venkatram Nalla , Xu Fang , João Valente , Handong Sun , Nikolay I Zheludev

We demonstrate suppression and enhancement of spontaneous parametric down- conversion via quantum interference with two weak fields from a local oscillator (LO). Pairs of LO photons are observed to upconvert with high efficiency for…

Quantum Physics · Physics 2009-11-07 K. J. Resch , J. S. Lundeen , A. M. Steinberg

We report Doppler-free two-photon absorption of N$_2$O at $\lambda$ = 4.53 $\mu$m, measured by cavity ring-down spectroscopy. High power was achieved by optical self-locking of a quantum cascade laser to a linear resonator of finesse $F$ =…

Chemical Physics · Physics 2020-07-01 Gang Zhao , D. Michelle Bailey , Adam J. Fleisher , Joseph T. Hodges , Kevin K. Lehmann

We have expressed the nonlinear optical absorption of a semiconductor in terms of its linear spectrum. We determined that the two-photon absorption coefficient in a strong DC-electric field of a direct gap semiconductor can be expressed as…

Optics · Physics 2009-11-13 Hernando Garcia , Ramki Kalyanaraman

We present non-standard optical Ramsey schemes that use pulses individually tailored in duration, phase, and frequency to cancel spurious frequency shifts related to the excitation itself. In particular, the field shifts and their…