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Monolayer transition-metal dichalcogenides (TMDCs) have recently emerged as possible candidates for valleytronic applications, as the spin and valley pseudospin are directly coupled and stabilized by a large spin splitting. In these…

We have investigated the exciton dynamics in transition metal dichalcogenide mono-layers using time-resolved photoluminescence experiments performed with optimized time-resolution. For MoSe2 monolayers, we measure $\tau_{rad}=1.8\pm0.2$ ps…

Materials Science · Physics 2016-05-18 C. Robert , D. Lagarde , F. Cadiz , G. Wang , B. Lassagne , T. Amand , A. Balocchi , P. Renucci , S. Tongay , B. Urbaszek , X. Marie

We develop an analytically solvable model able to qualitatively explain nonhydrogenic exciton spectra observed recently in two-dimensional (2d) semiconducting transition metal dichalcogenides. Our exciton Hamiltonian explicitly includes…

Mesoscale and Nanoscale Physics · Physics 2016-07-11 Maxim Trushin , Mark Oliver Goerbig , Wolfgang Belzig

Transition metal dichalcogenide (TMD) monolayers are two-dimensional semiconductors with two valleys in their band structure that can be selectively addressed using circularly polarized light. Their photoluminescence spectrum is…

Mesoscale and Nanoscale Physics · Physics 2020-10-26 Joris J. Carmiggelt , Michael Borst , Toeno van der Sar

We present a many-body theory for exciton-trion-polaritons in doped two-dimensional materials. Exciton-trion-polaritons are robust coherent hybrid excitations involving excitons, trions, and photons. Signatures of these polaritons have been…

Mesoscale and Nanoscale Physics · Physics 2021-03-31 Farhan Rana , Okan Koksal , Minwoo Jung , Gennady Shvets , A. Nick Vamivakas , Christina Manolatou

Fabricating van der Waals (vdW) bilayer heterostructures (BL-HS) by stacking the same or different two-dimensional (2D) layers, offers a unique physical system with rich electronic and optical properties. Twist-angle between component…

Mesoscale and Nanoscale Physics · Physics 2020-12-17 Kha Tran , Junho Choi , Akshay Singh

We present a microscopic many-body theory of the recently measured two-dimensional coherent spectroscopy (2DCS) of excitons and trions in monolayer MoSe$_{2}$ materials {[}K. Hao \textit{et al.}, Nano Lett. \textbf{16}, 5109 (2016){]},…

Mesoscale and Nanoscale Physics · Physics 2024-01-18 Hui Hu , Jia Wang , Xia-Ji Liu

Monolayers of transition metal dichalcogenides (TMDC) became one of the most studied nanostructures in the last decade. Combining two different TMDC monolayers results in a heterostructure whose properties can be individually tuned by the…

Mesoscale and Nanoscale Physics · Physics 2024-03-29 Marten Richter

The nature of trions and their interaction with light has remained a puzzle. The composition and dispersion of polaritons involving trions provide insights into this puzzle. Trions and excitons in doped two-dimensional (2D) materials are…

Mesoscale and Nanoscale Physics · Physics 2021-07-28 Okan Koksal , Minwoo Jung , Christina Manolatou , A. Nick Vamivakas , Gennady Shvets , Farhan Rana

Controlling excitons and their transport in two-dimensional (2D) transition metal dichalcogenides (TMDs) heterostructures is central to advancing photonics and electronics on-chip integration. We investigate the controlled generation and…

Cavity-integrated transition metal dichalcogenide excitons have recently emerged as a promising platform to study strong light-matter interactions and related cavity quantum electrodynamics phenomena. While this exciton-cavity system is…

Applied Physics · Physics 2020-03-10 David Rosser , Taylor Fryett , Albert Ryou , Abhi Saxena , Arka Majumdar

Two dimensional (2D) transition metal dichalcogenide (TMDC) materials, such as MoS2, WS2, MoSe2, and WSe2, have received extensive attention in the past decade due to their extraordinary physical properties. The unique properties make them…

The optical response of semiconducting monolayer transition-metal dichalcogenides (TMDCs) is dominated by strongly bound excitons that are stable even at room temperature. However, substrate-related effects such as screening and disorder in…

Charged excitons, or trions, offering unique spin and charge degrees of freedom, have primarily been investigated in doped systems where charges are long considered indispensable. Here, we present an alternative route to ultra-efficient…

Mesoscale and Nanoscale Physics · Physics 2026-02-17 N. Fang , U. Erkilic , Y. R. Chang , S. Fujii , D. Yamashita , C. F. Fong , S. Morito , K. Kanahashi , T. Taniguchi , K. Watanabe , K. Ueno , K. Nagashio , Y. K. Kato

We have accurately determined the exciton binding energy and reduced mass of single crystals of methylammonium lead tri-iodide using magneto-reflectivity at very high magnetic fields. The single crystal has excellent optical properties with…

Excitonic effects play a particularly important role in the optoelectronic behavior of two-dimensional (2D) semiconductors. To facilitate the interpretation of experimental photoabsorption and photoluminescence spectra we provide…

Mesoscale and Nanoscale Physics · Physics 2018-01-04 M. Szyniszewski , E. Mostaani , N. D. Drummond , V. I. Fal'ko

Excitons in bilayer transition metal dichalcogenides (2L-TMDs) are Coulomb-bound electron/hole pairs that can be viewed as broadly tunable analogs of atomic or molecular systems. Here, we study the properties of 2L-TMD excitons under strong…

Mesoscale and Nanoscale Physics · Physics 2023-03-20 S. Kovalchuk , K. Greben , A. Kumar , S. Pessel , K. Watanabe , T. Taniguchi , D. Christiansen , M. Selig , A. Knorr , K. I. Bolotin

Recent optical studies of monolayer transition metal dechalcogenides have demonstrated that their excitonic absorption feature splits into two widely separated peaks at finite carrier densities. The additional peak is usually attributed to…

Mesoscale and Nanoscale Physics · Physics 2017-01-25 Dmitry K. Efimkin , Allan H. MacDonald

A fully microscopic model of the doping-dependent exciton and trion line widths in the absorption spectra of monolayer transition metal dichalcogenides in the low temperature and low doping regime is explored. The approach is based on…

Mesoscale and Nanoscale Physics · Physics 2020-06-24 Matthew R. Carbone , Matthew Z. Mayers , David R. Reichman

We measure the optical absorption spectra and optical conductivities of excitons and trions in monolayers of metal dichalcogenide MoS$_{2}$ and compare the results with theoretical models. Our results show that the Wannier-Mott model for…

Mesoscale and Nanoscale Physics · Physics 2014-06-04 Changjian Zhang , Haining Wang , Weimin Chan , Christina Manolatou , Farhan Rana