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Related papers: Giant Rydberg Excitons in Cuprous Oxide

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The ability to generate and control strong long-range interactions via highly excited electronic states has been the foundation for recent breakthroughs in a host of areas, from atomic and molecular physics [1, 2] to quantum optics [3, 4]…

Mesoscale and Nanoscale Physics · Physics 2021-07-14 Julian Heckötter , Valentin Walther , Stefan Scheel , Manfred Bayer , Thomas Pohl , Marc Aßmann

High-lying Rydberg states of Mott-Wannier excitons are receiving considerable interest due to the possibility of adding long-range interactions to the physics of exciton-polaritons. Here, we study Rydberg excitation in bulk synthetic…

Rydberg excitons are, with their ultrastrong mutual interactions, giant optical nonlinearities, and very high sensitivity to external fields, promising for applications in quantum sensing and nonlinear optics at the single-photon level. To…

Excitons, i.e. the bound states of an electron and a positively charged hole are the solid state analogue of the hydrogen atom. As such they exhibit a Rydberg series, which in cuprous oxide has been observed up to high principal quantum…

Mesoscale and Nanoscale Physics · Physics 2025-11-18 Jan Ertl , Patric Rommel , Jörg Main

Hosting giant Rydberg excitons with principal quantum numbers up to n = 30, cuprous oxide (Cu2O) provides a rare solid-state setting for exploring Rydberg physics, as exemplified by the blockade effect. Here we access the strongly…

Rydberg excitons (analogues of Rydberg atoms in condensed matter systems) are highly excited bound electron-hole states with large Bohr radii. The interaction between them as well as exciton coupling to light may lead to strong optical…

We report experimental and theoretical investigations of interacting excitons of the yellow series in cuprous oxide (Cu$_2$O) with principal quantum numbers up to $n=7$ by means of second harmonic generation (SHG). Using picosecond pulsed…

Cuprous oxide (Cu$_2$O) is a semiconductor with large exciton binding energy and significant technological importance in applications such as photovoltaics and solar water splitting. It is also a superior material system for quantum optics…

Rydberg excitons in the semiconductor Cu$_2$O have been observed in absorption experiments up to a principal quantum number of n = 28 at millikelvin temperatures [1]. Here, we extend the experimental parameter space by variing both…

Mesoscale and Nanoscale Physics · Physics 2025-11-03 Julian Heckötter , David Janas , Marc Aßmann , Manfred Bayer

Highly-excited states of excitons in cuprous oxide have recently been observed at a record quantum number of up to $n=25$. Here, we evaluate the long-range interactions between pairs of Rydberg excitons in Cu$_2$O, which are due to direct…

Quantum Gases · Physics 2018-10-17 Valentin Walther , Sjard Ole Krüger , Stefan Scheel , Thomas Pohl

We theoretically investigate the nonlinear optical transmission through a cuprous oxide crystal for wavelengths that cover the series of highly excited excitons, observed in recent experiments. Since such Rydberg excitons have strong van…

Mesoscale and Nanoscale Physics · Physics 2020-09-02 Valentin Walther , Thomas Pohl

The enhanced Coulomb interaction in two-dimensional (2D) semiconductors leads to the tightly bound electron-hole pairs known as excitons. The large binding energy of excitons enables the formation of Rydberg excitons with high principal…

Mesoscale and Nanoscale Physics · Physics 2024-02-21 Zhen Lian , Yun-Mei Li , Li Yan , Lei Ma , Dongxue Chen , Takashi Taniguchi , Kenji Watanabe , Chuanwei Zhang , Su-Fei Shi

When an electron in a semiconductor gets excited to the conduction band the missing electron can be viewed as a positively charged particle, the hole. Due to the Coulomb interaction electrons and holes can form a hydrogen-like bound state…

Mesoscale and Nanoscale Physics · Physics 2024-10-03 Jan Ertl , Sebastian Rentschler , Jörg Main

Cuprous oxide (Cu${}_2$O) has recently been proposed as a promising solid-state host for excitonic Rydberg states with large principal quantum numbers ($n$), whose exaggerated wavefunction sizes ($\propto n^2)$ facilitate gigantic…

Quantum Physics · Physics 2022-11-01 Jacob DeLange , Kinjol Barua , Val Zwiller , Stephan Steinhauer , Hadiseh Alaeian

Rydberg excitons in two-dimensional semiconductors provide sensitive and non-destructive probes of physics in proximal sample layers that host correlated electronic states. In particular, electron or hole doping of the sample layer is…

Mesoscale and Nanoscale Physics · Physics 2025-12-09 Arthur Christianen , Anna M. Seiler , Alperen Tüğen , Ataç İmamoğlu

We report exciton-mediated coupling between microwave and optical fields in cuprous oxide (Cu$_2$O) at low temperatures. Rydberg excitonic states with principal quantum number up to $n=12$ were observed at 4~K using both one-photon…

The quantum confinement of Rydberg excitons is an important step towards exploiting their large nonlinearities for quantum applications. We observe Rydberg excitons in natural nanoparticles of Cu$_2$O. We resolve up to the principal quantum…

Rydberg excitons in Cu2O can be an emergent platform for solid-state quantum information processing by utilizing the exaggerated properties of high-lying excited states within the material. To develop practical quantum systems,…

Mesoscale and Nanoscale Physics · Physics 2021-05-19 Dungeon Daniel Kang , Aaron Gross , HeeBong Yang , Yusuke Morita , Kyung Soo Choi , Kosuke Yoshioka , Na Young Kim

Solid-state platforms provide exceptional opportunities for advancing on-chip quantum technologies by enhancing interaction strengths through coupling, scalability, and robustness. Cuprous oxide ($\text{Cu}_{2}\text{O}$) has recently…

We investigate the interaction between highly excited Rydberg excitons and charged impurities in the semiconductor Cuprous Oxide. We find that it is long-ranged and based on charge-induced dipole interactions. We demonstrate that we can…

Mesoscale and Nanoscale Physics · Physics 2023-10-19 Martin Bergen , Valentin Walther , Binodbihari Panda , Mariam Harati , Simon Siegeroth , Julian Heckötter , Marc Aßmann
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