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We study the second harmonic generation (SHG) in a suspension of small spherical particles confined within a slab, assuming undepleted pump and applying (i) single scattering approximation and (ii) diffusion approximation. In the case (i),…

Optics · Physics 2007-05-23 E. V. Makeev , S. E. Skipetrov

Optical second harmonic generation (SHG) has been measured for the first time in reflection from the nanometer-thick films (6 to 40 nm) of the topological insulator Bi2Se3 using 1.51 eV (820 nm) Ti:Sapphire laser photons and revealed a…

Mesoscale and Nanoscale Physics · Physics 2015-06-11 Yuri D. Glinka , Sercan Babakiray , Trent A. Johnson , Mikel B. Holcomb , David Lederman

The generation of second and third harmonics by an acoustic wave propagating along one dimension in a weakly nonlinear elastic medium that is loaded harmonically in time with frequency $\omega_0$ at a single point in space, is analyzed by…

Materials Science · Physics 2024-12-11 Fernando Lund

We report about the experimental observation and characterization of nonlinear optical properties of individual silicon nanowires of different dimensions. Our results show that the nonlinear light has different components, one of them…

Mesoscale and Nanoscale Physics · Physics 2017-04-13 Peter R. Wiecha , Arnaud Arbouet , Houssem Kallel , Priyanka Periwal , Thierry Baron , Vincent Paillard

We report on strong enhancement of mid-infrared second harmonic generation (SHG) from SiC nanopillars due to the resonant excitation of localized surface phonon-polaritons within the Reststrahlen band. The magnitude of the SHG peak at the…

We aim to clarify the role that absorption plays in nonlinear optical processes in a variety of metallic nanostructures and show how it relates to emission and conversion efficiency. We define a figure of merit that establishes the…

A central goal of condensed-matter physics is to understand how the diverse electronic and optical properties of crystalline materials emerge from the wavelike motion of electrons through periodically arranged atoms. However, more than 90…

Materials Science · Physics 2021-11-09 J. B. Costello , S. D. O'Hara , Q. Wu , D. C. Valovcin , L. N. Pfeiffer , K. W. West , M. S. Sherwin

We derive an expression for the effective second-harmonic coefficient of a dilute suspension of coated spherical particles. It is assumed that the coating material, but not the core or the host, has a nonlinear susceptibility for…

Disordered Systems and Neural Networks · Physics 2009-11-10 P. M. Hui , C. Xu , D. Stroud

In addition to their strong nonlinear optical response, transition metal dichalcogenides (TMDCs) possess a high refractive index in the visible and infrared regime. Therefore, by patterning those TMDCs into dielectric nanoresonators, one…

Second-harmonic-generation (SHG) in centrosymmetric material such as Si(111) is usually understood either from the phenomenology theory or more recently using the Simplified Bond-Hyperpolarizability Model (SBHM) [G. D. Powell, J. F. Wang,…

Materials Science · Physics 2015-06-12 Hendradi Hardhienata , Andrii Prylepa , David Stifter , Kurt Hingerl

Second-order nonlinear optical responses, including photogalvanic effect (PGE) and second harmonic generation (SHG), are important physical phenomena in nonlinear optics. The PGE (SHG) related to linearly and circularly polarized light are…

Mesoscale and Nanoscale Physics · Physics 2023-06-01 Yuan Liu , Zhen-Gang Zhu , Gang Su

We demonstrate supermode-based second harmonic generation in an integrated nonlinear interferometer made of linear and nonlinear directional couplers. We use a fully-fibered pump shaper to demonstrate second harmonic generation pumped by…

Comparative analysis of second harmonic generation in ordinary and backward-wave settings is presented. Extraordinary properties of frequency doubling nonlinear optical reflectivity and pulse shaping through phase matching of ordinary and…

Optics · Physics 2016-02-02 Alexander K. Popov , Sergey A. Myslivets

We experimentally study the optical second harmonic generation (SHG) from deep subwavelength gold-silver heterodimer and silver-silver and gold-gold homodimers. Our results show that the SHG from the heterodimer is about an order of…

High-order harmonic generation (HHG) in solids has emerged as a versatile platform for exploring ultrafast and quantum-coherent phenomena in condensed matter. Recent advances reveal Berry-phase and topological effects in harmonic emission,…

Optics · Physics 2025-10-20 Marcelo F. Ciappina

The majority of sources of coherent optical radiation rely on laser oscillators driven by population inversion. Despite their technological importance in communications, medicine, industry, and other fields, it remains a challenge to access…

Optics · Physics 2021-10-22 Lamia Ateshian , Hyeongrak Choi , Mikkel Heuck , Dirk Englund

We study optical harmonic generation on the 1S exciton-polariton in the semiconductor ZnSe. Intense and spectrally narrow exciton resonances are found in optical second (SHG), third (THG), and fourth (FHG) harmonic generation spectra. The…

Optics · Physics 2020-07-29 Johannes Mund , Dmitri R. Yakovlev , Marina A. Semina , Manfred Bayer

We study the second-harmonic generation in left-handed metamaterials with a quadratic nonlinear response. We demonstrate a novel type of the exact phase matching between the backward propagating wave of the fundamental frequency and the…

Optics · Physics 2009-11-11 Ilya V. Shadrivov , Alexander A. Zharov , Yuri S. Kivshar

Nonlinear metamaterials show potential for realizing flat nonlinear optical devices but generally lack in terms of achievable conversion efficiencies. Recent work has focused on enhancing nonlinear processes by utilizing high quality factor…

Notwithstanding its long history, the study of nonlinear optics from metal surfaces is still an active field of research. For instance, in view of the presence of absorption questions remain concerning the possibility of significantly…

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