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We present molecular dynamics (MD) simulations results for dense fluids of ultrasoft, fully-penetrable particles. These are a binary mixture and a polydisperse system of particles interacting via the generalized exponential model, which is…

Soft Condensed Matter · Physics 2012-12-24 Daniele Coslovich , Marco Bernabei , Angel J. Moreno

We use molecular dynamics computer simulations to investigate the local motion of the particles in a supercooled simple liquid. Using the concept of the distance matrix we find that the alpha-relaxation corresponds to a small number of…

Disordered Systems and Neural Networks · Physics 2015-06-25 G. A. Appignanesi , J. A. Rodriguez Fris , R. A. Montani , W. Kob

We review recent developments in structural-dynamical phase transitions in trajectory space. An open question is how the dynamic facilitation theory of the glass transition may be reconciled with thermodynamic theories that posit a…

Statistical Mechanics · Physics 2020-08-04 C. Patrick Royall , Francesco Turci , Thomas Speck

A large-scale molecular dynamics simulation is performed on a glass-forming Lennard-Jones mixture to determine the nature of dynamical heterogeneities which arise in this model fragile liquid. We observe that the most mobile particles…

Disordered Systems and Neural Networks · Physics 2009-10-30 Claudio Donati , Jack F. Douglas , Walter Kob , Steven J. Plimpton , Peter H. Poole , Sharon C. Glotzer

We numerically investigate slow dynamics of a binary mixture of ultrasoft particles interacting with the generalized Hertzian potential. If the softness parameter, $\alpha$, is small, the particles at high densities start penetrating each…

Soft Condensed Matter · Physics 2019-03-27 Ryoji Miyazaki , Takeshi Kawasaki , Kunimasa Miyazaki

The existence of heterogeneity in the dynamics of supercooled liquids is believed to be one of the hallmarks of the glass transition. Intense research has been carried out in the past to understand the origin of this heterogeneity in…

Soft Condensed Matter · Physics 2020-07-01 Indrajit Tah , Smarajit Karmakar

For a large class of fluids exhibiting ultrasoft bounded pair potentials, particles form crystals consisting of clusters located in the lattice sites, with a density-independent lattice constant. Here we present an investigation on the…

Soft Condensed Matter · Physics 2009-11-13 Angel J. Moreno , Christos N. Likos

One of the central problems of the liquid-glass transition is whether there is a structural signature that can qualitatively distinguish different dynamic behaviors at different degrees of supercooling. Here, we propose a novel structural…

Soft Condensed Matter · Physics 2015-09-24 Yan-Wei Li , You-Liang Zhu , Zhao-Yan Sun

The relaxation properties of viscous liquids close to their glass transition (GT) have been widely characterised by the statistical tool of time correlation functions. However, the strong influence of ubiquitous non-linearities calls for…

Soft Condensed Matter · Physics 2021-09-14 Antonio Tripodo , Francesco Puosi , Marco Malvaldi , Dino Leporini

We present simulation results addressing the dynamics of a colloidal system with attractive interactions close to gelation. Our interaction also has a soft, long range repulsive barrier which suppresses liquid-gas type phase separation at…

Soft Condensed Matter · Physics 2007-05-23 Antonio M. Puertas , Matthias Fuchs , Michael E. Cates

We study the hydrodynamic interactions between colloids suspended in a compressible fluid inside a rigid channel. Using lattice-Boltzmann simulations and a simplified hydrodynamic theory, we find that the diffusive dynamics of density…

Soft Condensed Matter · Physics 2013-02-13 Derek Frydel , Haim Diamant

We prove the emergence of spatially correlated dynamics in slowly compacting dense granular media by analyzing analytically and numerically multi-point correlation functions in a simple particle model characterized by slow non-equilibrium…

Statistical Mechanics · Physics 2009-11-10 Alexandre Lefèvre , Ludovic Berthier , Robin Stinchcombe

Using molecular dynamics simulations we study the slow dynamics of a hard sphere fluid confined in a disordered porous matrix. The presence of both discontinuous and continuous glass transitions as well as the complex interplay between…

Soft Condensed Matter · Physics 2009-09-29 Jan Kurzidim , Daniele Coslovich , Gerhard Kahl

Structural relaxation in binary hard spherical particles has been shown recently to exhibit a wealth of remarkable features when size disparity or mixture's composition is varied. In this paper, we test whether or not similar dynamical…

Soft Condensed Matter · Physics 2014-12-03 Wen-Sheng Xu , Zhao-Yan Sun , Li-Jia An

The interaction between passive and active/driven particles has introduced a new way to control colloidal suspension properties from particle aggregation to crystallization. Here, we focus on the hydrodynamic interaction between a single…

Soft Condensed Matter · Physics 2024-02-07 Shih-Yuan Chen , Hector Lopez-Rios , Monica Olvera de la Cruz , Michelle M. Driscoll

We study the role of hydrodynamic interactions in the collective behaviour of collections of microscopic active particles suspended in a fluid. We introduce a novel calculational framework that allows us to separate the different…

Soft Condensed Matter · Physics 2017-09-06 Natsuhiko Yoshinaga , Tanniemola B. Liverpool

We study a colloidal suspension confined between two quasi-parallel walls as a model system for glass transitions in confined geometries. The suspension is a mixture of two particle sizes to prevent wall-induced crystallization. We use…

Soft Condensed Matter · Physics 2007-08-09 Carolyn R. Nugent , Kazem V. Edmond , Hetal N. Patel , Eric R. Weeks

We compare the slow dynamics of irreversible gels, colloidal gels, glasses and spin glasses by analyzing the behavior of the so called non-linear dynamical susceptibility, a quantity usually introduced to quantitatively characterize the…

Soft Condensed Matter · Physics 2015-06-25 A. Coniglio , T. Abete , A. de Candia , E. Del Gado , A. Fierro

We study aging in a colloidal suspension consisting of micron-sized particles in a liquid. This system is made glassy by increasing the particle concentration. We observe samples composed of particles of two sizes, with a size ratio of…

Soft Condensed Matter · Physics 2008-10-02 Jennifer M. Lynch , Gianguido C. Cianci , Eric R. Weeks

The slow dynamics in a glassy hard-sphere system is dominated by cage breaking events, i.e., rearrangements where a particle escapes from the cage formed by its neighboring particles. We study such events for an overdamped colloidal system…

Soft Condensed Matter · Physics 2016-10-26 Matthias Kohl , Andreas Härtel , Michael Schmiedeberg
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