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We investigate the behavior of a patchy particle model close to a hard-wall via Monte Carlo simulation and density functional theory (DFT). Two DFT approaches, based on the homogeneous and inhomogeneous versions of Wertheim's first order…

We calculate density profiles of a simple model fluid in contact with a planar surface using density functional theory (DFT), in particular for the case where there is a vapour layer intruding between the wall and the bulk liquid. We apply…

Soft Condensed Matter · Physics 2019-04-16 Hanyu Yin , David N. Sibley , Andrew J. Archer

We look at the wetting of a pure fluid in contact with a charged flat surface. In the bulk, the fluid is a classical van der Waals fluid containing dissociated ions. The presence of wall and ions leads to strong dielectrophoretic and…

Statistical Mechanics · Physics 2021-11-16 Yoav Tsori

I use the method of classical density-functional theory in the weighted-density approximation of Tarazona to investigate the phase diagram and the interface structure of a two-dimensional lattice-gas model with three phases -- vapour,…

Statistical Mechanics · Physics 2009-11-10 S. Prestipino

We consider fluid wetting on a corrugated substrate using effective interfacial Hamiltonian theory and show that breaking the translational invariance along the wall can induce an 'unbending' phase transition in addition to unbinding. Both…

Soft Condensed Matter · Physics 2009-10-31 C. Rascon , A. O. Parry , A. Sartori

A simple two dimensional model of a phase growing on a substrate is introduced. The model is characterized by an adsorption rate q, and a desorption rate p. It exhibits a wetting transition which may be viewed as an unbinding transition of…

Statistical Mechanics · Physics 2009-10-30 Haye Hinrichsen , Roberto Livi , David Mukamel , Antonio Politi

Depinning of an interface from a random self--affine substrate with roughness exponent $\zeta_S$ is studied in systems with short--range interactions. In 2$D$ transfer matrix results show that for $\zeta_S<1/2$ depinning falls in the…

Condensed Matter · Physics 2009-10-28 G. Giugliarelli , A. L. Stella

As a first step towards a microscopic understanding of the effective interaction between colloidal particles suspended in a solvent we study the wetting behavior of one-component fluids at spheres and fibers. We describe these phenomena…

Condensed Matter · Physics 2015-06-25 T. Bieker , S. Dietrich

Hydrodynamic density functional theory (DFT) is applied to analyse dynamic contact angles of droplets in order to assess its predictive capability regarding wetting phenomena at the microscopic scale and to evaluate its feasibility for…

Fluid Dynamics · Physics 2025-08-06 Benjamin Bursik , Rolf Stierle , Hamza Oukili , Martin Schneider , Gernot Bauer , Joachim Gross

We have carried out extensive equilibrium molecular dynamics (MD) simulations to study the structure and the interfacial properties in the liquid-vapor (LV) phase coexistence of partially miscible binary Lennard-Jones (LJ) mixtures. By…

Soft Condensed Matter · Physics 2009-11-10 Enrique Díaz-Herrera , José A. Moreno-Razo , Guillermo Ramírez-Santiago

We numerically and experimentally investigate evaporation of a sessile droplet on a heated substrate. We develop a finite element (FE) model in two-dimensional axisymmetric coordinates to solve coupled transport of heat in the droplet and…

Applied Physics · Physics 2019-07-15 Manish Kumar , Rajneesh Bhardwaj

Our understanding of both structure and dynamics of adsorbed liquids heavily relies on the capillary wave Hamiltonian, but a thorough test of this model is still lacking. Here we study the capillary wave fluctuations of a liquid film with…

Soft Condensed Matter · Physics 2013-09-06 Luis G. MacDowell , Jorge Benet , Nebil A. Katcho

Fundamental properties of the multicomponent diffuse-interface model (DIM), such as the maximum entropy principle and conservation laws, are used to explore the basic interfacial dynamics and phase transitions in fluids. Flat interfaces…

Fluid Dynamics · Physics 2023-05-02 E. S. Benilov

Mean field analysis of the effective interfacial Hamiltonian shows that with increasing temperature the adsorption on a periodically corrugated substrate can proceed in two steps: first, there is the filling transition in which the…

Statistical Mechanics · Physics 2009-10-31 K. Rejmer , M. Napiorkowski

We present numerical studies of complete, first-order and critical wedge filling transitions, at a right angle corner, using a microscopic fundamental measure density functional theory. We consider systems with short-ranged, cut-off…

Statistical Mechanics · Physics 2015-06-16 Alexandr Malijevsky , Andrew O Parry

The finite element simulation of dynamic wetting phenomena, requiring the computation of flow in a domain confined by intersecting a liquid-fluid free surface and a liquid-solid interface, with the three-phase contact line moving across the…

Computational Physics · Physics 2012-02-20 J. E. Sprittles , Y. D. Shikhmurzaev

The dihedral contact angles between interfaces in three-fluid-phase equilibria must be continuous functions of the bulk thermodynamic fields. This general argument, which we propose, predicts a nonwetting gap in the phase diagram,…

Statistical Mechanics · Physics 2022-12-07 Joseph O. Indekeu , Kenichiro Koga

Heterogeneous condensation of vapours mixed with a carrier gas in the stagnation point boundary layer flow near a cold wall is considered in the presence of solid particles much larger than the mean free path of vapour particles. The…

Other Condensed Matter · Physics 2009-07-22 J. C. Neu , A. Carpio , L. L. Bonilla

Simulations of water near extended hydrophobic spherical solutes have revealed the presence of a region of depleted density and accompanying enhanced density fluctuations.The physical origin of both phenomena has remained somewhat obscure.…

Soft Condensed Matter · Physics 2023-02-01 Mary K. Coe , Robert Evans , Nigel B. Wilding

We investigate the properties of water along the liquid/vapor coexistence line in the supercooled regime down to the no-man's land. Extensive molecular dynamics simulations of the TIP4P/2005 liquid/vapor interface in the range 198 -- 348 K…

Soft Condensed Matter · Physics 2023-02-15 Alexander Gorfer , Christoph Dellago , Marcello Sega