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The pyrochlore iridates R2Ir2O7 have emerged as a unique playground for exploring exotic quantum phenomena arising from the intricate interplay of strong spin-orbit coupling, electron correlations, and geometric frustration. While bulk…

Strongly Correlated Electrons · Physics 2026-05-27 Xiaoran Liu , Michael Terilli , Ana-Marija Nedic , Jiandong Guo , Jak Chakhalian

We report a single-crystal neutron diffraction study of the layered $\rm Sr_2IrO_4$. This work unambiguously determines the magnetic structure of the system and reveals that the spin orientation rigidly tracks the staggered rotation of the…

Strongly Correlated Electrons · Physics 2013-04-23 Feng Ye , Songxue Chi , Bryan C. Chakoumakos , Jaime A. Fernandez-Baca , Tongfei Qi , G. Cao

Bulk studies have revealed a first-order valence phase transition in Ba$_2$PrRu$_{1-x}$Ir$_x$O$_6$ ($0.10 \le x \le 0.25$), which is absent in the parent compounds with $x = 0$ (Pr$^{3+}$) and $x =1$ (Pr$^{4+}$), which exhibit…

We report the observation of metal-like to insulator transition (MTI) in the 3dpyrochlore oxide Tb2Ti2O7 at 603 K due to the interaction of empty 3d orbitals of Ti4+ with O2- ions, evidenced by the transition in resistivity. Magnetisation,…

Materials Science · Physics 2020-07-28 B. Santhosh Kumar , C. Venkateswaran

We investigate the metal-insulator transition (MIT) of the osmium pyrochlore oxide Cd2Os2O7 through transport and magnetization measurements. The MIT and a magnetic transition to the all-in/all-out (AIAO) order occur simultaneously at 227…

Strongly Correlated Electrons · Physics 2015-02-03 Z. Hiroi , J. Yamaura , T. Hirose , I. Nagashima , Y. Okamoto

We have studied the effect of nonmagnetic Ti substitution Eu2(Ir1-xTix)2O7 with the help of electrical transport and magnetic measurement. The minor structural modification enhances the orbital overlapping and favours its electrical…

Strongly Correlated Electrons · Physics 2024-07-09 Sampad Mondal , B. Maji , M. Modak , Swapan K. Mandal , S. Banerjee

The consequences of nonmagnetic-ion dilution for the pyrochlore family Y$_{2}$($M_{1-x}N_{x}$)$_{2}$O$_{7}$ ($M$ = magnetic ion, $N$ = nonmagnetic ion) have been investigated. As a first step, we experimentally examine the magnetic…

Strongly Correlated Electrons · Physics 2017-10-04 L. Shen , C. Greaves , R. Riyat , T. C. Hansen , E. Blackburn

Sr2IrO4 exhibits a novel insulating state assisted by spin-orbit interactions. A series of polycrystalline samples of Sr2-xIrO4 have been synthesized. It is found that deep Sr-vacancies of Sr2-xIrO4 greatly reduce the rotation of IrO6…

Strongly Correlated Electrons · Physics 2016-11-01 Xuanyong Sun , S. L. Liu , Haiyun Wang , Bin Li , Jie Cheng , Z. H. Wang

We report a detailed study of structural and magnetic properties of the pyrochlore-type (Bi2-xPrx)Ru2O7 series. Eleven compositions with 0 <= x <= 2 were prepared by solid state reaction at 1050 degrees C and found to form a solid solution…

Materials Science · Physics 2008-12-16 Siwar Zouari , Rafik Ballou , Abdelwaheb Cheikh-Rouhou , Pierre Strobel

The dispersion of the low-energy magnetic excitations of the Pr sublattice in PrBa2Cu3O6.2 is determined by inelastic neutron scattering measurements on a single crystal. The dispersion, which shows the effect of interactions with the Cu…

Recent experiments in the original cuprate high temperature superconductor, La$_2-x$Ba$_x$CuO$_4$, have revealed a remarkable sequence of transitions [1]. Here we investigate such crystals with Kerr effect which is sensitive to…

Superconductivity · Physics 2012-10-10 Hovnatan Karapetyan , M. Hucker , G. D. Gu , J. M. Tranquada , M. M. Fejer , Jing Xia , A. Kapitulnik

The 5d pyrochlore oxide superconductor Cd2Re2O7 (CRO) has attracted significant interest as a spin-orbit-coupled metal (SOCM) that spontaneously undergoes a phase transition to an odd-parity multipole phase by breaking the spatial inversion…

Strongly Correlated Electrons · Physics 2023-09-18 Daigorou Hirai , Atsuhito Fukui , Hajime Sagayama , Takumi Hasegawa , Zenji Hiroi

Magnetic-rare-earth pyrochlore iridates exhibit a rich variety of unconventional phases, driven by the complex interactions within and between the rare-earth and the iridium sublattices. In this study, we investigate the peculiar magnetic…

Strongly Correlated Electrons · Physics 2026-01-05 Y. Alexanian , E. Lhotel , J. Robert , S. Petit , E. Lefrançois , P. Lejay , A. Hadj-Azzem , F. Damay , J. Ollivier , B. Fåk , R. Ballou , S. De Brion , V. Simonet

The compound, Nd7Rh3, crystallizing in Th7Fe3-type hexagonal structure, has been shown recently by us to exhibit a signature of magnetic phase-coexistence phenomenon below 10 K after a field cycling, uncharacteristic of stoichiometric…

Strongly Correlated Electrons · Physics 2009-11-11 Kausik Sengupta , E. V. Sampathkumaran

The optical properties of a V4O7 single crystal have been investigated from the high temperature metallic phase down to the low temperature antiferromagnetic insulating one. The temperature dependent behavior of the optical conductivity…

Strongly Correlated Electrons · Physics 2015-06-22 I. Lo Vecchio , M. Autore , F. D'Apuzzo , F. Giorgianni , A. Perucchi , U. Schade , V. N. Andreev , V. A. Klimov , S. Lupi

An intriguing idea of spin-orbit Mott insulator has been proposed to explain magnetic insulating behavior in various iridates. This scenario relies on the strength of the spin-orbit coupling being comparable to electronic correlations, and…

Strongly Correlated Electrons · Physics 2013-05-30 Jean-Michel Carter , Hae-Young Kee

Neutron diffraction is used to examine the polarization of weak static antiferromagnetism in high quality single crystalline URu2Si2. As previously documented, elastic Bragg-like diffraction develops for temperature T<T_{HO}= 17.5 K at…

Strongly Correlated Electrons · Physics 2015-06-18 K. A. Ross , L. Harriger , Z. Yamani , W. J. L. Buyers , J. D. Garrett , A. A. Menovsky , J. A. Mydosh , C. L. Broholm

We study the prototype 5d pyrochlore iridate Y2Ir2O7 from first principles using the local density approximation and dynamical mean-field theory (LDA+DMFT). We map out the phase diagram in the space of temperature, onsite Coulomb repulsion…

Strongly Correlated Electrons · Physics 2015-10-14 Hiroshi Shinaoka , Shintaro Hoshino , Matthias Troyer , Philipp Werner

Full pattern Le-Bail refinement using x-ray powder diffraction profiles of Sr1-xCaxTiO3 for x=0.02, 0.04 in the temperature range 12 to 300 K reveals anomalies in the unit cell parameters at 170, 225 K due to an antiferrodistortive (cubic…

Materials Science · Physics 2015-05-13 Sanjay Kumar Mishra , Dhananjai Pandey

We investigate the effect of partial replacement of extended 5d Ir4+ sites by localized 3d Cr3+ moments on the magnetocaloric properties of Y2Ir2O7 (YIO) pyrochlore iridates. We find that Y2Ir2-xCrxO7 (YICO) undergoes cluster glass…

Strongly Correlated Electrons · Physics 2021-10-08 Vinod Kumar Dwivedi , Prabhat Mandal , Soumik Mukhopadhyay