English
Related papers

Related papers: Dynamic orbitals in high-harmonic generation from …

200 papers

We explore the impact of optical excitation using two interfering ultrashort optical pulses on ultrafast magnetization dynamics. Our investigation focuses on Pt/Co/Pt multilayers and TbCo alloy samples, employing a dual pump approach. We…

Attosecond pulses created by high-order harmonic generation in gases often exhibit strong chromatic aberrations, arising from the broad bandwidth and wavelength-dependent nonlinear light-matter interaction. When the driving laser intensity…

Because molecules can have their orientation locked when embedded into a solid rare-gas matrix, their hyperfine structure is strongly perturbed relative to the freely rotating molecule. The addition of an electric field further perturbs the…

Atomic Physics · Physics 2018-10-03 A. C. Vutha , M. Horbatsch , E. A. Hessels

We discuss harmonic generation in the case of laser field-dressed Hamiltonians that are invariant under so-called dynamical symmetry operations. Examples for such systems are molecules which exhibit a discrete rotational symmetry of order N…

Atomic Physics · Physics 2016-09-08 F. Ceccherini , D. Bauer , F. Cornolti

On the basis of real-time ab initio calculations, we study the non-perturbative interaction of two-color laser pulses with MgO crystal in the strong field regime to generate isolated attosecond pulse from high-harmonic emissions from MgO…

This paper presents the method for the first time to generate intense high-order optical vortices that carry orbital angular momentum in the extreme ultraviolet region. In three-dimensional particle-in-cell simulation, both the reflected…

Intense attosecond magnetic field pulses are predicted to be produced by intense few cycle circularly polarized UV pulses. Numerical solutions of the time dependent Schr\"{o}dinger equation for H$_2^+$ are used to study the dynamical…

Optics · Physics 2013-07-24 Kai-Jun Yuan , Andre D. Bandrauk

We discuss the influence of periodic orbits on the dissociation of a model diatomic molecule driven by a strong bichromatic laser fields. Through the stability of periodic orbits we analyze the dissociation probability when parameters like…

Chaotic Dynamics · Physics 2009-11-13 S. Huang , C. Chandre , T. Uzer

We present a theoretical study of the impact of an electrostatic field combined with non-resonant linearly polarized laser pulses on the rotational dynamics of linear molecules. Within the rigid rotor approximation, we solve the…

Atomic Physics · Physics 2015-06-05 Juan J. Omiste , Rosario González-Férez

We find that, for sufficiently strong mid-IR fields, transitions between different conduction bands play an important role in the generation of high-order harmonics in a dielectric. The transitions make a significant contribution to the…

Other Condensed Matter · Physics 2015-06-22 Peter G. Hawkins , Misha Yu. Ivanov , Vladislav S. Yakovlev

We study the role of transition rule in high-order harmonic generation from solids driven by linearly polarized laser elds. The orientation-dependent transition dipoles can regulate the emergence of the multi-plateau structure. In the…

Optics · Physics 2019-03-07 Tao-Yuan Du , Si-Jing Ding

Various methods of obtaining longitudinally polarized positrons for future linear colliders are reviewed. Special attention is paid to the schemes using circularly polarized high-energy photons for positron production. Most effectively such…

High Energy Physics - Phenomenology · Physics 2009-11-10 V. Strakhovenko , X. Artru , R. Chehab , M. Chevallier

Inducing and controlling the ultrafast molecular rotational dynamics using shaped laser fields is essential in numerous applications. Several approaches exist that allow following the coherent molecular motion in real-time, including…

We develop a new model of laser-matter interaction based on Optical Bloch Equations, which includes photo-ionization, impact ionization, and various relaxation processes typical of dielectric materials. This approach is able to describe the…

Coulomb interactions that occur in electronic structure calculations are correlated by allowing basis function components of the interacting densities to polarize, thereby reducing the magnitude of the interaction. Exchange integrals of…

Chemical Physics · Physics 2022-05-16 Jerry L. Whitten

We study high-order harmonic generation in aligned molecules close to the ionization threshold. Two distinct contributions to the harmonic signal are observed, which show very different responses to molecular alignment and ellipticity of…

Atomic Physics · Physics 2011-09-16 H. Soifer , P. Botheron , D. Shafir , A. Diner , O. Raz , B. D. Bruner , Y. Mairesse , B. Pons , N. Dudovich

We report the first experimental observation of non-adiabatic field-free orientation of a heteronuclear diatomic molecule (CO) induced by an intense two-color (800 and 400 nm) femtosecond laser field. We monitor orientation by measuring…

The interaction of a helium atom with intense short 800 nm laser pulse is studied theoretically beyond the single-active-electron approximation. For this purpose, the time-dependent Schr\"odinger equation for the two-electron wave packet…

Atomic and Molecular Clusters · Physics 2017-03-08 Anton N. Artemyev , Lorenz S. Cederbaum , Philipp V. Demekhin

In this work using three-dimensional particle-in-cell simulations and analytical considerations we demonstrate intense high-order plasma surface harmonics carrying a time-varying orbital angular momentum (OAM) -- the self-torque. We show…

Plasma Physics · Physics 2022-01-03 Jingwei Wang , Matt Zepf , Yuxin Leng , Ruxin Li , Sergey G. Rykovanov

This work theoretically investigates high-order harmonic generation in rare gas atoms driven by two temporally delayed ultrashort laser pulses. Apart from their temporal delay, the two pulses are identical. Using a single-atom model of the…