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Over the last few decades, classical density-functional theory (DFT) and its dynamic extensions (DDFTs) have become powerful tools in the study of colloidal fluids. Recently, previous DDFTs for spherically-symmetric particles have been…

Statistical Mechanics · Physics 2016-08-02 Miguel A. Durán-Olivencia , Benjamin D. Goddard , Serafim Kalliadasis

Density functional theory (DFT), the most widely adopted method in modern computational chemistry, fails to describe accurately the electronic structure of strongly correlated systems. Here we show that DFT can be formally and practically…

Chemical Physics · Physics 2022-04-18 Daniel Gibney , Jan-Niklas Boyn , David A. Mazziotti

Transport properties of dense fluids are fundamentally challenging, because the powerful approaches of equilibrium statistical physics cannot be applied. Polar fluids compound this problem, because the long-range interactions preclude the…

Soft Condensed Matter · Physics 2020-06-16 Faezeh Pousaneh , Astrid S. de Wijn

The superadiabatic dynamical density functional theory (superadiabatic-DDFT) is a promising new method for the study of colloidal systems out-of-equilibrium. Within this approach the viscous forces arising from interparticle interactions…

Soft Condensed Matter · Physics 2024-06-10 S. M. Tschopp , J. M. Brader

Quantum-chemical processes in liquid environments impact broad areas of science, from molecular biology to geology to electrochemistry. While density-functional theory (DFT) has enabled efficient quantum-mechanical calculations which…

Chemical Physics · Physics 2017-10-16 Kendra Letchworth-Weaver , Ravishankar Sundararaman , T. A. Arias

We analyze theoretically a high-speed drainage of liquid films squeezed between a hydrophilic sphere and a textured super-hydrophobic plane, that contains trapped gas bubbles. A super-hydrophobic wall is characterized by parameters $L$…

Fluid Dynamics · Physics 2014-01-23 Evgeny S. Asmolov , Aleksey V. Belyaev , Olga I. Vinogradova

We propose an in-silico experiment to introduce classical density functional theory (cDFT). Den- sity functional theories, whether quantum or classical, rely on abstract concepts that are non- intuitive. However, they are at the heart of…

Chemical Physics · Physics 2014-10-16 Guillaume Jeanmairet , Nicolas Levy , Maximilien Levesque , Daniel Borgis

We investigate theoretically the morphology of a thin nematic film adsorbed at flat substrate patterned by stripes with alternating aligning properties, normal and tangential respectively. We construct a simple "exactly-solvable" effective…

Soft Condensed Matter · Physics 2017-02-01 Nuno M. Silvestre , Margarida M. Telo da Gama , Mykola Tasinkevych

The vertical transport of solid material in a stratified medium is fundamental to a number of environmental applications, with implications for the carbon cycle and nutrient transport in marine ecosystems. In this work, we study the…

Fluid Dynamics · Physics 2024-09-05 Robert Hunt , Roberto Camassa , Richard M. McLaughlin , Daniel M. Harris

The journey of theoretical study on semiconductors is reviewed in a non-conventional way. We have started with the basic introduction of Hartree-Fock method and introduce the fundamentals of Density Functional Theory (DFT). From the oldest…

Materials Science · Physics 2021-05-04 Sujoy Datta , Debnarayan Jana

In this paper, a new method to model solidification of thin liquid films is proposed. \blue{This method is targeted at applications like aircraft icing and tablet coating where the formation of liquid films from impinging droplets on a…

Fluid Dynamics · Physics 2024-04-11 Anand S Bharadwaj , Elisa Thiel , Pratik Suchde

The freezing transition of hard spheres has been well described by various versions of density-functional theory (DFT). These theories should possess the close-packed crystal as a special limit, which represents an extreme testing ground…

Soft Condensed Matter · Physics 2009-10-31 Benito Groh , Bela Mulder

We consider the deposition of a film of viscous liquid on a flat plate being withdrawn from a bath, experimentally and theoretically. For any plate speed $U$, there is a range of ``thick'' film solutions whose thickness scales like…

Fluid Dynamics · Physics 2008-03-28 J. H. Snoeijer , J. Ziegler , B. Andreotti , M. Fermigier , J. Eggers

Density functional theory (DFT) provides a theoretical framework for efficient and fairly accurate calculations of the electronic structure of molecules and crystals. The main features of density functional theory are described and DFT…

Chemical Physics · Physics 2012-06-12 Hauke Paulsen , Alfred Xaver Trautwein

A thin liquid film covered with an insoluble surfactant in the vicinity of a first-order phase transition is discussed. Within the lubrication approximation we derive two coupled equations to describe the height profile of the film and the…

Pattern Formation and Solitons · Physics 2009-07-15 M. H. Köpf , S. V. Gurevich , R. Friedrich

The structural and interfacial properties of a nanoscopic liquid drops are assessed by means of mechanical, thermodynamical, and statistical mechanical approaches that are discussed in detail, including original developments at both the…

Soft Condensed Matter · Physics 2012-11-12 Alexandr Malijevsky , George Jackson

Classical density functional theory (DFT) of fluids is a valuable tool to analyze inhomogeneous fluids. However, few numerical solution algorithms for three-dimensional systems exist. Here we present an efficient numerical scheme for fluids…

The DFT/vdW-WF2s1 method based on the generation of localized Wannier functions, recently developed to include the van der Waals interactions in the Density Functional Theory and describe adsorption processes on metal surfaces by taking…

Chemical Physics · Physics 2016-04-06 Pier Luigi Silvestrelli , Alberto Ambrosetti

Linear scaling density functional theory approaches to electronic structure are often based on the tendency of electrons to localize even in large atomic and molecular systems. However, in many cases of actual interest, for example in…

Chemical Physics · Physics 2022-03-25 Marcel David Fabian , Ben Shpiro , Roi Baer

Several model fluids in contact with planar, spherical, and cylindrical walls are investigated for small number densities within density functional theory. The dependence of the solid-fluid interfacial tension on the curvature of spherical…

Statistical Mechanics · Physics 2015-05-05 Andreas Reindl , Markus Bier , S. Dietrich