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The thermoelectric properties of a molecular junction model, appropriate for large molecules such as fullerenes, are studied within a non-equilibrium adiabatic approach in the linear regime at room temperature. A self-consistent calculation…

Mesoscale and Nanoscale Physics · Physics 2014-09-26 C. A. Perroni , D. Ninno , V. Cataudella

Superconducting resonators used in millimeter-submillimeter astronomy would greatly benefit from deposited dielectrics with a small dielectric loss. We deposited hydrogenated amorphous silicon films using plasma-enhanced chemical vapor…

Instrumentation and Methods for Astrophysics · Physics 2023-02-03 Bruno T. Buijtendorp , Juan Bueno , David J. Thoen , Vignesh Murugesan , Paolo M. Sberna , Jochem J. A. Baselmans , Sten Vollebregt , Akira Endo

Molecular beam experiments that use low-temperature bolometers as (energy-) detectors are well suited to the study of physisorption and recombination of hydrogen on low-temperature surfaces. Experiments where this technique is combined with…

Chemical Physics · Physics 2007-05-23 Thomas Govers

The negatively charged boron-vacancy center ($\mathrm{V}_{\mathrm{B}}^-$) in hexagonal boron nitride (hBN) has recently emerged as a highly promising quantum sensor. Compared to the nitrogen-vacancy (NV) center in diamond, the change with…

Using a recently developed thermodynamic integration method, we compute the precise values of the excess Gibbs free energy (G^e) of the high density liquid (HDL) phase with respect to the crystalline phase at different temperatures (T) in…

Statistical Mechanics · Physics 2012-11-13 Pankaj A. Apte , Arvind K. Gautam

The vibrational dynamics of adsorbate molecules in single-molecule junctions depend critically on the geometric structure and electronic interactions between molecule and substrate. Vibrations, excited mechanochemically or by external…

Mesoscale and Nanoscale Physics · Physics 2025-09-17 Lukas Hörmann , Reinhard J. Maurer

Atomic hydrogen energy levels calculated to high precision are required to assist experimental researchers working on spectroscopy in the pursuit of testing quantum electrodynamics (QED) and probing for physics beyond the Standard Model.…

Atomic Physics · Physics 2023-09-12 David M. Jacobs , Marko Horbatsch

Adsorption in nanoporous materials is one strategy that can be used to store hydrogen at conditions of temperature and pressure that are economically viable. Adsorption capacity of nanoporous materials depends on surface area which can be…

Materials Science · Physics 2024-05-28 Siddharth Gautam , David R. Cole , Zoltán Imre Dudás , Indu Dhiman

Specific heat measurements of hydrogenated amorphous silicon prepared by hot-wire chemical vapor deposition show a large density of two-level systems at low temperature. Annealing at 200 {\deg}C, well below the growth temperature, does not…

Materials Science · Physics 2021-07-21 M. Molina-Ruiz , H. C. Jacks , D. R. Queen , T. H. Metcalf , X. Liu , F. Hellman

The adsorption and diffusion of hydrogen atoms on Cu(001) are studied using first-principles calculations. By taking into account the contribution of zero-point energy (ZPE), the originally identical barriers are shown to be different for H…

Mesoscale and Nanoscale Physics · Physics 2023-06-09 Xiaofan Yu , Yangwu Tong , Yong Yang

Vibrational properties of iron-chalcogenide superconductor K$_{0.75}$Fe$_{1.75}$Se$_{2}$ with $T_{c}\sim$ 30 K have been measured by Raman and optical spectroscopies over temperature range of 3-300 K. Sample undergoes \textit{I4/m} $\to $…

Superconductivity · Physics 2015-06-11 A. Ignatov , A. Kumar , P. Lubik , R. H. Yuan , W. T. Guo , N. L. Wang , K. Rabe , G. Blumberg

Flexoelectricity, an electromechanical coupling between strain gradient and polarization, offers a promising dimension to enrich silicon-based devices. Although the flexoelectricity of silicon is known, some fundamental aspects remain…

Materials Science · Physics 2025-06-26 Lingtong Lv , Qianqian Ma , Kailu Wang , Xin Wen , Shengping Shen

We calculate ionization energies and fundamental vibrational transitions for H$_2^+$, D$_2^+$, and HD$^+$ molecular ions. The NRQED expansion for the energy in terms of the fine structure constant $\alpha$ is used. Previous calculations of…

Atomic Physics · Physics 2017-06-14 Vladimir I. Korobov , Laurent Hilico , Jean-Philippe Karr

The efficiency of energy conversion in thermoelectric generators (TEGs) is directly proportional to electrical conductivity and Seebeck coefficient while inversely to thermal conductivity. The challenge is to optimize these interdependent…

Carbon stopping-power (SP) data for heavy ions (HIs), obtained around Bohr velocities, revealed remarkably lower values than those predicted by the SRIM/TRIM calculations/simulations. An attempt was made to extract the elastic (collisional)…

Atomic Physics · Physics 2023-03-02 R. N. Sagaidak

In this paper we discuss the application of current it ab initio computer simulation techniques to hydrogenated amorphous silicon (a-Si:H). We begin by discussing thermal fluctuation in the number of coordination defects in the material,…

Materials Science · Physics 2009-11-13 D. A. Drabold , T. A. Abtew , F. Inam , Y. Pan

Si hyperdoped with chalcogens (S, Se, Te) is well-known to possess unique properties such as an insulator-to-metal transition and a room-temperature sub-bandgap absorption. These properties are expected to be sensitive to a post-synthesis…

Applied Physics · Physics 2019-05-01 Mao Wang , R. Hubner , Chi Xu Yufang Xie , Y. Berencen , R. Heller , L. Rebohle , M. Helm , S. Prucnal , Shengqiang Zhou

Molecular hydrogen adsorption in a nanoporous metal organic framework structure (MOF-74) was studied via van der Waals density-functional calculations. The primary and secondary binding sites for H$_2$ were confirmed. The low-lying…

Mesoscale and Nanoscale Physics · Physics 2015-05-13 Lingzhu Kong , Guillermo Román-Pérez , José M. Soler , David C. Langreth

The free energy and other thermodynamic properties of hexagonal-close-packed iron are calculated by direct {\em ab initio} methods over a wide range of pressures and temperatures relevant to the Earth's core. The {\em ab initio}…

Condensed Matter · Physics 2007-05-23 D. Alfe` , G. D. Price , M. J. Gillan

Water is an ubiquitous liquid that has several exotic and anomalous properties. Despite its apparent simple chemical formula, its capability of forming a dynamic network of hydrogen bonds leads to a rich variety of physics. Here we study…

Soft Condensed Matter · Physics 2023-08-15 R. Vuilleumier , A. P. Seitsonen