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Exciton binding energy and electron-hole recombination probability are presented as the two important metrics for investigating effect of dot size on electron-hole interaction in CdSe quantum dots. Direct computation of electron-hole…

Chemical Physics · Physics 2013-10-09 Jennifer M. Elward , Arindam Chakraborty

The electron-hole states of semiconductor quantum dots are investigated within the framework of empirical tight-binding descriptions for Si, as an example of an indirect gap material, and InAs and CdSe as examples of typical III-V and II-VI…

Condensed Matter · Physics 2009-10-31 Seungwon Lee , Lars Jonsson , John W. Wilkins , Garnett W. Bryant , Gerhard Klimeck

The region surrounding the excitonic insulator phase is a three-component plasma composed of electrons, holes, and excitons. Due to the extended nature of the excitons, their presence influences the surrounding electrons and holes. We…

Strongly Correlated Electrons · Physics 2015-06-22 B Zenker , D Ihle , F X Bronold , H Fehske

Electron-hole correlation in quantum-dot quantum wells (QDQW's) is investigated by incorporating Coulomb and exchange interactions into an empirical tight-binding model. Sufficient electron and hole single-particle states close to the band…

Materials Science · Physics 2009-11-10 Rui-Hua Xie , Garnett W. Bryant , Seungwon Lee , W. Jaskolski

We present a self-consistent treatment of the electron-hole correlations in optically excited quantum wires within the ladder approximation, and using a contact potential interaction. The limitations of the ladder approximation to the…

Condensed Matter · Physics 2009-10-31 Francesco Tassone , Carlo Piermarocchi

Using semi-analytical models we calculate the energy, effective Bohr radius and radiative lifetime of neutral excitons confined in CdSe colloidal nanoplatelets (NPLs). The excitonic properties are largely governed by the electron-hole…

Mesoscale and Nanoscale Physics · Physics 2017-08-31 Fernando Rajadell , Juan I. Climente , Josep Planelles

The effects of strong Coulomb correlations in dense three-dimensional electron-hole plasmas are studied by means of unbiased direct path integral Monte Carlo simulations. The formation and dissociation of bound states, such as excitons and…

Strongly Correlated Electrons · Physics 2009-11-13 V. S. Filinov , H. Fehske , M. Bonitz , V. E. Fortov , P. Levashov

We point out that a typical two-electron distribution function in atoms and molecules often called the intracule depends sensitively on the electron-electron repulsion which leads to the so-called Coulomb correlation. The difference between…

Atomic Physics · Physics 2020-05-13 Golam Ali Sekh , Benoy Talukdar , Supriya Chatterjee

Double layer systems where one layer has electrons and the holes are in a parallel layer a distance d away are expected to undergo excitonic condensation at low temperature. This excitonic condensate is traditionally described by a…

Strongly Correlated Electrons · Physics 2009-10-19 Christopher R. Jamell , Chang-hua Zhang , Yogesh N. Joglekar

Single-layer quantum dot gate potential causes type-II band alignment, i.e. electrostatically confines holes and repels electrons, or vice versa. Hence, the confinement of excitons in gated type II quantum dots involves a delicate balance…

Mesoscale and Nanoscale Physics · Physics 2024-06-25 Daniel Miravet , Ludmiła Szulakowska , Maciej Bieniek , Marek Korkusiński , Paweł Hawrylak

The localization length of a low energy tightly bound electron-hole pair (excitons) is calculated by exact diagonalization for small interacting disordered systems. The exciton localization length (which corresponds to the thermal…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 Richard Berkovits

The optical spectra of CdSe nanocrystals up to 55 A in diameter are analyzed in a wide range of energies from the fine structure of the low-energy excitations to the so-called high-energy transitions. We apply a symmetry-based method in two…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 J. Perez-Conde , A. K. Bhattacharjee

In density functional theory the exchange-correlation (XC) energy functional can be defined exactly through the coupling-constant ($\lambda$) averaged XC hole $\bar{n}_\text{xc}(\mathbf{r},\mathbf{r}')$, representing the probability…

Chemical Physics · Physics 2023-03-31 Lin Hou , Tom J. P. Irons , Yanyong Wang , James W. Furness , Andrew M. Teale , Jianwei Sun

We show that electron-hole correlation can be used to tune interband and intraband optical transition rates in semiconductor nanostructures with at least one weakly confined direction. The valence-to-conduction band transition rate can be…

Mesoscale and Nanoscale Physics · Physics 2018-08-24 Josep Planelles , Alexander W. Achtstein , Riccardo Scott , Nina Owschimikow , Juan I. Climente

Two-dimensional electron-hole gases in colloidal semiconductors have a wide variety of applications. Therefore, a proper physical understanding of these materials is of great importance. In this paper we present a detailed theoretical…

Mesoscale and Nanoscale Physics · Physics 2019-12-18 F. García Flórez , Aditya Kulkarni , Laurens D. A. Siebbeles , H. T. C. Stoof

Coupled two-dimensional electron-hole bilayers provide a unique platform to study strongly correlated Bose-Fermi mixtures in condensed matter. Electrons and holes in spatially separated layers can bind to form interlayer excitons, composite…

Theory of electronic and optical properties of exciton and bi-exciton complexes confined in CdSe spherical nanocrystals is presented. The electron and hole states are computed using atomistic $sp^3d^5s^*$ tight binding Hamiltonian including…

Mesoscale and Nanoscale Physics · Physics 2015-05-20 Marek Korkusinski , Oleksandr Voznyy , Pawel Hawrylak

he properties of excitons formed in spherical quantum dots are studied using the $\mathbf{k}\cdot\mathbf{p}$ method within the Hartree approximation. The spherical quantum dots considered have a central core and several concentric layers of…

Mesoscale and Nanoscale Physics · Physics 2019-10-11 Mariano Garagiola , Omar Osenda

We review the effects of Coulomb correlation on the linear and non-linear optical properties of semiconductor quantum wires, with emphasis on recent results for the bound excitonic states. Our theoretical approach is based on generalized…

Materials Science · Physics 2009-10-30 G. Goldoni , F. Rossi , E. Molinari

Methods for estimating the correlation energy of molecules and other electronic systems are discussed based on the assumption that the correlation energy can be partitioned between atomic regions. In one method, the electron density is…

Chemical Physics · Physics 2022-05-16 Jerry L. Whitten
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