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Energy transfer from photoexcited zero-dimensional systems to metallic systems plays a prominent role in modern day materials science. A situation of particular interest concerns the interaction between a photoexcited dipole and an…

Chemical Physics · Physics 2013-04-30 Zheyuan Chen , Stéphane Berciaud , Colin Nuckolls , Tony F. Heinz , Louis E. Brus

Using time-resolved photoluminescence spectroscopy, we explore the transient behavior of bound and free excitons in GaN nanowire ensembles. We investigate samples with distinct diameter distributions and show that the pronounced…

Van der Waals heterostructures made from atomically thin transition metal dichalcogenides (TMD) and graphene have emerged as a building block for optoelectronic devices. Such systems are also uniquely poised to investigate interfacial…

Recent experiments have shown that highly efficient energy transfer can take place in organic nanocrystals at extremely low acceptor densities. This striking phenomenon has been ascribed to the formation of exciton polaritons thanks to the…

Chemical Physics · Physics 2021-01-12 R. Sáez-Blázquez , J. Feist , F. J. García-Vidal , A. I. Fernández-Domínguez

Calculations of time-resolved fluorescence anisotropy from a pair of chromophores coupled by an excitation transfer interaction are presented. For the purpose of investigating the effects of nuclear motion on the energy transfer and…

chem-ph · Physics 2008-02-03 Alexander Matro , Jeffrey A. Cina

We present results on the rates of interlayer energy transfer between excitons in two-dimensional transition metal dichalcogenides (TMDs). We consider both radiative (mediated by real photons) and non-radiative (mediated by virtual photons)…

Mesoscale and Nanoscale Physics · Physics 2016-04-22 Christina Manolatou , Haining Wang , Weimin Chan , Sandip Tiwari , Farhan Rana

The near-field Coulomb interaction between a nano-emitter and a graphene monolayer results in strong F\"orster-type resonant energy transfer and subsequent fluorescence quenching. Here, we investigate the distance dependence of the energy…

We report about investigations of time-dependent structural modifications in single crystal graphene due to laser irradiation even at moderate power levels of 1mW in a diffraction limited spot. The structural modifications have been…

By performing spectroscopic single-particle measurements at cryogenic temperatures over the course of hours we study %By performing spectroscopic longtime single-particle measurements at cryogenic temperatures we study both the spectral…

Mesoscale and Nanoscale Physics · Physics 2017-11-13 Sven-Hendrik Lohmann , Christian Strelow , Alf Mews , Tobias Kipp

We have developed an ab-initio-based fully-quantum numerically-accurate methodology for the simulation of the exciton dynamics and time- and frequency-resolved fluorescence spectra of the cavity-controlled two-dimensional materials at…

Mesoscale and Nanoscale Physics · Physics 2023-03-29 Kewei Sun , Kaijun Shen , Maxim F. Gelin , Yang Zhao

To provide physical insight into the recently observed photoluminescence saturation behaviors in single-walled carbon nanotubes implying the existence of an upper limit of exciton densities, we have performed a time-dependent theoretical…

Mesoscale and Nanoscale Physics · Physics 2015-05-13 Ajit Srivastava , Junichiro Kono

Nonradiative transfer processes are often regarded as loss channels for an optical emitter1, since they are inherently difficult to be experimentally accessed. Recently, it has been shown that emitters, such as fluorophores and nitrogen…

In this paper, we study the near-field radiative energy, linear-momentum, and angular-momentum transfer from a current-biased graphene to nanoparticles. The electric current through the graphene sheet induces nonequilibrium fluctuations,…

Optics · Physics 2024-02-19 Huimin Zhu , Gaomin Tang , Lei Zhang , Jun Chen

The near-field interaction between fluorescent emitters and graphene exhibits rich physics associated with local dipole-induced electromagnetic fields that are strongly enhanced due to the unique properties of graphene. Here, we measure…

Mesoscale and Nanoscale Physics · Physics 2013-07-08 L. Gaudreau , K. J. Tielrooij , G. E. D. K. Prawiroatmodjo , J. Osmond , F. J. Garcia de Abajo , F. H. L. Koppens

Non-radiative optical energy transfer from a GaAs quantum well to a thin overlayer of an infrared organic semiconductor dye is unambiguously demonstrated. The dynamics of exciton transfer are studied in the time-domain using pump-probe…

Other Condensed Matter · Physics 2009-11-13 S. Chanyawadee , P. G. Lagoudakis , R. T. Harley , D. G. Lidzey , M. Henini

Non-radiative exciton relaxation processes are critical for energy transduction efficiencies in optoelectronic materials, but how these processes are connected to the underlying crystal structure and its associated electron, exciton, and…

Materials Science · Physics 2023-05-09 Galit Cohen , Jonah B. Haber , Jeffrey B. Neaton , Diana Y. Qiu , Sivan Refaely-Abramson

Fluorescence studies of natural photosynthetic complexes on a graphene layer demonstrate pronounced influence of the excitation wavelength on the energy transfer efficiency to graphene. Ultraviolet light yields much faster decay of…

Mesoscale and Nanoscale Physics · Physics 2015-07-13 Sebastian Mackowski , Izabela Kamińska

Transmission of low-energetic electrons through two-dimensional materials leads to unique scattering resonances. These resonances contribute to photoemission from occupied bands where they appear as strongly dispersive features of…

Materials Science · Physics 2017-11-22 M. Krivenkov , D. Marchenko , J. Sánchez-Barriga , O. Rader , A. Varykhalov

Here we describe an optical method to determine the dynamics of optically excited carriers in nanostructured composite samples. By combining pump-probe time-resolved reflectivity with scattering measurements, we extract the characteristic…

Mesoscale and Nanoscale Physics · Physics 2015-06-05 J. Barreto , T. Roger , A. Kaplan

We study theoretically the interaction of twisted light with graphene. The light-matter interaction matrix elements between the tight-binding states of electrons in graphene are determined near the Dirac points. We examine the dynamics of…

Mesoscale and Nanoscale Physics · Physics 2015-06-17 M. B. Farías , G. F. Quinteiro , P. I. Tamborenea
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