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Coordinate scaling of each spin density separately is considered in spin density functional theory. A virial theorem relates the spin-scaled correlation energy to the spin-scaled correlation potentials. An adiabatic connection formula…

Materials Science · Physics 2009-11-07 R. J. Magyar , T. K. Whittingham , K. Burke

Density scaling has a rich history in density functional theory, providing exact conditions for use in the construction of ever more accurate approximations to the unknown exchange-correlation functional. We define a conjugate potential…

Other Condensed Matter · Physics 2009-06-02 Peter Elliott , Kieron Burke

We analyze a decomposition of the Coulomb electron-electron interaction into a long-range and a short-range part in the framework of density functional theory, deriving some scaling relations and the corresponding virial theorem. We study…

Chemical Physics · Physics 2015-06-26 Julien Toulouse , Paola Gori-Giorgi , Andreas Savin

Finite temperature density functional theory provides, in principle, an exact description of the thermodynamical equilibrium of many-electron systems. In practical applications, however, the functionals must be approximated. Efficient and…

Statistical Mechanics · Physics 2015-05-19 S. Pittalis , C. R. Proetto , A. Floris , A. Sanna , C. Bersier , K. Burke , E. K. U. Gross

The virial theorem relates averages of kinetic energy and forces in confined systems. It is widely used to relate stresses in molecular simulation as measured at a boundary and in the interior of a system. In periodic systems, the theorem…

Chemical Physics · Physics 2023-02-27 A. C. Maggs

Stellar and galactic systems are objects in dynamical equilibrium that are composed of ordinary baryonic matter hypothetically embedded in extended dominant dark matter halos. Our aim is to investigate the scaling relations and…

Cosmology and Nongalactic Astrophysics · Physics 2011-02-14 Andre L. B. Ribeiro , Christine C. Dantas

A previous analysis of scaling, bounds, and inequalities for the non-interacting functionals of thermal density functional theory is extended to the full interacting functionals. The results are obtained from analysis of the related…

Statistical Mechanics · Physics 2016-12-14 James W. Dufty , S. B. Trickey

Density-functional theory simplifies many-electron calculations by approximating the exchange and correlation interactions with a one-electron operator that is a functional of the density. Hybrid functionals incorporate some amount of exact…

Materials Science · Physics 2021-02-03 John Vinson

Density-functional theory is a formally exact description of a many-body quantum system in terms of its density; in practice, however, approximations to the universal density functional are required. In this work, a model based on deep…

Computational Physics · Physics 2016-08-02 Jeffrey M. McMahon

Liquids displaying strong virial-potential energy correlations conform to an approximate density scaling of their structural and dynamical observables. This scaling property does not extend to the entire phase diagram, in general. The…

Soft Condensed Matter · Physics 2020-12-23 Thibaud Maimbourg , Jeppe C. Dyre , Lorenzo Costigliola

We develop a direct derivation for the primary contribution to the vibrational polarizability for molecules, clusters and other finite systems. The vibrational polarizability is then calculated within the generalized gradient approximation…

Other Condensed Matter · Physics 2007-05-23 Mark R. Pederson , Tunna Baruah , Philip B. Allen , Christian Schmidt

Partition density functional theory is a formally exact procedure for calculating molecular properties from Kohn-Sham calculations on isolated fragments, interacting via a global partition potential that is a functional of the fragment…

Other Condensed Matter · Physics 2015-05-13 Peter Elliott , Kieron Burke , Morrel H. Cohen , Adam Wasserman

The response of an infinite, periodic, insulating, solid to an infinitesimally small electric field is investigated in the framework of Density Functional Theory. We find that the applied perturbing potential is not a unique functional of…

mtrl-th · Physics 2016-09-07 X. Gonze , Ph. Ghosez , R. W. Godby , .

An interesting fundamental problem in density-functional theory of electronic structure of matter is to construct the exact Kohn-Sham (KS) potential for a given density. The exact potential can then be used to assess the accuracy of…

Atomic and Molecular Clusters · Physics 2019-05-22 Ashish Kumar , Rabeet Singh , Manoj K. Harbola

The coupling constant dependence is derived in time-dependent {\em current} density functional theory. The scaling relation can be used to check approximate functionals and in conjunction with the adiabatic connection formula to obtain the…

Materials Science · Physics 2009-11-11 Maxime Dion , Kieron Burke

The virial theorem is established in the framework of resolution-scale relativity for stochastic dynamics characterized by a diffusion constant D. It only relies on a simple time average just like the classical virial theorem, while the…

General Physics · Physics 2022-09-16 Tugdual LeBohec

Density Functional Theory relies on universal functionals characteristic of a given system. Those functionals in general are different for the electron gas and for jellium (electron gas with uniform background). However, jellium is…

Statistical Mechanics · Physics 2017-05-23 James W. Dufty

We present a brief review of the classical density functional theory of atomic and molecular fluids. We focus on the application of the theory to the determination of the solvation properties of arbitrary molecular solutes in arbitrary…

Chemical Physics · Physics 2015-04-06 Guillaume Jeanmairet , Maximilien Levesque , Volodymyr Sergiievskyi , Daniel Borgis

The scaling property of the thermodynamic free energy ($\Phi$) of a system at global equilibrium has been examined using a real-time method known as the virial theorem. We demonstrate these scaling properties through a derived relation…

High Energy Physics - Theory · Physics 2025-04-28 Sourav Dey

The virial theorem is considered for a system of randomly moving particles that are tightly bound to each other by the gravitational and electromagnetic fields, acceleration field and pressure field. The kinetic energy of the particles of…

General Physics · Physics 2018-01-22 Sergey G. Fedosin
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