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We describe in detail how attosecond delays in laser-assisted photoionization can be computed using perturbation theory based on two-photon matrix elements. Special emphasis is laid on above-threshold ionization, where the electron…

Atomic Physics · Physics 2015-06-19 J. M. Dahlström , E. Lindroth

We show that the correlation dynamics in coherently excited doubly excited resonances of helium can be followed in real time by two-photon interferometry. This approach promises to map the evolution of the two-electron wave packet onto…

Quantum Physics · Physics 2013-05-24 J. Feist , S. Nagele , C. Ticknor , B. I. Schneider , L. A. Collins , J. Burgdörfer

Ultrafast laser excitation can create coherent superpositions of electronic states in molecules and trigger ultrafast flow of electron density on few- to sub-femtosecond time scales. While recent attosecond experiments have addressed…

Chemical Physics · Physics 2020-11-18 Yuki Kobayashi , Daniel M. Neumark , Stephen R. Leone

We discuss level splitting and sideband transitions induced by a modulated coupling between a superconducting quantum circuit and a nanomechanical resonator. First, we show how to achieve an unconventional time-dependent longitudinal…

Quantum Physics · Physics 2018-08-15 Xin Wang , Adam Miranowicz , Hong-Rong Li , Fu-Li Li , Franco Nori

The dissociation dynamics of the $\tilde{A}$-state of ammonia have been studied using a resonant multiphoton ionisation probe in a photoelectron spectroscopy experiment. The use of a resonant intermediate in the multiphoton ionisation…

The attosecond high harmonic pulses obtained from a long Ar-filled gas cell were characterized by two techniques - the reconstruction of attosecond beating by interference of two-photon transition (RABITT) and frequency-resolved optical…

Many superconducting qubit systems use the dispersive interaction between the qubit and a coupled harmonic resonator to perform quantum state measurement. Previous works have found that such measurements can induce state transitions in the…

Attosecond interferometry in a two-color field is central to attosecond metrology and spectroscopy. In this technique, a photoelectron wave packet is released when a single photon from an extreme ultraviolet comb is absorbed. The wave…

We propose a general technique to retrieve the information of dipole-forbidden resonances in the autoionizing region. In the simulation, a helium atom is pumped by an isolated attosecond pulse in the extreme ultraviolet (EUV) combined with…

Atomic Physics · Physics 2014-03-28 Wei-Chun Chu , Toru Morishita , C. D. Lin

Attosecond pulses can ionize atoms in a coherent process. Since the emerging fragments are entangled, however, each preserves only a fraction of the initial coherence, thus limiting the chance of guiding the ion subsequent evolution. In…

Atomic Physics · Physics 2021-06-30 Saad Mehmood , Eva Lindroth , Luca Argenti

We propose a two-photon beating experiment based upon biphotons generated from a resonant pumping two-level system operating in a backward geometry. On the one hand, the linear optical-response leads biphotons produced from two sidebands in…

Quantum Physics · Physics 2009-11-13 Jianming Wen , Shengwang Du , Morton H. Rubin , Eun Oh

We performed quantum manipulations of the multi-level spin system S=5/2 of a Mn$^{2+}$ ion, by means of a two-tone pulse drive. The detuning between the excitation and readout radio frequency pulses allows one to select the number of…

Mesoscale and Nanoscale Physics · Physics 2015-10-29 S. Bertaina , M. Martens , M. Egels , D. Barakel , I. Chiorescu

We propose a new technique to fully characterize the temporal structure of extreme ultraviolet pulses by ionizing a bound coherent electronic wavepacket. The populated energy levels make it possible to interfere different spectral…

Optics · Physics 2016-07-19 Stefan Pabst , Jan Marcus Dahlström

Coherent control of interfering one- and two-photon processes has for decades been the subject of research to achieve the redirection of photocurrent. The present study develops two-pathway coherent control of ground state helium atom…

Atomic Physics · Physics 2021-06-02 Yimeng Wang , Chris H. Greene

Ultrashort electron pulses with a high average current provide a powerful means of enhancing time-resolved imaging and photon generation. In this study, we report the attosecond shaping of sub-relativistic electron beams using membranes in…

Radiative nonlinear four-wave mixing can monitor the evolution of electronic wave packets, providing access to lifetimes and quantifies the light induced couplings between excited states. We report the observation of quantum beats in an…

Atomic Physics · Physics 2025-11-25 S. Yanez-Pagans , M. A. Alarcon , C. H. Greene , A. Sandhu

We report two-photon resonance fluorescence of an individual semiconductor artificial atom. By non-linearly driving a single quantum dot via a two-photon transition, we probe the linewidth of the two-photon processes and show that, similar…

Mesoscale and Nanoscale Physics · Physics 2016-04-20 P. -L. Ardelt , M. Koller , T. Simmet , L. Hanschke , A. Bechtold , A. Regler , J. Wierzbowski , H. Riedl , K. Müller , J. J. Finley

A second plateau in the harmonic spectra of laser-driven two-electron atoms is observed both in the numerical solution of a low-dimensional model helium atom and using an extended strong field approximation. It is shown that the harmonics…

Atomic Physics · Physics 2009-11-13 P. Koval , F. Wilken , D. Bauer , C. H. Keitel

Resonant Raman excitation by ultrafast vacuum ultraviolet laser pulses is a powerful means to study electron dynamics in molecules, but experiments must contend with linear background ionization: frequencies high enough to reach resonant…

Chemical Physics · Physics 2015-06-23 S. Miyabe , P. Bucksbaum

We present an experimental feasible scheme to synthesize two-mode continuous-variable entangled states of two superconducting resonators that are interconnected by two gap-tunable superconducting qubits. We show that, with each artificial…

Quantum Physics · Physics 2015-06-05 Peng-Bo Li , Shao-Yan Gao , Fu-Li Li