Related papers: Ramsey-type microwave spectroscopy on CO ($a^3\Pi$…
Molecular laser cooling and trapping requires addressing all spontaneous decays to excited vibrational states that occur at the $\gtrsim 10^{-4} - 10^{-5}$ level, which is accomplished by driving repumping transitions out of these states.…
We experimentally show that an electric dipole moment of more than 1 Debye can be induced in the dysprosium (Dy) atom, in a long-lived state that is about 17513 cm$^{-1}$ above the ground state. This metastable state is part of a strongly…
We study a modified Ramsey spectroscopy technique employing slowly decaying states for quantum metrology applications using dense ensembles. While closely positioned atoms exhibit superradiant collective decay and dipole-dipole induced…
We use optical-optical double-resonance (OODR) spectroscopy to measure for the first time hot-band transitions of ethylene (C${_2}$H${_4}$) between states in the 3000 cm$^{-1}$ and 9000 cm$^{-1}$ energy ranges. A 3.2 ${\mu}$m continuous…
We report the measurement of sub-Doppler double-resonance transitions in methane using a 3.3 $\mu$m continuous wave optical parametric oscillator to pump transitions in the fundamental $\nu_3$ band and a 1.67 $\mu$m frequency comb to probe…
We perform laser induced fluorescence(LIF) spectroscopy on a pulsed supersonic beam of tungsten carbide(WC) molecules, which has been proposed as a candidate molecular system for a permanent Electric Dipole Moment(EDM) search of the…
The remarkable progress in the field of laser spectroscopy induced by the invention of the frequency-comb laser has enabled many new high-precision tests of fundamental theory and searches for new physics. Extending frequency-comb based…
We devise a perturbation-immune version of Ramsey's method of separated oscillatory fields. Spectroscopy of an atomic clock transition without compromising the clock's accuracy is accomplished by actively balancing the spectroscopic…
Band oscillator strengths for electronic transitions in CO were obtained at the Synchrotron Radiation Center of the University of Wisconsin-Madison. Our focus was on transitions that are observed in interstellar spectra with the Far…
We describe experimental investigations on an optical frequency standard based on a laser cooled 171Yb+ ion confined in a radiofrequency Paul trap. The electric-quadrupole transition from the 2S1/2(F=0) ground state to the 2D3/2(F=2) state…
We investigate a ionising electronic transition under resonant pumping. We demonstrate that, above a critical value of the pump intensity, a novel metastable electronic bound state is created, which can decay into the free electron…
We have performed for the first time direct laser spectroscopy of the 1S0-3P0 optical clock transition at 265.6 nm in fermionic isotopes of neutral mercury laser-cooled in a magneto-optical trap. Spectroscopy is performed by measuring the…
We find a superradiant quantum phase transition in the model of triangular molecular magnets coupled to the electric component of a microwave cavity field. The transition occurs when the coupling strength exceeds a critical value which, in…
We propose a set of experiments in which Ramsey-fringe techniques are tailored to probe transitions originating and terminating on the same ground state level. When pulses of resonant radiation, separated by a time delay $% T, $ interact…
We present the first broadband lambda = 1 mm spectrum toward the z=2.56 Cloverleaf Quasar, obtained with Z-Spec, a 1-mm grating spectrograph on the 10.4-meter Caltech Submillimeter Observatory. The 190-305 GHz observation band corresponds…
We demonstrate coherent control of both the rotational and hyperfine state of ultracold, chemically stable $^{87}$Rb$^{133}$Cs molecules with external microwave fields. We create a sample of ~2000 molecules in the lowest hyperfine level of…
We demonstrate a proof-of-principle magnetometer that relies on the active oscillation of a cold atom Raman laser to continuously map a field-sensitive atomic phase onto the phase of the radiated light. We demonstrate wideband sensitivity…
The hyperfine structure of the S1/2-D5/2 quadrupole transition at 729 nm in 43Ca+ has been investigated by laser spectroscopy using a single trapped 43Ca+ ion. We determine the hyperfine structure constants of the metastable level as…
We propose an experiment to search for a permanent atomic electric-dipole moment (EDM) using laser-cooled $^{171}$Yb atoms launched in an atomic fountain. A uniform B field sets the quantization axis, and the Ramsey…
Carbon monoxide molecules in their electronic, vibrational, and rotational ground state are highly attractive for trapping experiments. The optical or ac electric traps that can be envisioned for these molecules will be very shallow,…