Related papers: A Two-Photon E1-M1 Optical Clock
Recent developments in frequency metrology and optical clocks have been based on electronic transitions in atoms and singly charged ions as references. These systems have enabled relative frequency uncertainties at a level of a few parts in…
We study the $^1$S$_0 - ^3$D$_2$ and $^1$S$_0 - ^3$D$_3$ transitions in Cu II and the $^1$S$_0 - ^3$P$^{\rm o}_2$ transition in Yb III as possible candidates for the optical clock transitions. A recently developed version of the…
Electron-glasses can be readily driven far from equilibrium by a variety of means. Several mechanisms to excite the system and their relative merits are reviewed. In this study we focus on the process of exciting electron-glasses by…
The proposal for the development of a nuclear optical clock has triggered a multitude of experimental and theoretical studies. In particular the prediction of an unprecedented systematic frequency uncertainty of about $10^{-19}$ has…
Highly charged ions (HCIs) are promising candidates for the next generation of atomic clocks, owing to their tightly bound electron cloud, which significantly suppresses the common environmental disturbances to the quantum oscillator. Here…
Ionic clocks exhibit as the most promising candidates for the frequency standards. Recent investigations show the profound advantages of interrogating two laser beams with different frequencies in developing the frequency standards. Here we…
Optical clocks benefit from tight atomic confinement enabling extended interrogation times as well as Doppler- and recoil-free operation. However, these benefits come at the cost of frequency shifts that, if not properly controlled, may…
We explore the potential of the electric quadrupole transitions $7s\,^2S_{1/2}$ - $6d\,^2D_{3/2}$, $6d\,^2D_{5/2}$ in radium isotopes as single-ion optical frequency standards. The frequency shifts of the clock transitions due to external…
Optical clocks represent the most precise experimental devices, finding application in fields spanning from frequency metrology to fundamental physics. Recently, the first highly charged ions (HCI) based optical clock was demonstrated using…
Molecular magnets are attractive as spin qubits due to their chemical tunability, addressability through electron-spin resonance techniques, and long coherence times. Clock transitions (CTs), for which the system is immune to the effect of…
We identify Ba$^{4+}$ (Te-like) as a promising candidate for a high-accuracy optical clock. The lowest-lying electronic states are part of a $^3P_J$ fine structure manifold with anomalous energy ordering, being non-monotonic in $J$. We…
A viable qubit must have a long coherence time $T_2$. In molecular nanomagnets $T_2$ is often limited at low temperatures by the presence of dipole and hyperfine interactions, which are often mitigated through sample dilution, chemical…
We address the problem of lattice light shifts in the Sr clock caused by multipolar M1 and E2 atom-field interactions. We presented a simple but accurate formula for the magnetic-dipole polarizability that takes into account both the…
We experimentally investigate an optical clock based on $^{171}$Yb ($I=1/2$) atoms confined in an optical lattice. We have evaluated all known frequency shifts to the clock transition, including a density-dependent collision shift, with a…
We demonstrate coherent three-photon excitation of the strontium clock transition with a contrast of 51(12)% using a Bose-Einstein condensate. We follow it up with a demonstration of three-photon STIRAP-like transfer, overcoming the typical…
We present an algorithm for synchronizing two clocks based on second-order quantum interference between entangled photons generated by parametric down-conversion. The procedure is distinct from the standard Einstein two-way clock…
With the advent of optical clocks featuring fractional frequency uncertainties on the order of $10^{-17}$ and below, new applications such as chronometric levelling with few-cm height resolution emerge. We are developing a transportable…
Future transportable optical clocks require compact and reliable light sources. Here, broadband, unpolarized repumper and state clearout sources for Sr+ single-ion optical clocks are reported. These turn-key devices require no frequency…
Active optical clock, a new conception of atomic clock, has been proposed recently. In this report, we propose a scheme of active optical clock based on four-level quantum system. The final accuracy and stability of two-level quantum system…
Photons carrying a well-defined orbital angular momentum have been proven to modify spectroscopic selection rules in atomic matter. Excitation profiles of electric quadrupole transitions have been measured with single trapped $^{40}$Ca$^+$…