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One-hundred-nm-scale electronic structure calculations were carried out on the K supercomputer by our original simulation code ELSES (http://www.elses.jp/) The present paper reports preliminary results of transport calculations for…

Materials Science · Physics 2016-12-21 Hiroto Imachi , Seiya Yokoyama , Takami Kaji , Yukiya Abe , Tomofumi Tada , Takeo Hoshi

In Paper I, the effective one-electron potentials (OEP) method was introduced and demonstrated as an efficient approach to reduce the computational cost of evaluation of the charge-transfer interaction energy within the effective fragment…

Chemical Physics · Physics 2020-02-04 Bartosz Błasiak , Robert W. Góra , Wojciech Bartkowiak

The account of electron correlation and its efficient separation into dynamic and nondynamic parts plays a key role in the development of computational methods. In this paper we suggest a physically-sound matrix formulation to split…

Chemical Physics · Physics 2016-08-16 Eloy Ramos-Cordoba , Pedro Salvador , Eduard Matito

Targeting simulations on parallel hardware architectures, this paper presents computational kernels for efficient computations in mortar finite element methods. Mortar methods enable a variationally consistent imposition of coupling…

Numerical Analysis · Mathematics 2023-08-25 Matthias Mayr , Alexander Popp

The exact computation of orbits of discrete dynamical systems on the interval is considered. Therefore, a multiple-precision floating point approach based on error analysis is chosen and a general algorithm is presented. The correctness of…

Mathematical Software · Computer Science 2010-06-03 Christoph Spandl

The ideas behind the concept of algebraic ("integration-by-parts") algorithms for multiloop calculations are reviewed. For any topology and mass pattern, a finite iterative algebraic procedure is proved to exist which transforms the…

High Energy Physics - Phenomenology · Physics 2011-04-15 Fyodor V. Tkachov

In this paper we present in detail Newton's method and its modification, based on the Continuous analog of Newton's method for computing periodic orbits of the planar three-body problem. The linear system at each step of the method is…

Chaotic Dynamics · Physics 2021-11-23 I. Hristov , R. Hristova , I. Puzynin , T. Puzynina , Z. Sharipov , Z. Tukhliev

The multiplicative Newton-like method developed by the author et al. is extended to the situation where the dynamics is restricted to the orthogonal group. A general framework is constructed without specifying the cost function. Though the…

Machine Learning · Computer Science 2007-05-23 Toshinao Akuzawa

We introduce an energy functional for ground-state electronic structure calculations. Its variables are the natural spin-orbitals of singlet many-body wave functions and their joint occupation probabilities deriving from controlled…

Chemical Physics · Physics 2016-12-04 Ralph Gebauer , Morrel H. Cohen , Roberto Car

We adapt the simulated annealing algorithm to the search of periodic orbits for classical multi-electron atomic systems. This is done by minimizing the n-th return distance to the initial position on a Poincare surface of section under an…

Atomic Physics · Physics 2011-02-17 Francois Mauger , Cristel Chandre , Turgay Uzer

The performance of basis sets made of numerical atomic orbitals is explored in density-functional calculations of solids and molecules. With the aim of optimizing basis quality while maintaining strict localization of the orbitals, as…

Materials Science · Physics 2009-11-07 Javier Junquera , Oscar Paz , Daniel Sanchez-Portal , Emilio Artacho

A new concept of the molecular structure optimization method based on quantum dynamics computations is presented. Nuclei are treated as quantum mechanical particles, as are electrons, and the many-body wave function of the system is…

A characteristic feature of the state-of-the-art of real-space methods in electronic structure calculations is the diversity of the techniques used in the discretization of the relevant partial differential equations. In this context, the…

There are many numerical methods for solving partial different equations (PDEs) on manifolds such as classical implicit, finite difference, finite element, and isogeometric analysis methods which aim at improving the interoperability…

Numerical Analysis · Mathematics 2023-11-17 Wenrui Hao , Jonathan D. Hauenstein , Margaret H. Regan , Tingting Tang

Various properties of the general two-center two-electron integral over the explicitly correlated exponential function are analyzed for the potential use in high precision calculations for diatomic molecules. A compact one dimensional…

Chemical Physics · Physics 2015-06-11 Krzysztof Pachucki

In this article we introduce a novel coupled algorithm for massively parallel direct numerical simulations of electrophoresis in microfluidic flows. This multiphysics algorithm employs an Eulerian description of fluid and ions, combined…

Computational Engineering, Finance, and Science · Computer Science 2018-05-29 Dominik Bartuschat , Ulrich Rüde

The quantum phase estimation algorithm stands as the primary method for determining the ground state energy of a molecular electronic Hamiltonian on a quantum computer. In this context, the ability to initialize a classically tractable…

An efficient method for calculating the electronic structure of systems that need a very fine sampling of the Brillouin zone is presented. The method is based on the variational optimization of a "single" (i.e. common to all points in the…

Materials Science · Physics 2009-10-31 Sandro Scandolo , Jorge Kohanoff

We present a natural orbital-based implementation of the intermediate Hamiltonian Fock space coupled-cluster method for (1,1) sector of Fock space. The use of natural orbital significantly reduces the computational cost and can…

Chemical Physics · Physics 2021-09-07 Soumi Haldar , Achintya Kumar Dutta

Natural orbital theory is a computationally useful approach to the few and many-body quantum problem. While natural orbitals are known and applied since many years in electronic structure applications, their potential for time-dependent…

Atomic Physics · Physics 2014-10-08 J. Rapp , M. Brics , D. Bauer
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