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Maximum efficiency of ideal single-junction photovoltaic (PV) cells is limited to 33% (for one sun illumination) by intrinsic losses such as band edge thermalization, radiative recombination, and inability to absorb below-bandgap photons.…

Optics · Physics 2015-06-17 Svetlana V. Boriskina , Gang Chen

Single-junction photovoltaic cells are considered to be efficient solar energy converters, but even ideal cells cannot exceed the their fundamental thermodynamic efficiency limit, first analysed by Shockley and Queisser (SQ). For moderated…

Optics · Physics 2015-05-21 Assaf Manor , Carmel Rotschild

Thermophotovotaics convert thermal radiation from local heat sources to electricity. A new breakthrough in creating highly efficient thin-film solar cells can potentially enable thermophotovoltaic systems with unprecedented high efficiency.…

Optics · Physics 2018-02-08 Vidya Ganapati , T. Patrick Xiao , Eli Yablonovitch

The Shockley-Queisser (SQ) limit, introduced by W. Shockley and H. J. Queisser in 1961, is the most well-established fundamental efficiency limit for single-junction photovoltaic solar cells. For widely-studied semiconductors such as Si,…

Applied Physics · Physics 2021-06-09 Qian Zhou , Arfa Karani , Yaxiao Lian , Baodan Zhao , Richard H. Friend , Dawei Di

We propose a solar thermal energy conversion system consisting of a solar absorber, a thermoradiative cell or negative illumination photodiode, and a photovoltaic cell. Because it is a heat engine, this system can also be paired with…

Photovoltaic materials are recognized for their potential as sustainable energy sources that enable the conversion between light and electrical energy. However, solar cells have been unable to surpass the theoretical limit of 32%, known as…

Applied Physics · Physics 2024-06-18 Jeonggyu Hwang

The Shockley-Queisser limit is one of the most fundamental results in the field of photovoltaics. Based on the principle of detailed balance, it defines an upper limit for a single junction solar cell that uses an absorber material with a…

Materials Science · Physics 2017-06-29 Marnik Bercx , Rolando Saniz , Bart Partoens , Dirk Lamoen

The bulk photovoltaic effect (BPVE) leads to directed photo-currents and photo-voltages in bulk materials. Unlike photo-voltages in p-n junction solar cells that are limited by carrier recombination to values below the bandgap energy of the…

Applied Physics · Physics 2023-03-17 Andreas Pusch , Udo Römer , Dimitrie Culcer , Nicholas J. Ekins-Daukes

The Shockley-Queisser (SQ) limit provides a convenient metric for predicting light-to-electricity conversion efficiency of a solar cell based on the band gap of the light-absorbing layer. In reality, few materials approach this radiative…

Computational Physics · Physics 2020-05-22 Sunghyun Kim , José A. Márquez , Thomas Unold , Aron Walsh

Photoluminescence (PL) is a fundamental light-matter interaction, which conventionally involves the absorption of energetic photon, thermalization and the emission of a red-shifted photon. Conversely, in optical-refrigeration the absorption…

Optics · Physics 2014-12-23 Assaf Manor , Leopoldo L. Martin , Carmel Rotschild

The Shockley-Queisser limit describes the maximum solar energy conversion efficiency achievable for a particular material and is the standard by which new photovoltaic technologies are compared. This limit is based on the principle of…

Optics · Physics 2014-12-04 Yunlu Xu , Tao Gong , Jeremy N. Munday

Thermophotovoltaic devices are energy-conversion systems generating an electric current from the thermal photons radiated by a hot body. In far field, the efficiency of these systems is limited by the thermodynamic Schockley-Queisser limit…

Mesoscale and Nanoscale Physics · Physics 2016-07-19 Riccardo Messina , Philippe Ben-Abdallah

To absorb the photons below the band-gap energy effectively, we proposed a quantum dot (QD) photocell modeled by multi-level system for the quantum yields and photo-to-charge efficiency limits. The theoretical results show the quantum…

Mesoscale and Nanoscale Physics · Physics 2024-02-26 Shun-Cai Zhao , Jing-Yi Chen

The photovoltaic solar cell is a mature technology, with silicon-based technologies deployed at scale, yet current technologies are limited by the Shockley-Queisser thermodynamic limit, known since the early 1960s. The single-junction…

Materials Science · Physics 2026-01-26 Gabriel J. Man

The theoretical maximum efficiency of a solar cell is typically characterized by a detailed balance of optical absorption and emission for a semiconductor in the limit of unity radiative efficiency and an ideal step-function response for…

Applied Physics · Physics 2021-03-09 Joeson Wong , Stefan T. Omelchenko , Harry A. Atwater

We employ a detailed balance approach to model a single-junction solar cell with a realistic narrow-band, non-unity-quantum-yield upconverter. As upconverter bandwidths are increased from 0 to 0.5 eV, maximum cell efficiencies increase from…

Optics · Physics 2013-09-23 Justin A. Briggs , Ashwin C. Atre , Jennifer A. Dionne

The ideal solar cell conversion efficiency limit known as the Shockley-Queisser (SQ) limit, which is based on a detailed balance between absorption and radiation, has long been a target for solar cell researchers. While the theory for this…

Applied Physics · Physics 2018-11-07 Kenji Kamide , Toshimitsu Mochizuki , Hidefumi Akiyama , Hidetaka Takato

Harnessing low energy photons is of paramount importance for multi-junction high efficiency solar cells as well as for thermo-photovoltaic applications. However, semiconductor absorbers with bandgap lower than 0.8 eV have been limited to…

Absorbed sunlight in a solar cell produces electrons and holes. But, at the open circuit condition, the carriers have no place to go. They build up in density and, ideally, they emit external fluorescence that exactly balances the incoming…

Optics · Physics 2013-08-02 Owen D. Miller , Eli Yablonovitch , Sarah R. Kurtz

The Shockley and Queisser limit, a well-known efficiency limit for a solar cell, is based on unrealistic physical assumptions and its maximum limit is seriously overestimated. To understand the power loss mechanisms of record-efficiency…

Applied Physics · Physics 2019-08-28 Yoshitsune Kato , Shohei Fujimoto , Masayuki Kozawa , Hiroyuki Fujiwara
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