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We use a quantum trajectory-based semi-classical method to account for Coulomb interaction between the photoelectron and the parent ion in the classically forbidden, sub-barrier region during strong-field tunneling ionization processes. We…

Atomic Physics · Physics 2017-11-21 Tian-Min Yan , D. Bauer

Ultrafast pump-probe experiments open the possibility to track fundamental material behaviour like changes in its electronic configuration in real time. To date, most of these experiments are performed using an electron or a high-energy…

Spectroscopic photoemission microscopy is a well-established method to investigate the electronic structure of surfaces. In modern photoemission microscopes the electron optics allows imaging of the image plane, momentum plane, or…

Recent advancements in time-resolved electron and photon detection enable novel correlative measurements of electrons and their associated cathodoluminescence (CL) photons within a transmission electron microscope. These studies are pivotal…

We theoretically study the process of photoelectron emission of the Helium atom by a high-intensity short-wavelength laser at a resonance condition of the residual singly charged ion. Photoionization followed by strong resonance coupling in…

Atomic Physics · Physics 2014-01-14 Song Bin Zhang , Nina Rohringer

We demonstrate time-resolved nonlinear extreme-ultraviolet absorption spectroscopy on multiply charged ions, here applied to the doubly charged neon ion, driven by a phase-locked sequence of two intense free-electron laser pulses.…

We experimentally and theoretically investigate the influence of the magnetic component of an electromagnetic field on high-order above-threshold ionization of xenon atoms driven by ultrashort femtosecond laser pulses. The nondipole shift…

Nonlinear optical phenomena such as parametric amplification and frequency conversion are typically driven by external optical fields. Free electrons can also act as electromagnetic sources, offering unmatched spatial precision. Combining…

Mesoscale and Nanoscale Physics · Physics 2025-08-04 Leila Prelat , Eduardo J. C. Dias , F. Javier García de Abajo

The linearly polarized quasi-real photons from the highly Lorentz-contracted Coulomb fields of relativistic heavy ions can fluctuate to quark-antiquark pairs, scatter off a target nucleus and emerge as vector mesons. In the process, the two…

High Energy Physics - Phenomenology · Physics 2021-03-03 Wangmei Zha , James Daniel Brandenburg , Lijuan Ruan , Zebo Tang , Zhangbu Xu

Imaging in real time the complete dynamics of a process as fundamental as photoemission has long been out of reach due to the difficulty of combining attosecond temporal resolution with fine spectral and angular resolutions. Here, we…

We investigate the angle-resolved photoelectron spectra from laser-assisted photoionization for helium and neon atoms using an \textit{ab initio} method based on time-dependent surface flux and configuration interaction singles. We find…

Atomic Physics · Physics 2020-08-26 Mattias Bertolino , David Busto , Felipe Zapata , Jan Marcus Dahlström

A second plateau in the harmonic spectra of laser-driven two-electron atoms is observed both in the numerical solution of a low-dimensional model helium atom and using an extended strong field approximation. It is shown that the harmonics…

Atomic Physics · Physics 2009-11-13 P. Koval , F. Wilken , D. Bauer , C. H. Keitel

We demonstrate the generation of Coulomb-correlated pair, triple and quadruple states of free electrons by femtosecond photoemission from a nanoscale field emitter inside a transmission electron microscope. Event-based electron spectroscopy…

Mesoscale and Nanoscale Physics · Physics 2023-11-28 Rudolf Haindl , Armin Feist , Till Domröse , Marcel Möller , John H. Gaida , Sergey V. Yalunin , Claus Ropers

Electron energy loss spectroscopy is consolidating as a powerful tool to explore electronic (as well as vibrational) excitations of matter, including molecules. Performed in a scanning transmission electron microscope, this technique is…

Chemical Physics · Physics 2021-03-05 Ciro A. Guido , Enzo Rotunno , Matteo Zanfrognini , Stefano Corni , Vincenzo Grillo

We consider the elastic scattering of electrons by hydrogen atoms in the presence of a two-color circularly polarized laser field in the domain of moderate intensities below $10^{13}$ W/cm$^2$ and high projectile energies. A hybrid approach…

Atomic Physics · Physics 2023-06-16 Gabriela Buica

Two-dimensional electronic spectroscopy provides information on coupling and energy transfer between excited states on ultrafast timescales. Only recently, incoherent fluorescence detection has made it possible to combine this method with…

Optics · Physics 2025-05-14 Sanchayeeta Jana , Simon Durst , Lucas Ludwig , Markus Lippitz

Intense light-matter interactions have revolutionized our ability to probe and manipulate quantum systems at sub-femtosecond time scales, opening routes to all-optical control of electronic currents in solids at petahertz rates. Such…

Multidimensional coherent optical spectroscopy is one of the most powerful tools for investigating complex quantum mechanical systems. While it was conceived decades ago in magnetic resonance spectroscopy using micro- and radio-waves, it…

We calculate two-dimensional photoelectron momentum distributions and energy spectra after multiphoton ionization of Li atoms subject to intense laser fields in one-photon Rabi-flopping regime. The time-dependent Schr\"{o}dinger equation is…

Atomic Physics · Physics 2019-09-24 D. A. Tumakov , Dmitry A. Telnov , G. Plunien , V. M. Shabaev

A nonlinear interferometry scheme is described theoretically to induce and resolve electron wave- function beating on time scales shorter than the optical cycle of the time-delayed pump and probe pulses. By employing two moderately intense…

Chemical Physics · Physics 2017-08-23 Christian Ott , Philipp Raith , Thomas Pfeifer
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