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Related papers: Nonharmonic Phonons in $\alpha$-Iron at High Tempe…

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Body-centered cubic (bcc) Fe-Mn systems are known to exhibit a complex and atypical magnetic behaviour from both experiments and 0 K electronic-structure calculations, which is due to the half-filled 3d-band of Mn. We propose effective…

Materials Science · Physics 2021-01-20 Anton Schneider , Chu-Chun Fu , Osamu Waseda , Cyrille Barreteau , Tilmann Hickel

We have investigated the anisotropic thermal expansion of graphite using ab-initio calculation of lattice dynamics and anharmonicity of the phonons, which reveal that the negative thermal expansion (NTE) in the a-b plane below 600 K and…

Materials Science · Physics 2021-05-05 Ranjan Mittal , Mayanak K. Gupta , Baltej Singh , S. K. Mishra , Samrath L. Chaplot

For over a century, x-ray scattering has been the most powerful tool for determining the equilibrium structure of crystalline materials. Deviations from perfect periodicity, for example due to thermal motion of the atoms, reduces the…

Materials Science · Physics 2013-05-29 M. Trigo , Y. M Sheu , J. Chen , V. H. Vishwanath , T. Graber , R. Henning , D. A. Reis

Diamond is studied by path integral molecular dynamics simulations of the atomic nuclei in combination with a tight-binding Hamiltonian to describe its electronic structure and total energy. This approach allows us to quantify the influence…

Materials Science · Physics 2009-11-11 Rafael Ramirez , Carlos P. Herrero , Eduardo R. Hernandez

We performed ultrasonic measurements on (Ta$_{0.952}$V$_{0.048}$)$_2$NiSe$_5$ to investigate the contribution of acoustic phonons at the zone center to structural and possible excitonic transitions. The transverse elastic constant $C_{55}$…

Strongly Correlated Electrons · Physics 2022-01-19 Ryosuke Kurihara , Yusuke Hirose , Sumika Sano , Keisuke Mitsumoto , Atsushi Miyake , Masashi Tokunaga , Rikio Settai

Although the rutile structure of TiO$_2$ is stable at high temperatures, the conventional quasiharmonic approximation predicts that several acoustic phonons decrease anomalously to zero frequency with thermal expansion, incorrectly…

Materials Science · Physics 2015-08-19 Tian Lan , C. W. Li , O. Hellman , D. Kim , J. A. Muñoz , H. Smith , D. L. Abernathy , B. Fultz

The anharmonicity resulted from the intrinsic phonon interaction is neglected by quasiharmonic approximation. Although the intensive researches about anharmonicity have been done, up to now the free energy contributed by the anharmonicity…

Statistical Mechanics · Physics 2007-05-23 Zhongqing Wu , Renata M. Wentzcovitch

Under pressure cesium undergoes a transition from a high-pressure fcc phase (Cs-II) to a collapsed fcc phase (Cs-III) near 4.2GPa. At 4.4GPa there follows a transition to the tetragonal Cs-IV phase. In order to investigate the lattice…

Materials Science · Physics 2009-10-31 Y. Kong , O. Jepsen

We compute the transient dynamics of phonons in contact with high energy "hot" charge carriers in 12 polar and non-polar semiconductors, using a first-principles Boltzmann transport framework. For most materials, we find that the decay in…

Mesoscale and Nanoscale Physics · Physics 2017-10-03 Sridhar Sadasivam , Maria K. Y. Chan , Pierre Darancet

The dephasing and relaxation kinetics of bosonic excitons interacting with a thermal bath of acoustic phonons is studied after coherent pulse excitation. The kinetics of the induced excitonic polarization is calculated within Markovian…

Statistical Mechanics · Physics 2009-10-31 O. M. Schmitt , D. B. Tran Thoai , P. Gartner , H. Haug

The femtosecond optical pump-probe technique was used to study dynamics of photoexcited electrons and coherent optical phonons in transition metals Zn and Cd as a function of temperature and excitation level. The optical response in time…

Strongly Correlated Electrons · Physics 2009-11-11 Muneaki Hase , Kunie Ishioka , Jure Demsar , Kiminori Ushida , Masahiro Kitajima

We present Gibbs free-energy phase diagrams for compressed iron within a pressure range of 20 to 300 GPa and electronic temperature up to 3 eV obtained using finite-temperature density functional and density functional perturbation…

Materials Science · Physics 2025-11-07 S. Azadi , S. M. Vinko

Phonons as bosons are different from electrons as fermions. Unlike interatomic electron hopping that can be either positive or negative and further tuned by spin-orbit coupling, interatomic spring constant is positive, or the structure of…

Materials Science · Physics 2022-09-07 Bowen Xia , Hang Liu , Feng Liu

We determine the nature of coupled phonons and magnetic excitations in AlFeO3 using inelastic light scattering from 5 K to 315 K covering a spectral range from 100-2200 cm-1 and complementary first-principles density functional theory-based…

Strongly Correlated Electrons · Physics 2012-05-01 Pradeep Kumar , A. Bera , D. V. S. Muthu , S. N. Shirodkar , R. Saha , A. Shireen , A. Sundaresan , U. V. Waghmare , A. K. Sood , C. N. R. Rao

We show how the coupling between the phonons and electrons in a strongly correlated metal can result in phonon frequencies which have a non-monotonic temperature dependence. Dynamical mean-field theory is used to study the Hubbard-Holstein…

Strongly Correlated Electrons · Physics 2009-10-31 J. Merino , Ross H. McKenzie

We report on the study of phonon properties and electron-phonon coupling in thin NbTiN films, which are intensively exploited in superconducting devices. Studied NbTiN films with thicknesses less than 10~nm are disordered with respect to…

Superconductivity · Physics 2021-12-01 M. Sidorova , A. Semenov , H. -W. Huebers , S. Gyger , S. Steinhauer , X. Zhang , A. Schilling

We solve for the finite temperature collective mode dynamics in the Holstein-double exchange problem, using coupled Langevin equations for the phonon and spin variables. We present results in a strongly anharmonic regime, close to a…

Strongly Correlated Electrons · Physics 2020-03-30 Sauri Bhattacharyya , Sankha Subhra Bakshi , Saurabh Pradhan , Pinaki Majumdar

The strongly correlated material FeSi exhibits several unusual thermal, magnetic, and structural properties under varying pressure-temperature (P-T) conditions. It is a potential thermoelectric alloy and a materials of several geological…

While the thermoelectric figure of merit zT above 300K has seen significant improvement recently, the progress at lower temperatures has been slow, mainly limited by the relatively low Seebeck coefficient and high thermal conductivity. Here…

Materials Science · Physics 2016-02-17 Jiawei Zhou , Bolin Liao , Bo Qiu , Samuel Huberman , Keivan Esfarjani , Mildred S. Dresselhaus , Gang Chen

We report detailed measurements of composition as well as temperature dependence of the phonon density-of-states in a new series of FeAs compounds with composition CaFe1\_{1-x}Co\_{x}AsF (x = 0, 0.06, 0.12). The composition as well as…

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