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Recently colossal positive volume thermal expansion has been found in the framework compounds Ag3Co(CN)6 and Ag3Fe(CN)6. Phonon spectra have been measured using the inelastic neutron scattering technique as a function of temperature and…

Materials Science · Physics 2015-06-05 R Mittal , M. Zbiri , H. Schober , S. N. Achary , A. K. Tyagi , S. L. Chaplot

We report on the temperature dependent Raman spectroscopic studies of orthorombic distorted perovskite YCrO3 in the temperature range of 20-300K. Temperature dependence of DC-magnetization measurement under field cooled and zero field…

Materials Science · Physics 2013-09-30 Yogesh Sharma , Satyaprakash Sahoo , W. Perez , Ram S. Katiyar

Phonons in single crystals of PrFeAsO_{1-y} are investigated using high-resolution inelastic x-ray scattering and ab initio pseudopotential calculations. Extensive measurements of several samples at temperatures spanning the magnetic…

Strongly Correlated Electrons · Physics 2011-08-12 T. Fukuda , A. Q. R. Baron , H. Nakamura , S. Shamoto , M. Ishikado , M. Machida , H. Uchiyama , A. Iyo , H. Kito , J. Mizuki , M. Arai , H. Eisaki

We investigate the effects of nonequilibrium phonon dynamics on the operation of a GaAs-based midinfrared quantum cascade laser over a range of temperatures (77--300 K) via a coupled ensemble Monte Carlo simulation of electron and…

Mesoscale and Nanoscale Physics · Physics 2016-07-28 Y. B. Shi , I. Knezevic

Diffusion is the underlying mechanism for many complicated materials phenomena, and understanding it is basic to the discovery of novel materials with desired physical and mechanical properties. Certain groups of solid phases, such as the…

Materials Science · Physics 2023-07-06 Sara Kadkhodaei , Ali Davariashtiyani

We apply a general first-principles approach to derive the phase diagram of metallic Lithium at ambient pressure between 0 and 350 K, including identification of candidate phases. We use ab initio random structure searching (AIRSS) to…

Materials Science · Physics 2019-01-29 Michael Hutcheon , Richard Needs

Despite the widespread use of silicon in modern technology, its peculiar thermal expansion is not well-understood. Adapting harmonic phonons to the specific volume at temperature, the quasiharmonic approximation, has become accepted for…

Experimental investigation as well as theoretical calculations, of the Fe-partial phonon density-of-states (DOS) for nominally Fe_52.5Cr_47.5 alloy having (a) alpha- and (b) sigma-phase structure were carried out. The former at sector 3-ID…

Materials Science · Physics 2015-05-14 S. M. Dubiel , J. Cieslak , W. Sturhahn , M. Sternik , P. Piekarz , S. Stankov , K. Parlinski

We present the results of inelastic x-ray scattering for magnetite and analyze the energies and spectral widths of the phonon modes with different symmetries in a broad range of temperature 125<T<293 K. The phonon modes with X_4 and Delta_5…

The thermodynamic properties of hcp-iron ({\epsilon}-Fe) are essential for investigating planetary cores' internal structure and dynamic properties. Despite their importance to planetary sciences, experimental investigations of…

Materials Science · Physics 2021-04-21 Jingyi Zhuang , Hongjin Wang , Qi Zhang , Renata M. Wentzcovitch

Structural stability of paramagnetic (PM) body-centered cubic (bcc) Fe under pressure is investigated based on first-principles phonon calculations. Spin configurations of the PM phase are approximated using a binary special quasi-random…

Materials Science · Physics 2015-06-22 Yuji Ikeda , Atsuto Seko , Atsushi Togo , Isao Tanaka

All phonons in a single crystal of NaBr were measured by inelastic neutron scattering at temperatures of 10, 300 and 700 K. Even at 300 K the phonons, especially the longitudinal-optical (LO) phonons, showed large shifts in frequencies, and…

Materials Science · Physics 2020-08-26 Y. Shen , C. N. Saunders , C. M. Bernal , D. L. Abernathy , M. E. Manley , B. Fultz

At room temperature, PbTe and SnTe are efficient thermoelectrics with a cubic structure. At low temperature, SnTe undergoes a ferroelectric transition with a critical temperature strongly dependent on the hole concentration, while PbTe is…

Magnetic dc susceptibility between 1.5 and 800 K, ac susceptibility and magnetization, thermodynamic properties, temperature dependence of radio and audio-wave dielectric constants and conductivity, contact-free dielectric constants at…

Materials Science · Physics 2010-07-22 Jun Lu , A. Günther , F. Schrettle , F. Mayr , S. Krohns , P. Lunkenheimer , A. Pimenov , V. D. Travkin , A. A. Mukhin , A. Loidl

Parent compounds of Fe-based superconductors undergo a structural phase transition from a tetragonal to an orthorhombic structure. We investigated the temperature dependence of the frequencies of transverse acoustic (TA) phonons that…

Superconductivity · Physics 2015-05-13 D. Parshall , L. Pintschovius , D. Lamago , J. -P. Castellan , J. L. Niedziela , Th. Wolf , D. Reznik

The temperature dependence of the phonon spectrum in the superconducting transition metal dichalcogenide 2H-NbS$_2$ is measured by diffuse and inelastic x-ray scattering. A deep, wide and strongly temperature dependent softening, of the two…

While the vibrational thermodynamics of materials with small anharmonicity at low temperatures has been understood well based on the harmonic phonons approximation; at high temperatures, this understanding must accommodate how phonons…

Materials Science · Physics 2015-10-20 Tian Lan

The anharmonic phonon properties of SnSe in the Pnma phase were investigated with a combination of experiments and first-principles simulations. Using inelastic neutron scattering (INS) and nuclear resonant inelastic X-ray scattering…

We report an investigation of the lattice dynamical properties in a range of Fe$_{1+y}$Te$_{1-x}$Se$_{x}$ compounds, with special emphasis on the c-axis polarized vibration of Fe with B$_{1g}$ symmetry, a Raman active mode common to all…

Zn(CN)2 is known to have an isotropic negative thermal expansion (NTE) coefficient (about -51 x 10-6 K-1) over 10-370 K that is twice as large as that of ZrW2O8. We have measured the pressure dependence of the phonon spectra up to 30 meV…

Materials Science · Physics 2015-05-13 R. Mittal , S. L . Chaplot , H. Schober