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We report on a study of Dynamic Nuclear Polarization and electron and nuclear spin relaxation of atomic hydrogen and deuterium in solid molecular matrices of H$_{2}$, D$_{2}$, and HD mixtures. The electron and nuclear spin relaxation times…

Atomic and Molecular Clusters · Physics 2017-02-08 S. Sheludiakov , J. Ahokas , J. Järvinen , O. Vainio , L. Lehtonen , S. Vasiliev , D. M. Lee , V. V. Khmelenko

We propose a new mechanism for polarizing nuclear spins in quantum dots, based on periodic modulation of the hyperfine coupling by electric driving at the electron spin resonance frequency. Dynamical nuclear polarization results from…

Mesoscale and Nanoscale Physics · Physics 2008-04-14 M. S. Rudner , L. S. Levitov

Due to their long coherence times, nuclear spins have gained considerable attention as physical qubits. Two-qubit gates between nuclear spins of distinct resonance frequencies can be mediated by electron spins, usually employing a sequence…

Quantum Physics · Physics 2021-01-26 Benedikt Tratzmiller , Jan F. Haase , Zhenyu Wang , Martin B. Plenio

The magnetic interactions between the spin of an unpaired electron and the surrounding nuclear spins can be exploited to gain structural information, to reduce nuclear relaxation times as well as to create nuclear hyperpolarization via…

We study the spin dynamics in charged quantum dots in the situation where the resident electron is coupled to only about 200 nuclear spins and where the electron spin splitting induced by the Overhauser field does not exceed markedly the…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 D. H. Feng , I. A. Akimov , F. Henneberger

We consider, in the framework of the central spin $s=1/2$ model, driven dynamics of two electrons in a double quantum dot subject to hyperfine interaction with nuclear spins and spin-orbit coupling. The nuclear subsystem dynamically evolves…

Mesoscale and Nanoscale Physics · Physics 2015-06-17 Arne Brataas , Emmanuel I. Rashba

Nuclear spins show long coherence times and are well isolated from the environment, which are properties making them promising for quantum information applications. Here, we present a method for nuclear spin readout by probing the…

Mesoscale and Nanoscale Physics · Physics 2021-06-30 Jonas Mielke , Jason R. Petta , Guido Burkard

In dissolution-dynamic nuclear polarization, nuclear spins are hyperpolarized at cryogenic temperatures using radicals and microwave irradiation. The hyperpolarized solid is dissolved with hot solvent and the solution is transferred to a…

Instrumentation and Detectors · Physics 2019-06-20 Karel Kouřil , Hana Kouřilová , Samuel Bartram , Malcolm H. Levitt , Benno Meier

Spin current perpendicular to the electric current is investigated around Landau level filling factor $\nu=3$ in a GaAs/AlGaAs two-dimensional electron system. Measurements of dynamic nuclear polarization in the vicinity of the edge of a…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 Yosuke Komori , Satoru Sakuma , Tohru Okamoto

We have studied hyperfine interactions between spin-polarized electrons and lattice nuclei in Al_0.1Ga_0.9As/GaAs quantum well (QW) heterostructures. The spin-polarized electrons are electrically injected into the semiconductor…

Materials Science · Physics 2009-11-11 J. Strand , X. Lou , C. Adelmann , B. D. Schultz , A. F. Isakovic , C. J. Palmstrom , P. A. Crowell

Control over nuclear spin fluctuations is essential for processes that rely on preserving the quantum state of an embedded system. For this purpose, squeezing is a viable alternative, so far that has not been properly exploited for the…

Quantum Physics · Physics 2016-01-14 Yağmur Aksu Korkmaz , Ceyhun Bulutay

Coherent dynamics of localized spins in semiconductors is limited by spectral diffusion arising from dipolar fluctuation of lattice nuclear spins. Here we extend the semiclassical theory of spectral diffusion for nuclear spins I=1/2 to the…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Rogerio de Sousa , Neil Shenvi , K. Birgitta Whaley

For applications of solid state quantum computing and quantum simulations, high fidelity initialisation of thermally mixed electronic and nuclear spin qubits is essential. Whereas electronic spins can readily be initialised optically to…

Quantum Physics · Physics 2024-04-12 O. T. Whaites , T. S. Monteiro

Dynamic Nuclear Polarization (DNP) has revolutionized the field of solid-state NMR spectroscopy by significantly enhancing the sensitivity of nuclear magnetic resonance experiments. Conventionally, cross effect DNP relies on biradicals to…

Chemical Physics · Physics 2023-09-28 Amaria Javed , Asif Equbal

Electron spin dephasing in a singly charged semiconductor quantum dot can partially be suppressed by periodic laser pulsing. We propose a semi-classical approach describing the decoherence of the electron spin polarization governed by the…

Mesoscale and Nanoscale Physics · Physics 2017-11-15 Natalie Jäschke , Andreas Fischer , E. Evers , V. V. Belykh , Alex Greilich , Manfred Bayer , Frithjof B. Anders

We report the detection and polarization of nuclear spins in diamond at room temperature by using a single nitrogen-vacancy (NV) center. We use Hartmann-Hahn double resonance to coherently enhance the signal from a single nuclear spin while…

We demonstrate dynamical nuclear spin polarization in the absence of an external magnetic field, by resonant circularly polarized optical excitation of a single electron or hole charged quantum dot. Optical pumping of the electron spin…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 C. W. Lai , P. Maletinsky , A. Badolato , A. Imamoglu

We have theoretically analyzed coherent nuclear-spin dynamics induced by electron transport through a quantum-dot spin valve. The hyperfine interaction between electron and nuclear spins in a quantum dot allows for the transfer of angular…

Mesoscale and Nanoscale Physics · Physics 2015-06-23 Stefano Chesi , W. A. Coish

We investigate interactions between electrons and nuclear spins by using the resistance (Rxx) peak which develops near filling factor n = 2/3 as a probe. By temporarily tuning n to a different value, ntemp, with a gate, the Rxx peak is…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 K. Hashimoto , K. Muraki , T. Saku , Y. Hirayama

The electron-nuclei (hyperfine) interaction is central to spin qubits in solid state systems. It can be a severe decoherence source but also allows dynamic access to the nuclear spin states. We study a double quantum dot exposed to an…

Mesoscale and Nanoscale Physics · Physics 2013-06-13 Gunnar Petersen , Eric A. Hoffmann , Dieter Schuh , Werner Wegscheider , Geza Giedke , Stefan Ludwig