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Dual-comb spectroscopy in the ultraviolet (UV) and visible would enable broad bandwidth electronic spectroscopy with unprecedented frequency resolution. However, there are significant challenges in generation, detection and processing of…

Novel table-top sources of extreme-ultraviolet light based on high-harmonic generation yield unique insight into the fundamental properties of molecules, nanomaterials, or correlated solids, and enable advanced applications in imaging or…

The optical frequency comb has made a significant impact in precision spectroscopy and on our ability to probe atomic, molecular and, recently, nuclear transitions to further our understanding of their fundamental properties and how their…

Optics · Physics 2026-02-17 John J. McCauley , DylanP. Tooley , R. Jason Jones

Refraction is a well-known optical phenomenon that alters the direction of light waves propagating through matter. Microscopes, lenses and prisms based on refraction are indispensable tools for controlling the properties of light beams at…

The generation of coherent light pulses in the extreme ultraviolet (XUV) spectral region with attosecond pulse durations constitutes the foundation of the field of attosecond science. Twenty years after the first demonstration of isolated…

The highly energetic photons of ultraviolet light drive electronic and rovibronic transitions in all molecular species. This radiation is thus a prime tool for strongly selective spectroscopic fingerprinting and real-time environmental…

The development of schemes for coherent nonlinear time-domain spectroscopy in the extreme-ultraviolet regime (XUV) has so far been impeded by experimental difficulties that arise at these short wavelengths. In this work we present a novel…

Recent progress in laser-based high-repetition rate extreme ultraviolet (EUV) lightsources and multidimensional photoelectron spectroscopy enable the build-up of a new generation of time-resolved photoemission experiments. Here, we present…

We report generation of spectrally bright vacuum ultraviolet (VUV) and deep UV (DUV) coherent radiations driven by quantum coherence in tunnel-ionized carbon monoxide (CO) molecules. Our technique allows us to switch between multiple…

The extreme ultraviolet (XUV) emission from dense plasmas generated with sub-10-fs laser pulses with varying peak intensities up to 3*10^16 W/cm^2 is investigated for different target materials. K shell spectra are obtained from low Z…

Plasma Physics · Physics 2009-11-13 J. Osterholz , F. Brandl , M. Cerchez , T. Fischer , D. Hemmers , B. Hidding , A. Pipahl , G. Pretzler , S. J. Rose , O. Willi

We analyze the spectral properties of high-order harmonic radiation with photon energies extending beyond the regular cutoff energy in standard high-order harmonic generation. The extension of the regular harmonic cutoff results from…

Atomic Physics · Physics 2026-01-30 R. Esteban Goetz , Anh-Thu Le

The lack of available table-top extreme ultraviolet (XUV) sources with high enough fluxes and coherence properties have limited the availability of nonlinear XUV and x-ray spectroscopies to free electron lasers (FEL). Here, we demonstrate…

A compact and robust coherent laser light source that provides spectral coverage from the ultraviolet to infrared is desirable for numerous applications, including heterodyne super resolution imaging[1], broadband infrared microscopy[2],…

The emission of high-order harmonics from solids \cite{ghimire11a,schubert14a,luu15a,golde08a} under intense laser-pulse irradiation is revolutionizing our understanding of strong-field solid-light interactions…

Waveform shaping and frequency synthesis based on waveform modulation is ubiquitous in electronics, telecommunication technology, and optics. For optical waveforms, the carrier frequency is on the order of several hundred THz, while the…

Vacuum ultraviolet (VUV) light is critical for the study of molecules and materials, but the generation of femtosecond pulses in the VUV region at high repetition rates has proven difficult. Here, we demonstrate the efficient generation of…

In this study the generation of energetic coherent extreme ultraviolet (XUV) radiation with controlled polarization, is reported. The XUV radiation results from the process of high harmonic generation (HHG), in a gas phase atomic medium,…

Atomic Physics · Physics 2021-06-17 E. Vassakis , I. Orfanos , I. Liontos , D. Charalambidis , P. Tzallas , E. Skantzakis

Infrared and visible light beams carrying orbital angular momentum (OAM) are currently thoroughly studied for their extremely broad applicative prospects, among which are quantum information, micromachining and diagnostic tools. Here we…

Optics · Physics 2016-08-31 R. Géneaux , A. Camper , T. Auguste , O. Gobert , J. Caillat , R. Taeïb , T. Ruchon