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Fundamental studies of the effect of specific ions on hydrophobic interactions are driven by the need to understand phenomena such as hydrophobically driven self-assembly or protein folding. Using beta-peptide-inspired nano-rods, we…

Chemical Physics · Physics 2016-08-08 Kai Huang , Sebastian Gast , C. Derek Ma , Nicholas L. Abbott , Izabela Szlufarska

A precise understanding of solvation is essential for rational search and design of electrolytes that can meet performance demands in Li-ion and beyond Li-ion batteries. In the context of Li-O$_2$ batteries, ion pairing is decisive in…

Intermolecular correlations in liquid acetonitrile (CH3CN) have been revisited by calculating orientational correlation functions. In the present approach, hydrogen atoms are included, so that a concept applicable for molecules of (nearly)…

Chemical Physics · Physics 2019-06-12 Szilvia Pothoczki , László Pusztai

In this work, we report the results from molecular dynamics simulations of lithium salt-ionic liquid electrolytes (ILEs) based either on the symmetric bis[(trifluoromethyl)sulfonyl]imide ($\text{TFSI}^-$) anion or its asymmetric analog…

Chemical Physics · Physics 2022-03-23 Alina Wettstein , Diddo Diddens , Andreas Heuer

We present a study of the isotropic-nematic interface in a system of hard spherocylinders. First we compare results from Monte Carlo simulations and Onsager density functional theory for the interfacial profiles of the orientational order…

Soft Condensed Matter · Physics 2009-11-11 S. Wolfsheimer , C. Tanase , K. Shundyak , R. van Roij , T. Schilling

We implement a comprehensive simulation of photon surface interactions using a Monte Carlo approach. This is effective in simulating the interaction of light with telescope mirrors and lenses. We use a full electromagnetic solution to…

Instrumentation and Methods for Astrophysics · Physics 2026-02-03 J. R. Peterson , D. Valls-Gabaud , A. Dutta , C. Kim , G. Sembroski

A theory is presented which allow us to accurately calculate the critical coagulation concentration (CCC) of hydrophobic colloidal suspensions. For positively charged particles the CCC's follow the Hofmeister (lyotropic) series. For…

Soft Condensed Matter · Physics 2011-06-07 Alexandre P. dos Santos , Yan Levin

We theoretically and experimentally investigate colloid-oil-water-interface interactions of charged, sterically stabilized, poly(methyl-methacrylate) colloidal particles dispersed in a low-polar oil (dielectric constant $\epsilon=5-10$)…

Progress in electrochemical applications of ionic liquids builds on an understanding of electrical double-layer. This computational study focuses on structure-determined quantities -- maximum packing density, potentials and capacitances --…

We calculate the ion and composition distributions around colloid particles in an aqueous mixture, accounting for preferential adsorption, electrostatic interaction, selective solvation among ions and polar molecules, and…

Soft Condensed Matter · Physics 2011-11-04 Ryuichi Okamoto , Akira Onuki

Grand canonical Monte Carlo simulation results are reported for an electric double layer modelled by a planar charged hard wall, anisotropic shape cations, and spherical anions at different electrolyte concentrations and asymmetric…

Soft Condensed Matter · Physics 2016-03-09 M. Kaja , S. Lamperski , W. Silvestre-Alcantara , L. B. Bhuiyan , D. Henderson

Monte Carlo simulations at constant pressure are performed to study coexistence and interfacial properties of the liquid-solid transition in hard spheres and in colloid-polymer mixtures. The latter system is described as a one-component…

Soft Condensed Matter · Physics 2015-05-18 T. Zykova-Timan , J. Horbach , K. Binder

Complex organic molecules (COMs) have been widely observed in molecular clouds and protostellar environments. One of the formation mechanisms of COMs is radical reactions on the icy grain surface driven by UV irradiation. While many…

Earth and Planetary Astrophysics · Physics 2024-06-04 Yoko Ochiai , Shigeru Ida , Daigo Shoji

(Abbreviated) In this paper we report on the development of a multiscale method for simulating complex liquid-liquid systems such as water in contact with oil containing asphaltenes. We consider simulations where water drops covered with…

The purpose of this study is to provide data for the primitive model of the electrical double layer, where ions are modeled as charged hard spheres, the solvent as an implicit dielectric background (with dielectric constant $\epsilon=…

Soft Condensed Matter · Physics 2017-12-01 Mónika Valiskó , Tamás Kristóf , Dirk Gillespie , Dezső Boda

We present Monte Carlo simulations of a coarse-grained model for Langmuir monolayers of amphiphile molecules on a polar substrate. The molecules are modelled as chains of Lennard-Jones beads, with one slightly larger end bead confined in a…

Soft Condensed Matter · Physics 2009-10-31 Christoph Stadler , Harald Lange , Friederike Schmid

The intercalation of alkali ions into layered materials has played an essential role in battery technology since the development of the first lithium-ion electrodes. Coulomb repulsion between the intercalants leads to ordering of the…

Colloidal particles suspended in liquid crystals can exhibit various effective anisotropic interactions that can be tuned and utilized in self-assembly processes. We simulate a two-dimensional system of hard disks suspended in a solution of…

Soft Condensed Matter · Physics 2020-07-30 David Müller , Tobias A. Kampmann , Jan Kierfeld

Ionic liquids (ILs) constitute one of the most active fields of research nowadays. Many organic and inorganic molecules can be converted into ions via relatively simple procedures. These ions can be combined into ILs. Amino acid based ILs…

Materials Science · Physics 2015-01-09 Eudes Eterno Fileti , Vitaly V. Chaban

Abstract. Ionic liquids (ILs) constitute an emerging field of research. New ILs are continuously introduced involving more and more organic and inorganic ions. Amino acid based ILs (AAILs) represent a specific interest due to their…

Materials Science · Physics 2014-07-23 Eudes Eterno Fileti , Vitaly V. Chaban