Related papers: Molecular beam depletion: a new approach
Molecules are ubiquitous in natural phenomena and man-made products, but their use in quantum optical applications has been hampered by incoherent internal vibrations and other phononic interactions with their environment. We have now…
The double laser pulse approach to relativistic electron beam (REB) collimation has been investigated at the LULI-ELFIE facility. In this scheme, the magnetic field generated by the first laser-driven REB is used to guide a second delayed…
The photon emission from a single molecule driven simultaneously by a laser and a slow electric radio frequency (rf) field is studied. We use a non-Hermitian Hamiltonian approach which accounts for the radiative decay of a two level system…
In this dissertation a simple Hamiltonian for a system of inter-acting molecules and radiation field is developed from a model of N Two-Level Molecules interacting, via a dipole approximation, with a single mode, quantized radiation field.…
We investigate photoisomerization (PI), the shape change of a molecule upon photoabsorption, in a dissipative environment using a simple spin-boson model. We identify two classes of environment depending on whether it "entangles" with the…
Recent Feshbach-resonance experiments with 85Rb Bose-Einstein condensates have led to a host of unexplained results: dramatic losses of condensate atoms for an across-resonance sweep of the magnetic field, a collapsing condensate with a…
Two-photon Raman excitation between the ground hyperfine states $|5 \ ^2S_{1/2}, F = 2\rangle$ and $|5 \ ^2S_{1/2}, F = 1\rangle$ of $^{87}$Rb atom has been experimentally studied. The Rabi coupling strengths of various transition involved…
We investigate the interaction of two two-level atoms with a single mode cavity field. One of the atoms is exactly at resonance with the field, while the other is well far from resonance and hence is treated in the dispersive limit. We find…
We give a theoretical treatment of the interaction of electronic excitations (excitons) in biomolecules and quantum dots with the surrounding polar solvent. Significant quantum decoherence occurs due to the interaction of the electric…
This paper presents an analysis of a model problem, consisting of two interacting rigid rings, for the rotation of molecules in liquid $^4$He. Due to Bose symmetry, the excitation of the rotor corresponding to a ring of N helium atoms is…
We thoroughly investigate vibrational quantum dynamics of dimers attached to He droplets motivated by recent measurements with K-2 [1]. For those femtosecond pump-probe experiments, crucial observed features are not reproduced by gas phase…
Understanding ultracold collisions involving molecules is of fundamental importance for current experiments, where inelastic collisions typically limit the lifetime of molecular ensembles in optical traps. Here we present a broad study of…
Neutrinoless Double Beta Decay ($0\nu\beta\beta$) is presently the only known experiment to distinguisch between Dirac neutrinos, different from their antiparticles, and Majorana neutrinos, identical with their antiparticles. In addition…
We present various techniques that make orbit-following Monte Carlo simulations faster and more reliable when assessing collisionless fast particle losses due to magnetic field perturbations. These techniques are based on identifying…
We present a quantum optics-based detection method for determining the position and current of an electron beam. As electrons pass through a dilute vapor of rubidium atoms, their magnetic field perturb the atomic spin's quantum state and…
In recent studies it has become increasingly clear that presence of infinitely many instability bands of the parametric resonance plays crucial roles in the phenomenon of particle production under periodic classical field oscillation. We…
We study dipolar relaxation in both ultra-cold thermal and Bose-condensed chromium atom gases. We show three different ways to control dipolar relaxation, making use of either a static magnetic field, an oscillatory magnetic field, or an…
There is substantial interest in producing samples of ultracold molecules for possible applications in quantum computation, quantum simulation of condensed matter systems, precision measurements, controlled chemistry, and high precision…
We outline a general strategy for measuring spins, couplings and mixing angles in the case of a heavy partner decay chain terminating in an invisible particle. We consider the common example of a new scalar or fermion D decaying…
Exploring inelastic and reactive collisions on the quantum level is a main goal of the developing field of ultracold chemistry. We present first experimental studies of inelastic collisions of metastable ultracold triplet molecules in the…