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Kohn-Sham density functional theory (DFT) is the standard method for first-principles calculations in computational chemistry and materials science. More accurate theories such as the random-phase approximation (RPA) are limited in…

Materials Science · Physics 2023-10-25 Stefan Riemelmoser , Carla Verdi , Merzuk Kaltak , Georg Kresse

Isoscalar dipole strength distributions in spherical medium- and heavy-mass nuclei are calculated within random phase approximation (RPA) or quasiparticle RPA. Different Skyrme-type interactions corresponding to incompressibilities in the…

Nuclear Theory · Physics 2009-11-06 G. Colo` , N. Van Giai , P. F. Bortignon , M. R. Quaglia

We compare two different approaches to investigations of many-electron systems. The first is the Hartree-Fock (HF) method and the second is the Density Functional Theory (DFT). Overview of the main features and peculiar properties of the HF…

Materials Science · Physics 2009-11-07 M. Ya. Amusia , A. Z. Msezane , V. R. Shaginyan

The collective excitation phenomena in atomic nuclei are studied in two different formulations of the Random Phase Approximation (RPA): (i) RPA based on correlated realistic nucleon-nucleon interactions constructed within the Unitary…

Nuclear Theory · Physics 2009-11-11 N. Paar , P. Papakonstantinou , H. Hergert , R. Roth

We propose a high-speed and accurate hybrid dynamic density functional theory for the computer simulations of the phase separation processes of polymer melts and blends. The proposed theory is a combination of the dynamic self-consistent…

Soft Condensed Matter · Physics 2009-11-11 Takashi Honda , Toshihiro Kawakatsu

Kernel methods are powerful learning methodologies that allow to perform non-linear data analysis. Despite their popularity, they suffer from poor scalability in big data scenarios. Various approximation methods, including random feature…

Machine Learning · Statistics 2022-06-14 Bharath Sriperumbudur , Nicholas Sterge

We extend the capabilities of correlation energy functionals based on the adiabatic-connection fluctuation-dissipation theorem by implementing the analytical atomic forces within the random phase approximation (RPA), in the context of plane…

Materials Science · Physics 2026-03-19 Damian Contant , Maria Hellgren

Dielectric-dependent hybrid (DDH) functionals were recently shown to yield accurate energy gaps and dielectric constants for a wide variety of solids, at a computational cost considerably less than that of GW calculations. The fraction of…

Materials Science · Physics 2016-06-08 Jonathan H Skone , Marco Govoni , Giulia Galli

We investigate the behaviour of randomly cross-linked (co)polymer blends using a combination of replica theory and large-scale molecular dynamics simulations. In particular, we derive the analogue of the random phase approximation for…

Soft Condensed Matter · Physics 2009-11-13 A. V. Klopper , Carsten Svaneborg , Ralf Everaers

We have developed a fully consistent framework for calculations in the Quasiparticle Random Phase Approximation (QRPA) with $NN$ interactions from the Similarity Renormalization Group (SRG) and other unitary transformations of realistic…

Nuclear Theory · Physics 2011-07-04 H. Hergert , P. Papakonstantinou , R. Roth

The repulsive interaction between two atoms at short distances is studied in order to explore the range of validity of standard first-principles simulation techniques and improve the available short-range potentials for the description of…

Materials Science · Physics 2007-05-23 J. M. Pruneda , E. Artacho

We study the collective excitation spectrum of a d=3 site-disordered Anderson-Hubbard model at half-filling, via a random-phase approximation (RPA) about broken-symmetry, inhomogeneous unrestricted Hartree-Fock (UHF) ground states. We focus…

Strongly Correlated Electrons · Physics 2009-10-31 Yolande H. Szczech , Michael A. Tusch , David E. Logan

The random-phase approximation (RPA) as an approach for computing the electronic correlation energy is reviewed. After a brief account of its basic concept and historical development, the paper is devoted to the theoretical formulations of…

Materials Science · Physics 2017-07-26 Xinguo Ren , Patrick Rinke , Christian Joas , Matthias Scheffler

Ensemble density-functional theory (eDFT) suffers from the so-called "ghost interaction" error when approximate exchange-correlation functionals are used. In this work, we present a rigorous ghost interaction correction (GIC) scheme in the…

Chemical Physics · Physics 2016-07-21 Md. Mehboob Alam , Stefan Knecht , Emmanuel Fromager

Using the optimized effective potential method in conjunction with the semi-analytical approximation due to Krieger, Li and Iafrate, we have performed fully self-consistent exact exchange-only density-functional calculations for diatomic…

chem-ph · Physics 2008-02-03 T. Grabo , E. K. U. Gross

We propose a range-separated hybrid exchange-correlation functional to calculate solid-state material properties. The functional mixes Hartree-Fock exchange with the semilocal exchange of the meta-generalized gradient approximation…

Materials Science · Physics 2025-02-27 Subrata Jana , Abhishek Bhattacharjee , Suman Mahakal , Szymon Smiga , Prasanjit Samal

We present a low-scaling algorithm for the random phase approximation (RPA) with \textbf{k}-point sampling in the framework of tensor hypercontraction (THC) for electron repulsion integrals (ERIs). The THC factorization is obtained via a…

Materials Science · Physics 2023-12-01 Chia-Nan Yeh , Miguel A. Morales

Biologically functional liquid-liquid phase separation of intrinsically disordered proteins (IDPs) is driven by interactions encoded by their amino acid sequences. Little is currently known about the molecular recognition mechanisms for…

Biomolecules · Quantitative Biology 2017-11-15 Yi-Hsuan Lin , Jacob P. Brady , Julie D. Forman-Kay , Hue Sun Chan

A systematic analysis of giant quadrupole resonances is performed for several nuclei, from $^{30}$Si to $^{208}$Pb, within the subtracted second random--phase--approximation (SSRPA) model in the framework of the energy--density--functional…

Nuclear Theory · Physics 2018-10-17 Olivier Vasseur , Danilo Gambacurta , Marcella Grasso

We have used the Hartree-Fock Random Phase Approximation (HF-RPA) to study the interacting electron gas in a quantum wire. The spectra of intersubband spin-flip excitations reveal a considerable red shift with respect to single-particle HF…

Condensed Matter · Physics 2009-10-28 Arne Brataas , A. G. Mal'shukov , Vidar Gudmundsson , K. A. Chao
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