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We investigate the experimental signatures of Raman spectroscopy of bi- and tri-magnon excitations in the distorted triangular lattice antiferromagnets alpha-LCr2O4 (L=Sr, Ca). We utilize spin wave theory to analyze the nearly 120 degree…

Strongly Correlated Electrons · Physics 2023-05-23 Junli Li , Shangjian Jin , Trinanjan Datta , Dao-Xin Yao

Spin-phonon coupling, the interaction of spins with surrounding lattice is a key parameter to understand the underlying physics of multiferroics and engineer their magnetization dynamics. Elementary excitations in multiferroic materials are…

Materials Science · Physics 2020-11-05 Bommareddy Poojitha , Anjali Rathore , Ankit Kumar , Surajit Saha

The temperature and magnetic field dependence of lattice and carrier excitations in MnSi is studied in detail using inelastic light scattering. The pure symmetry components of the electronic response are derived from the polarization…

Strongly Correlated Electrons · Physics 2014-07-23 H. -M. Eiter , P. Jaschke , R. Hackl , A. Bauer , M. Gangl , C. Pfleiderer

We determine the nature of coupled phonons and magnetic excitations in AlFeO3 using inelastic light scattering from 5 K to 315 K covering a spectral range from 100-2200 cm-1 and complementary first-principles density functional theory-based…

Strongly Correlated Electrons · Physics 2012-05-01 Pradeep Kumar , A. Bera , D. V. S. Muthu , S. N. Shirodkar , R. Saha , A. Shireen , A. Sundaresan , U. V. Waghmare , A. K. Sood , C. N. R. Rao

We have performed Raman scattering investigations on the high energy magnetic excitations in a BiFeO$_3$ single crystal as a function of both temperature and laser excitation energy. A strong feature observed at 1250 cm$^{-1}$ in the Raman…

Strongly Correlated Electrons · Physics 2018-11-13 M. Cazayous , A. Sacuto , D. Lebeugle , D. Colson

The spin dynamics and magnetic excitations of the slightly distorted triangular s = 3/2 system alpha-CaCr2O4 are investigated by means of Raman spectroscopy and electron spin resonance (ESR) to elucidate its peculiar magnetic properties.…

Understanding the coupling between lattice vibrations and magnetic order is crucial for controlling properties of two-dimensional magnetic materials. Here, we investigate the vibrational properties of bulk and thick-flake CrCl$_\textrm{3}$…

Layered antiferromagnetic materials have emerged as a novel subset of the two-dimensional family providing a highly accessible regime with prospects for layer-number-dependent magnetism. Furthermore, transition metal phosphorous…

Materials Science · Physics 2024-01-09 Daniel J. Gillard , Daniel Wolverson , Oscar M. Hutchings , Alexander I. Tartakovskii

We have used Raman scattering to investigate the magnetic excitations and lattice dynamics in the prototypical spin-orbit Mott insulators Sr2IrO4 and Sr3Ir2O7. Both compounds exhibit pronounced two-magnon Raman scattering features with…

Strongly Correlated Electrons · Physics 2016-04-06 H. Gretarsson , N. H. Sung , M. Hoeppner , B. J. Kim , B. Keimer , M. Le Tacon

We report an inelastic light scattering study of single-crystalline NaCu$_2$O$_2$, a spin-chain compound known to exhibit a phase with helical magnetic order at low temperatures. Phonon excitations were studied as a function of temperature…

Strongly Correlated Electrons · Physics 2009-11-11 K. -Y. Choi , V. P. Gnezdilov , P. Lemmens , L. Capogna , M. R. Johnson , M. Sofin , A. Maljuk , M. Jansen , B. Keimer

We present a Raman scattering study of Ca$_2$RuO$_4$, in which we investigate the temperature-dependence of the lattice dynamics and the electron-phonon interaction below the metal-insulator transition temperature ({\it T}$_{\rm MI}$).…

Strongly Correlated Electrons · Physics 2009-11-11 H. Rho , S. L. Cooper , S. Nakatsuji , H. Fukazawa , Y. Maeno

We used Raman and terahertz spectroscopies to investigate lattice and magnetic excitations and their cross-coupling in the hexagonal YMnO3 multiferroic. Two phonon modes are strongly affected by the magnetic order. Magnon excitations have…

We use Raman scattering to study spin, charge, and lattice dynamics in various phases of Ca_{2-x}Sr_{x}RuO_{4}. With increasing substitution of Ca by Sr in the range 0 =< x < 0.2, we observe (1) evidence for an increase of the…

Strongly Correlated Electrons · Physics 2009-11-10 H. Rho , S. L. Cooper , S. Nakatsuji , H. Fukazawa , Y. Maeno

Magneto-Raman spectroscopy is applied to study spin-phonon coupling in the layered two-dimensional (2D) van der Waals antiferromagnet CrSBr. We report on the effects of temperature and external magnetic field on Raman-active phonons of…

Materials Science · Physics 2025-03-20 Urszula D. Wdowik , Vaibhav Varade , Jana Vejpravova , Dominik Legut

We report low-temperature Raman signatures of the Heisenberg quantum magnet Ca$_{10}$Cr$_7$O$_{28}$, showing clear anomalies in phonon mode frequencies and linewidths below $\sim$100 K. This crossover temperature lies in between the…

Strongly Correlated Electrons · Physics 2023-12-12 Srishti Pal , Arnab Seth , Anzar Ali , Yogesh Singh , D. V. S. Muthu , Subhro Bhattacharjee , A. K. Sood

The ferrimagnetic spinels MnB2O4 (B = Mn,V) exhibit a similar series of closely spaced magnetic and structural phase transitions at low temperatures, reflecting both magnetic frustration and a strong coupling between the spin and lattice…

Strongly Correlated Electrons · Physics 2015-01-28 S. L. Gleason , T. Byrum , Y. Gim , A. Thaler , P. Abbamonte , G. J. MacDougall , L. W. Martin , H. D. Zhou , S. L. Cooper

In this letter we investigated the temperature-dependent Raman spectra of CaMn7O12 helimagnet from room temperature down to 10 K. The temperature dependence of the Raman mode parameters show remarkable anomalies for both antiferromagnetic…

We investigate the two-magnon Raman scattering from an anisotropic S=1/2 triangular Heisenberg antiferromagnet Cs2CuCl4. We find that the Raman response is very sensitive to magnon-magnon interactions and to scattering geometries, a feature…

Strongly Correlated Electrons · Physics 2015-06-12 Natalia B. Perkins , Gia-Wei Chern , Wolfram Brenig

We use polarized magneto-Raman scattering to study purely electronic excitations and the electron-phonon coupling in bulk graphite. At a temperature of 4.2 K and in magnetic fields up to 28 T we observe $K$-point electronic excitations…

Mesoscale and Nanoscale Physics · Physics 2015-05-30 P. Kossacki , C. Faugeras , M. Kühne , M. Orlita , A. A. L. Nicolet , J. M. Schneider , D. M. Basko , Y. I. Latyshev , M. Potemski

The interplay between spin dynamics and lattice vibration has been suggested as an important part of the puzzle of high-temperature superconductivity. Here we report the strong interaction between spin fluctuation and phonon in SmFeAsO, a…

Superconductivity · Physics 2010-10-29 L. Zhang , P. F. Guan , D. L. Feng , X. H. Chen , S. S. Xie , M. W. Chen
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