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Related papers: Orbital-dependent singlet dimers and orbital-selec…

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In the present review different effects related to the orbital degrees of freedom are discussed. Leaving aside such aspects as the superexchange mechanism of the cooperative Jahn-Teller distortions and different properties of…

Strongly Correlated Electrons · Physics 2018-03-12 S. V. Streltsov , D. I. Khomskii

It has been suggested that the metal-insulator transitions in a number of spinel materials with partially-filled t_2g d-orbitals can be explained as orbitally-driven Peierls instabilities. Motivated by these suggestions, we examine…

Strongly Correlated Electrons · Physics 2014-07-28 R. T. Clay , H. Li , S. Sarkar , S. Mazumdar , T. Saha-Dasgupta

We consider the superstructures, which can be formed in spinels containing on B-sites the transition-metal ions with partially filled t2g levels. We show that, when such systems are close to itinerant state (e.g. have an insulator-metal…

Strongly Correlated Electrons · Physics 2009-11-10 D. I. Khomskii , T. Mizokawa

We report a quantum phase transition between orbital-selective Mott states, with different localized orbitals, in a Hund's metals model. Using the density matrix renormalization group, the phase diagram is constructed varying the electronic…

Strongly Correlated Electrons · Physics 2014-12-09 Julian Rincon , Adriana Moreo , Gonzalo Alvarez , Elbio Dagotto

We experimentally realize a Peierls phase in the hopping amplitude of excitations carried by Rydberg atoms, and observe the resulting characteristic chiral motion in a minimal setup of three sites. Our demonstration relies on the intrinsic…

The role of orbital ordering on metal-insulator transition of transition-metal oxides is investigated by the cluster self-consistent field approach in the strong correlation regime. A clear dependence of the insulating gap on the orbital…

Strongly Correlated Electrons · Physics 2007-09-25 Dong-Meng Chen , Liang-Jian Zou

We review theoretical investigations on the origin of the orbital selective phase where localized and itinerant electrons coexist in the d shell at intermediate strength of the on-site Coulomb interactions between electrons. In particular,…

Strongly Correlated Electrons · Physics 2014-03-10 Yao Yao , Yu-Zhong Zhang , Hunpyo Lee , Harald O. Jeschke , Roser Valenti , Hai-Qing Lin , Chang-Qin Wu

We study \textit{ab initio} a pyrochlore compound, CsW$_{2}$O$_{6}$, which exhibits a yet unexplained metal-insulator transition. We find that (1) the reported low-$T$ structure is likely inaccurate and the correct structure has a twice…

Superconductivity · Physics 2017-01-10 S. V. Streltsov , I. I. Mazin , R. Heid , K. -P. Bohnen

Based on the analysis of a two-orbital Hubbard model within a mean-field approach, we propose a mechanism for an orbital selective phase transition (OSPT) where coexistence of localized and itinerant electrons can be realized. We show that…

Strongly Correlated Electrons · Physics 2012-01-31 Yu-Zhong Zhang , Hunpyo Lee , Hai-Qing Lin , Chang-Qin Wu , Harald O. Jeschke , Roser Valenti

We investigate the violation of the first Hund's rule in 4$d$ and 5$d$ transition metal oxides that form solids of dimers. Bonding states within these dimers reduce the magnetization of such materials. We parametrize the dimer formation…

Strongly Correlated Electrons · Physics 2019-01-16 Malte Harland , Alexander I. Poteryaev , Sergey V. Streltsov , Alexander I. Lichtenstein

The electronic properties of quarter-filled organic materials showing spin-Peierls transition are investigated theoretically. By studying the one-dimensional extended Peierls-Hubbard model analytically as well as numerically, we find that…

Strongly Correlated Electrons · Physics 2007-05-23 Makoto Kuwabara , Hitoshi Seo , Masao Ogata

We consider the dimer Hubbard model within Dynamical Mean Field Theory to study the interplay and competition between Mott and Peierls physics. We describe the various metal-insulator transition lines of the phase diagram and the break down…

Strongly Correlated Electrons · Physics 2018-01-17 O. Nájera , M. Civelli , V. Dobrosavljević , M. J. Rozenberg

The properties of transition metal compounds are largely determined by nontrivial interplay of different degrees of freedom: charge, spin, lattice, but also orbital ones. Especially rich and interesting effects occur in systems with orbital…

Strongly Correlated Electrons · Physics 2021-04-22 D. I. Khomskii , S. V. Streltsov

Using {\it ab initio} density functional theory, here we systematically study the monolayer MoOCl$_2$ with a $4d^2$ electronic configuration. Our main results is that an orbital-selective Peierls phase (OSPP) develops in MoOCl$_2$,…

Strongly Correlated Electrons · Physics 2021-08-11 Yang Zhang , Ling-Fang Lin , Adriana Moreo , Elbio Dagotto

We summarize some characteristic features of the frustrated magnetic interactions in spin-orbital models adequate for cubic transition metal oxides with orbital degeneracy. A generic tendency towards dimerization, found already in the…

Strongly Correlated Electrons · Physics 2015-06-24 Andrzej M. Oles

Interaction-driven metal-insulator transitions or Mott transitions are widely observed in condensed-matter systems. In multi-orbital systems, many-body physics is richer in which an orbital-selective metal-insulator transition is an…

Strongly Correlated Electrons · Physics 2018-11-09 Hanghui Chen

We use first principles density functional theory calculations to examine the effect of multiple anions on the Peierls distortion in the rutile oxyfluoride TiOF. By using a structure enumeration approach, we obtain the ground state atomic…

Materials Science · Physics 2024-05-14 Siddhartha S. Nathan , Danilo Puggioni , James M. Rondinelli

Orbital differentiation is a common theme in multiorbital systems, yet a complete understanding of it is still missing. Here, we consider a minimal model for orbital differentiation in Hund metals with a highly accurate method: We use the…

Strongly Correlated Electrons · Physics 2020-01-08 Fabian B. Kugler , Seung-Sup B. Lee , Andreas Weichselbaum , Gabriel Kotliar , Jan von Delft

We found direct experimental evidence for an orbital switching in the V 3d states across the metal-insulator transition in VO$_{2}$. We have used soft-x-ray absorption spectroscopy at the V $L_{2,3}$ edges as a sensitive local probe, and…

Spin- or orbital-selective behaviours in correlated electron materials offer rich promise for spintronics or orbitronics phenomena and applications deriving from them. Strong local electronic Coulomb correlations might lead to an…

Strongly Correlated Electrons · Physics 2024-06-03 Evgeny A. Stepanov , Silke Biermann
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