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Electron injection from an adsorbed molecule to the substrate (heterogeneous electron transfer) is studied. One reaction coordinate is used to model this process. The surface phonons and/or the electron-hole pairs together with the internal…

Chemical Physics · Physics 2009-11-07 Michael Schreiber , Ivan Kondov , Ulrich Kleinekathoefer

The influence of molecular vibrations on dissociative adsorption is studied by six-dimensional quantum dynamical calculations. For the system H_2 at Pd(100), which possesses non-activated pathways, it is shown that large vibrational effects…

mtrl-th · Physics 2009-10-30 Axel Gross , Matthias Scheffler

Nonlinear oscillations are commonly observed in complex systems far from equilibrium, such as living organisms. These oscillations are essential for sustaining vital processes, like neuronal firing, circadian rhythms, and heartbeats. In…

Statistical Mechanics · Physics 2026-04-15 Daiki Sekizawa , Sosuke Ito , Masafumi Oizumi

Recent experiments have shown that highly efficient energy transfer can take place in organic nanocrystals at extremely low acceptor densities. This striking phenomenon has been ascribed to the formation of exciton polaritons thanks to the…

Chemical Physics · Physics 2021-01-12 R. Sáez-Blázquez , J. Feist , F. J. García-Vidal , A. I. Fernández-Domínguez

We present here a brief overview of our work in developing a convolutionless quantum master equation approach suitable for mesoscopic sized systems. Our final equation can be used in the regimes where the golden rule approach is not…

Materials Science · Physics 2007-05-23 Eric R. Bittner , Andrey Pereverzev

We consider the reduced dynamics of a molecular chain weakly coupled to a phonon bath. With a small and constant inhomogeneity in the coupling, the excitation relaxation rates are obtained in closed form. They are dominated by transitions…

Statistical Mechanics · Physics 2021-04-16 B. A. Tay

We investigate how a single resonator with a time-modulated component extracts power from an external ambient source. However, the collected power is largely dependent on the precise choice of the modulation signal frequency. We focus on…

Applied Physics · Physics 2023-03-21 Alireza Nikzamir , Kasra Rouhi , Alexander Figotin , Filippo Capolino

In organic photovoltaic (OPV) systems, exciton dissociation and ultrafast charge separation at donor-acceptor heterojunctions both play a key role in controlling the efficiency of the conversion of excitation energy into free charge…

Chemical Physics · Physics 2020-07-01 Aaron Kelly

A multimode microcavity sensor based on a self-interference microring resonator is demonstrated experimentally. The proposed multimode sensing method is implemented by recording wideband transmission spectra that consist of multiple…

Dissipative optomechanics studies the coupling of the motion of an optical element to the decay rate of a cavity. We propose and theoretically explore a realization of this system in the optical domain, using a combined Michelson--Sagnac…

Optics · Physics 2011-11-17 André Xuereb , Roman Schnabel , Klemens Hammerer

A strong electromagnetic field interacting with an electron system generates both the Rabi oscillations and the Stark splitting of the electron density. Changing of the electron density gives rise to nonadiabatic effects due to existence of…

Mesoscale and Nanoscale Physics · Physics 2018-02-14 Andrei Ivanov

Based on the reduced density matrix method, we compare two different approaches to calculate the dynamics of the electron transfer in systems with donor, bridge, and acceptor. In the first approach a vibrational substructure is taken into…

Quantum Physics · Physics 2009-10-31 M. Schreiber , D. Kilin , U. Kleinekathoefer

Large exciton diffusion lengths generally improve the performance of organic semiconductor devices, since they enable energy to be transported farther during the exciton lifetime. However, the physics of exciton motion in disordered organic…

Chemical Physics · Physics 2023-03-17 Daniel Balzer , Ivan Kassal

Molecular vibrations play a critical role in the charge transport properties of weakly van der Waals bonded organic semiconductors. To understand which specific phonon modes contribute most strongly to the electron-phonon coupling and…

We present a combined treatment of the non-equilibrium dynamics and transport of electrons and phonons by carrying out \textit{ab initio} calculations of the fully coupled electron and phonon Boltzmann transport equations. We find that the…

Materials Science · Physics 2020-12-30 Nakib H. Protik , Boris Kozinsky

The reshaping and decorrelation of similar activity patterns by neuronal networks can enhance their discriminability, storage, and retrieval. How can such networks learn to decorrelate new complex patterns, as they arise in the olfactory…

Neurons and Cognition · Quantitative Biology 2015-06-04 Siu-Fai Chow , Stuart D. Wick , Hermann Riecke

We develop a classical microscopic model of a dielectric. The model features nonlinear interaction terms between polarizable dipoles and lattice vibrations. The lattice vibrations are found to act as a pseudo-reservoir, giving broadband…

Optics · Physics 2016-07-20 R. J. Churchill , T. G. Philbin

In this paper we consider the essential electronic excited states in parallel chains of semiconducting polymers that are currently being explored for photovoltaic and light-emitting diode applications. In particular, we focus upon various…

Materials Science · Physics 2009-11-11 Eric R. Bittner , John Glenn Santos Ramon , Stoyan Karabunarliev

Non-reciprocal devices are key components in both classical and quantum electronics. One approach to realizing passive non-reciprocal microwave devices is through capacitive coupling between external electrodes and materials exhibiting…

Mesoscale and Nanoscale Physics · Physics 2025-09-03 Stefano Bosco

The presence of magnetic fields and/or transport currents can cause penetration of vortices in superconductors. Their motion leads to dissipation and resistive state arises, which in turn strongly affects the performance of superconducting…

Superconductivity · Physics 2022-09-26 E. C. S. Duarte , E. Sardella , T. T. Saraiva , A. S. Vasenko , R. Zadorosny
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