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Multiferroic materials, which reveal magnetic and electric order, are in the focus of recent solid state research. Especially the simultaneous occurrence of ferroelectricity and ferromagnetism, combined with an intimate coupling of…

Strongly Correlated Electrons · Physics 2009-11-11 J. Hemberger , P. Lunkenheimer , R. Fichtl , H. -A. Krug von Nidda , V. Tsurkan , A. Loidl

We report here a comprehensive study on structural, magnetic, caloric and electronic properties of the monoclinic phase of double perovskite compound Tm2CoMnO6 (TCMO) in its polycrysttaline format. Magnetic measurements confirm the presence…

Materials Science · Physics 2023-07-13 A. Banerjee , Gangadhar Das , V. Rajaji , S. Majumdar , P. K. Chakrabarti

Multiferroicity and magnetodielectric coupling in metal-organic-frameworks (MOFs) is rare and so far restricted mainly to formate-based systems with perovskite structure. In the course of this work we designed a tetragonal framework…

Materials Science · Physics 2017-10-31 Tathamay Basu , A. Jesche , B. Bredenkotter , M. Grzywa , D. Denysenko , D. Volkmer , A. Loidl , S. Krohns

Perovskite manganites with small A-site ions, as the first and canonical branch of type-II multiferroics, are ideal systems to exhibit magnetism-induced ferroelectricity. Despite their established magnetoelectric phase diagrams under low…

Materials Science · Physics 2026-01-15 Ming Yang , Jun Chen , Junfeng Wang , Chao Dong , Chengliang Lu , Gang Xu , Jinguang Cheng , Jianshi Zhou , Shuai Dong

The emergence of altermagnets establishes a new paradigm for multiferroics. Unlike conventional multiferroics relying on direct magnetoelectric coupling, multiferroic altermagnets host a crystal-symmetry-mediated magnetoelectric interaction…

Materials Science · Physics 2026-01-12 Zhou Cui , Ziye Zhu , Xunkai Duan , Bowen Hao , Xianzhang Chen , Jiayong Zhang , Tong Zhou

There has been tremendous research activity in the field of magneto-electric (ME) multiferroics after Kimura et al. [1] showed that antiferromagnetic and ferroelectric order coexist in orthorhom- bically distorted perovskite TbMnO3 and are…

We have investigated dielectric properties in a series of crystals of $R$MnO$_{3}$ ($R$ is a rare earth ion) under magnetic fields and quasihydrostatic pressure. We have found that ferroelectric phase appeared in GdMnO$_3$ crystal below…

Strongly Correlated Electrons · Physics 2009-11-10 H. Kuwahara , K. Noda , J. Nagayama , S. Nakamura

Pyroxenes with the general formula $AM$Si$_2$O$_6$ ($A$ = mono- or divalent metal, $M$ = di- or trivalent metal) are shown to be a new class of multiferroic materials. In particular, we have found so far that NaFeSi$_2$O$_6$ becomes…

Strongly Correlated Electrons · Physics 2015-05-13 S. Jodlauk , P. Becker , J. A. Mydosh , D. I. Khomskii , T. Lorenz , S. V. Streltsov , D. C. Hezel , L. Bohaty

Double perovskite-based magnets wherein frustration and competition between emergent degrees of freedom are at play can lead to novel electronic and magnetic phenomena. Herein, we report the electronic structure and magnetic properties of…

Recently, the perovskite BiCoO$_3$ has been shown experimentally to be isostructural with PbTiO$_3$, while simultaneously the $d^6$ Co$^{3+}$ ion has a high spin ground state with $C$-type antiferromagnetic ordering. Using hybrid density…

Materials Science · Physics 2016-05-04 Leigh Weston , Xiangyuan Cui , Simon P. Ringer , Catherine Stampfl

The dielectric behavior of the single crystals of the spin-chain system Ca3Co2O6, undergoing geometrically frustrated antiferromagnetic ordering below 25 K, has been investigated as a function of temperature and magnetic field (H) and…

Materials Science · Physics 2016-03-17 Tathamay Basu , Kartik K. Iyer , P. L. Paulose , E. V. Sampathkumaran

We investigated the anisotropy of the magnetic and magnetocaloric properties of singlecrystalline double perovskite Tb2CoMnO6, which crystallizes in a monoclinic P21/n structure. Due to dissimilar magnetic anisotropy, the ferromagnetic…

Strongly Correlated Electrons · Physics 2018-12-17 J. Y. Moon , M. K. Kim , D. G. Oh , J. H. Kim , H. J. Shin , Y. J. Choi , N. Lee

In the present investigation, some novel magnetic behaviors exhibited by double perovskite (DP) Eu2CoMnO6(ECMO) has been reported. XRD analysis of ECMO showed that it has a monoclinic crystal structure (space group P 21/n). A second-order…

Materials Science · Physics 2019-09-30 Mohd Alam , Arkadeb Pal , Khyati Anand , Prajyoti Singh , Sandip Chatterjee

We describe the design of a new magnetic ferroelectric with large spontaneous magnetization and polarization using first-principles density functional theory. The usual difficulties associated with the production of robustly-insulating…

Materials Science · Physics 2011-11-09 Pio Baettig , Nicola Spaldin

Ferroic multipole orders break some symmetry and often activate unique physical properties, such as nonreciprocal directional dichroism and linear magnetoelectric effects. Here, we demonstrate the control of magnetic toroidal orientation in…

Strongly Correlated Electrons · Physics 2026-04-02 Shungo Aoyagi , Shunsuke Kitou , Taka-hisa Arima , Yusuke Tokunaga

The spin-driven component of electric polarization in a single crystal of multiferroic BiFeO$_{3}$ was experimentally investigated in pulsed high magnetic fields up to 41 T. Sequential measurements of electric polarization for various…

Strongly Correlated Electrons · Physics 2020-01-08 Shiro Kawachi , Shin Miyahara , Toshimitsu Ito , Atsushi Miyake , Nobuo Furukawa , Jun-ichi Yamaura , Masashi Tokunaga

Trirutile-type LiFe$_2$F$_6$ is a charge-ordered material with Fe$^{2+}$/Fe$^{3+}$ configuration. Here its physical properties, including magnetism, electronic structure, phase transition, and charge ordering, are studied theoretically. On…

Materials Science · Physics 2017-12-11 Ling-Fang Lin , Qiao-Ru Xu , Yang Zhang , Jun-Jie Zhang , Yan-Ping Liang , Shuai Dong

We have investigated the magnetoelectric coupling in the lone pair containing piezoelectric ferrimagnet Cu2OSeO3. Significant magnetocapacitance develops in the magnetically ordered state (TC = 60 K). We find critical behavior near TC and a…

Materials Science · Physics 2010-02-25 Jan-Willem G. Bos , Claire V. Colin , Thomas T. M. Palstra

The magnetic susceptibility, crystal and magnetic structures, and electronic structure of double perovskite Sr2ScOsO6 are reported. Using both neutron and x-ray powder diffraction we find that the crystal structure is monoclinic P21/n from…

Strongly Correlated Electrons · Physics 2015-04-06 A. E. Taylor , R. Morrow , D. J. Singh , S. Calder , M. D. Lumsden , P. M. Woodward , A. D. Christianson

We investigate a magnetic hysteresis loop with a remanent moment that couples to electric polarization to create coupled hysteretic multiferroic behavior in Lu2MnCoO6. Measurements of elastic neutron diffraction, muon spin relaxation, and…