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Working in the crystal-momentum representation, we calculate the optical conductivity of noncentrosymmetric insulating crystals at first order in the wave vector of light. The time-even part of this tensor describes natural optical activity…

Mesoscale and Nanoscale Physics · Physics 2010-12-30 Andrei Malashevich , Ivo Souza

Contrary to the optical spin angular momentum (SAM), the role played by the orbital angular momentum (OAM) of light in magneto-optics remains largely unexplored. However, the SAM and OAM are known to be coupled when light interacts with…

The Maxwell equations and the constitutive relations describe the classical propagation of electromagnetic waves in continuous matter. Here, we investigate the effects stemming from extended constitutive relations on the propagation of…

Classical Physics · Physics 2022-10-12 Pedro D. S. Silva , Rodolfo Casana , Manoel M. Ferreira

We derive the current response of noncentrosymmetric metal in normal and in superconducting states to the electromagnetic field with finite frequency and wave vector. The conductivity tensor is found contains the linear in wave vector off…

Strongly Correlated Electrons · Physics 2009-03-20 V. P. Mineev , Yu Yoshioka

Photoelectron circular dichroism refers to the forward/backward asymmetry in the photoelectron angular distribution with respect to the propagation axis of circularly polarized light. It has recently been demonstrated in femtosecond…

Quantum Physics · Physics 2017-01-16 R. E. Goetz , T. A. Isaev , B. Nikoobakht , R. Berger , C. P. Koch

Material anisotropy and chirality produce polarization-dependent light-matter interactions. Absorption leads to linear and circular dichroism, whereas elastic forward scattering produces linear and circular birefringence. Here we highlight…

Optics · Physics 2024-12-02 Kayn A. Forbes , Dale Green

The optical activity tensor (OAT) is explicitly derived. It is shown that to evaluate a large number of effects related to optical activity of some atomic/molecular system at arbitrary frequency $\omega$ of the incident light, one needs to…

Atomic and Molecular Clusters · Physics 2010-10-26 Alexei M. Frolov , David M. Wardlaw

We study light propagation in a medium with uniform torsion, modeled as a continuum of screw dislocations within the geometric theory of defects. By solving Maxwell's equations in covariant form, we show that torsion induces intrinsic…

Optics · Physics 2026-01-19 Humberto Belich , Edilberto O. Silva

Using 4x4 matrix formalism we analyzed electromagnetic wave propagation and Jones matrix components for reflectivity and transmittivity in bi-anisotropic materials. Analytic formulas for complex reflection and transmission coefficients for…

Optics · Physics 2011-05-26 P. D. Rogers , M. Kotelyanskii , A. A. Sirenko

The optical properties of some nanomaterials can be controlled by an external magnetic field, providing active functionalities for a wide range of applications, from single-molecule sensing to nanoscale nonreciprocal optical isolation.…

The phenomenon of molecular optical activity manifests itself as the rotation of the plane of linear polarization when light passes through chiral media. Measurements of optical activity and its wavelength dependence, optical rotatory…

We introduce chiral rotational spectroscopy: a new technique that enables the determination of the orientated optical activity pseudotensor components $B_{XX}$, $B_{YY}$ and $B_{ZZ}$ of chiral molecules, in a manner that reveals the…

Atomic and Molecular Clusters · Physics 2018-01-16 Robert P. Cameron , Jörg B. Götte , Stephen M. Barnett

We present an accurate and computationally efficient first-principles methodology to calculate the natural optical activity. Our approach is based on the long-wave density-functional perturbation theory and includes self-consistent field…

Materials Science · Physics 2023-04-04 Asier Zabalo , Massimiliano Stengel

It is shown theoretically that a nonchiral, two-dimensional array of metallic spheres exhibits optical activity as manifested in calculations of circular dichroism. The metallic spheres occupy the sites of a rectangular lattice and for…

Optics · Physics 2009-11-13 Vassilios Yannopapas

Inversion-symmetric crystals are optically isotropic and thus naively not expected to show dichroism effects in optical absorption and photoemission processes. Here, we find a strong linear dichroism effect (up to 42.4%) in the conduction…

Optical responses of ferromagnetic materials with spin gauge field that drives intrinsic spin curren is theoretically studied. The conductivity tensor is calculated based on a linear response theory to the applied electric field taking…

Mesoscale and Nanoscale Physics · Physics 2020-09-07 Evgeny Karashtin , Gen Tatara

Many wormlike micellar systems exhibit appreciable shear thinning due to shear induced alignment. As the micelles get aligned introducing directionality in the system, the viscoelastic properties are no longer expected to be isotropic. An…

Soft Condensed Matter · Physics 2011-05-09 Manas Khan , A. K. Sood

We discuss the expansion of interaction kernels between anisotropic rigid molecules. The expansion decouples the correlated orientational variables so that it can be utilized to derive macroscopic models. Symmetries of two types are…

Mathematical Physics · Physics 2022-11-09 Jie Xu

We present a theoretical analysis of photo-absorption spectroscopies in noncentrosymmetric systems, covering both x-ray and optical regions. Integrated dichroic spectra are interpreted using microscopic effective operators, which are…

Condensed Matter · Physics 2007-05-23 Paolo Carra , Andres Jerez , Ivan Marri

Optical activity is ubiquitous across natural and artificial media and is conventionally understood in terms of scattering from electric and magnetic moments. Here we demonstrate experimentally and confirm numerically a type of optical…