English
Related papers

Related papers: Landau-Zener type surface hopping algorithms

200 papers

With the aim of describing real-time electron dynamics, we introduce an adiabatic approximation for the equation of motion of the one-body reduced-density matrix (one-matrix). The eigenvalues of the one-matrix, which represent the…

Strongly Correlated Electrons · Physics 2012-09-18 Ryan Requist , Oleg Pankratov

We discuss solvable multistate Landau-Zener (MLZ) models whose Hamiltonians have commuting partner operators with $\sim 1/\tau$-time-dependent parameters. Many already known solvable MLZ models belong precisely to this class. We derive the…

Mathematical Physics · Physics 2020-06-29 Vladimir Y. Chernyak , Fuxiang Li , Chen Sun , Nikolai A. Sinitsyn

We generalize the Brundobler-Elser hypothesis in the multistate Landau-Zener problem to the case when instead of a state with the highest slope of the diabatic energy level there is a band of states with an arbitrary number of parallel…

Quantum Physics · Physics 2009-11-10 N. A. Sinitsyn

The powerful molecular dynamics (MD) simulation is basically based on a picture that the atoms experience classical-like trajectories under the exertion of classical force field determined by the quantum mechanically solved electronic…

Chemical Physics · Physics 2013-12-16 Wei Feng , Luting Xu , Xin-Qi Li , Weihai Fang

Non-adiabatic chemical reactions involving continuous circularly polarized light (cw CPL) have not attracted as much attention as dynamics in unpolarized/linearly polarized light. However, including circularly (in contrast to linearly)…

Chemical Physics · Physics 2022-09-20 Zeyu Zhou , Yanze Wu , Xuezhi Bian , Joseph Eli Subotnik

We study a nonlinear generalization of the Landau-Zener resonance-crossing problem relevant to coherent photo- and magneto-association of ultracold atoms. Due to the structure of the corresponding classical phase space, the adiabatic…

Quantum Gases · Physics 2010-03-16 R. Sokhoyan , D. Melikdzhanian , C. Leroy , H. -R. Jauslin , A. Ishkhanyan

The diagonal Born-Oppenheimer correction (DBOC) stems from the diagonal second derivative coupling term in the adiabatic representation, and it can have an arbitrary large magnitude when a gap between neighbouring Born-Oppenheimer (BO)…

Chemical Physics · Physics 2016-05-02 Rami Gherib , Liyuan Ye , Ilya G. Ryabinkin , Artur F. Izmaylov

An asymptotic approach for a Schroedinger type equation with non selfadjoint Hamiltonian of a special type in the case of two close degeneracy (turning) points is developed. Both real and complex degeneracy points are treated by a method of…

Mathematical Physics · Physics 2021-07-20 Ignat Fialkovsky , Maria Perel

We investigate two well-known approaches for extending the fewest switches surface hopping (FSSH) algorithm to periodic time-dependent couplings. The first formalism acts as if the instantaneous adiabatic electronic states were standard…

Chemical Physics · Physics 2019-10-07 Zeyu Zhou , Hsing-Ta Chen , Abraham Nitzan , Joseph Eli Subotnik

We investigate the quantum effects, in particular the Landau-level quantization, in the scattering of a particle the nonadiabatic classical dynamics of which is governed by an adiabatic invariant. As a relevant example, we study the…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 F. Dahlem , F. Evers , A. D. Mirlin , D. G. Polyakov , P. Woelfle

Two problems incorporating a set of horizontal linear potentials crossed by a sloped linear potential are analytically solved and compared with numerical results: (a) the case where boundary conditions are specified at the ends of a finite…

Atomic Physics · Physics 2009-10-31 V. A. Yurovsky , A. Ben-Reuven , P. S. Julienne , Y. B. Band

We discuss a one-dimensional version of the Landau-Pekar equations, which are a system of coupled differential equations with two different time scales. We derive an approximation on the slow time scale in the spirit of a non-linear…

Mathematical Physics · Physics 2019-06-20 Rupert L. Frank , Zhou Gang

In [Phys. Rev. Lett. 95, 080502 (2005)], Zheng proposed a scheme for implementing a conditional phase shift via adiabatic passages. The author claims that the gate is "neither of dynamical nor geometric origin" on the grounds that the…

Quantum Physics · Physics 2009-10-30 Ognyan Oreshkov , John Calsamiglia

We study a one dimensional nonequilibrium lattice model with competing features of particle attraction and non-local hops. The system is similar to a zero range process (ZRP) with attractive particles but the particles can make both local…

Statistical Mechanics · Physics 2015-05-14 Apoorva Nagar

Nonadiabatic dynamics methods are an essential tool for investigating photochemical processes. In the context of employing first principles electronic structure techniques, such simulations can be carried out in a practical manner using…

Chemical Physics · Physics 2024-05-08 Jonathan R. Mannouch , Aaron Kelly

The viability of adiabatic quantum computation depends on the slow evolution of the Hamiltonian. The adiabatic switching theorem provides an asymptotic series for error estimates in $1/T$, based on the lowest non-zero derivative of the…

Quantum Physics · Physics 2025-12-25 Thomas D. Cohen , Andrew Li , Hyunwoo Oh , Maneesha Sushama Pradeep

We study nuclear propagation through avoided crossings of electron energy levels. We construct a surface hopping semigroup, which gives an Egorov-type description of the dynamics. The underlying time-dependent Schroedinger equation has a…

Mathematical Physics · Physics 2017-06-07 Clotilde Fermanian Kammerer , Caroline Lasser

Akin to the traditional quasi-classical trajectory method for investigating the dynamics on a single adiabatic potential energy surface for an elementary chemical reaction, we carry out the dynamics on a 2-state ab initio potential energy…

Since the pioneering works by Landau, Zener, St\"uckelberg, and Majorana (LZSM), it has been known that driving a quantum two-level system results in tunneling between its states. Even though the interference between these transitions is…

Quantum Physics · Physics 2022-11-16 Oleh V. Ivakhnenko , Sergey N. Shevchenko , Franco Nori

We control the current of a single particle quantum ratchet by designing ramping schemes for experimentally accessible control parameters. We harvest on Landau-Zener transitions between Floquet states. Adiabatic and diabatic ramping allow…

Other Condensed Matter · Physics 2009-11-13 L. Morales-Molina , S. Flach , J. B. Gong