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A mixture of solvent particles with short-range, directional interactions and solute particles with short-range, isotropic interactions that can bond multiple times is of fundamental interest in understanding liquids and colloidal mixtures.…

Soft Condensed Matter · Physics 2016-09-21 Artee Bansal , D. Asthagiri , Kenneth R. Cox , Walter G. Chapman

We investigate the thermodynamics and percolation regimes of model binary mixtures of patchy colloidal particles. The particles of each species have three sites of two types, one of which promotes bonding of particles of the same species…

Soft Condensed Matter · Physics 2015-03-19 Daniel de las Heras , José Maria Tavares , Margarida M. Telo da Gama

The recently developed Perturbed-Chain Statistical Associating Fluid Theory (PC-SAFT) is investigated for a wide range of model parameters including the parameter m representing the chain length and the thermodynamic temperature T and…

Soft Condensed Matter · Physics 2009-11-11 L. Yelash , M. Mueller , W. Paul , K. Binder

We use a microscopic density functional theory based on Wertheim's first order thermodynamic perturbation theory to study wetting behavior of athermal mixtures of colloids and excluded-volume polymers. In opposition to the wetting behavior…

Soft Condensed Matter · Physics 2007-05-23 Pawel Bryk

In the present work, with the intent of exploring the out-of-equilibrium polymerization of active patchy particles in linear chains, we study a suspension of active bivalent Brownian particles (ABBPs). At all studied temperatures and…

Soft Condensed Matter · Physics 2024-11-19 Caterina Landi , John Russo , Francesco Sciortino , Chantal Valeriani

We investigate the thermal and structural properties of knotted diblock copolymer rings using a coarse-grained lattice model in an implicit solvent. The system is studied by means of the Wang--Landau Monte Carlo algorithm, allowing us to…

Soft Condensed Matter · Physics 2026-05-18 Neda Abbasi Taklimi , Franco Ferrari , Marcin R. Piątek , Luca Tubiana

Within the framework of the mode-coupling theory of super-cooled liquids, we investigate new phenomena in colloidal systems on approach to their glass transitions. When the inter-particle potential contains an attractive part, besides the…

Soft Condensed Matter · Physics 2009-11-07 K. A. Dawson , G. Foffi , F. Sciortino , P. Tartaglia , E. Zaccarelli

Colloidal aggregation could be implemented in various fields ranging from purely colloidal thermodynamics to protein interactions, their stability, and maybe folding. Indeed, colloidal aggregation is closely linked to the so-called…

Soft Condensed Matter · Physics 2013-01-03 Pierre de Thier

Thermodynamic perturbation theory for central-force (TPT-CF) type of associating potential is used to study the phase behavior of symmetric binary mixture of associating particles with spherically symmetric interaction. The model is…

Soft Condensed Matter · Physics 2013-12-18 Yu. V. Kalyuzhnyi , T. V. Hvozd

Two ring polymers close to each other in space may be either in a segregated phase if there is a strong repulsion between monomers in the polymers, or intermingle in a mixed phase if there is a strong attractive force between the monomers.…

Soft Condensed Matter · Physics 2022-11-23 EJ Janse van Rensburg , E Orlandini , MC Tesi , SG Whittington

In this paper we develop a thermodynamic perturbation theory for two site associating fluids which exhibit bond cooperativity. We include both steric hindrance and ring formation such that the equation of state is bond angle dependent. Here…

Soft Condensed Matter · Physics 2015-06-19 B. D. Marshall , Amin Haghmoradi , W. G. Chapman

Entropy alone can self-assemble hard particles into colloidal crystals of remarkable complexity whose structures are the same as atomic and molecular crystals, but with larger lattice spacings. Although particle-based molecular simulation…

Soft Condensed Matter · Physics 2021-07-06 Thi Vo , Sharon C. Glotzer

Dense or glassy active matter, as a result of its remarkable resemblance to passive glass-forming materials, is enjoying increasing scientific interest. To better grasp the subtle effect of active motion on the process of vitrification, a…

Soft Condensed Matter · Physics 2023-10-20 Vincent E. Debets , Liesbeth M. C. Janssen

We study a generic model of self-assembling chains which can branch and form networks with branching points (junctions) of arbitrary functionality. The physical realizations include physical gels, wormlike micells, dipolar fluids and…

Soft Condensed Matter · Physics 2009-11-07 A. G. Zilman , S. A. Safran

The thermal properties of coarse grained knotted polymers containing two kinds of monomers $A$ and $B$ fluctuating in a solution are investigated on a simple cubic lattice using the Wang-Landau MC algorithm. These knots have a more complex…

Soft Condensed Matter · Physics 2022-09-07 Neda Abbasi Taklimi , Franco Ferrari , Marcin Radosław Piątek , Luca Tubiana

First steps towards developing a new perturbation theory for molecular liquids are taken. By choosing a new form of splitting the site-site potential functions between molecules, we will get a set of atomic fluids as the reference system…

Chemical Physics · Physics 2017-11-21 Mehrdad Khanpour

It has been extensively demonstrated through first principles quantum mechanics calculations that water exhibits strong hydrogen bond cooperativity. Classical molecular simulation and statistical mechanics methods typically assume pairwise…

Soft Condensed Matter · Physics 2017-05-24 Bennett D. Marshall

The determination of the Landau free energy (the grand thermodynamic potential) by a perturbation theory is advanced to arbitrary order for the specific case of non-interacting fermionic systems perturbed by a one-particle potential.…

Statistical Mechanics · Physics 2018-07-11 Cezary Sliwa , Tomasz Dietl

We investigate the behavior of a patchy particle model close to a hard-wall via Monte Carlo simulation and density functional theory (DFT). Two DFT approaches, based on the homogeneous and inhomogeneous versions of Wertheim's first order…

We consider two species of self-propelled point particles: A-particles and B-particles. The orientations between nearby particles are subject to pair interactions of different strength for A-A-, A-B-(=B-A-) and B-B-interactions,…

Soft Condensed Matter · Physics 2023-04-13 Rüdiger Kürsten , Jakob Mihatsch , Thomas Ihle