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This work presents a rigorous statistical mechanical theory of solvation free energies, specifically useful for describing the long-range nature of ions in an electrolyte solution. The theory avoids common issues with field theories by…

Statistical Mechanics · Physics 2017-12-29 David M. Rogers

In plasma physics, collisionless charged particles are transported following the dynamics of a meanfield Vlasov equation with a self-consistent electric field generated by the charge density. Due to the long range interaction between…

Analysis of PDEs · Mathematics 2024-10-22 Toan T. Nguyen

We study charge regulation of colloidal particles inside aqueous electrolyte solutions. To stabilize colloidal suspension against precipitation, colloidal particles are synthesized with either acidic or basic groups on their surface. In…

Soft Condensed Matter · Physics 2020-09-16 Amin Bakhshandeh , Derek Frydel , Yan Levin

We extend our previous study of surface tension of ionic solutions and apply it to the case of acids (and salts) with strong ion-surface interactions. These ion-surface interactions yield a non-linear boundary condition with an effective…

Soft Condensed Matter · Physics 2017-02-17 Tomer Markovich , David Andelman , Rudi Podgornik

We implement a well-established concept to consider dispersion effects within a Poisson-Boltzmann approach of continuum solvation of proteins. The theoretical framework is particularly suited for boundary element methods. Free parameters…

Biological Physics · Physics 2007-11-28 Parimal Kar , Max Seel , Ulrich H. E. Hansmann , Siegfried Hoefinger

We consider a system of $N\gg 1$ interacting fermionic particles in three dimensions, confined in a periodic box of volume $1$, in the mean-field scaling. We assume that the interaction potential is bounded and small enough. We prove upper…

Mathematical Physics · Physics 2019-12-10 Christian Hainzl , Marcello Porta , Felix Rexze

This work contributes to the problem of determining effective interaction between asymmetrically (likely or oppositely) charged objects whose total charge is neutralized by mobile pointlike counter-ions of the same charge, the whole system…

Statistical Mechanics · Physics 2015-06-22 L. Samaj , E. Trizac

The aim of this paper is two-fold: in probing the statistical mechanical properties of interacting quantum fields, and in providing a field theoretical justification for a stochastic source term in the Boltzmann equation. We start with the…

High Energy Physics - Phenomenology · Physics 2008-11-26 Esteban Calzetta , Bei Lok Hu

The linear Boltzmann equation for elastic and/or inelastic scattering is applied to derive the distribution function of a spatially homogeneous system of charged particles spreading in a host medium of two-level atoms and subjected to…

Statistical Mechanics · Physics 2009-11-13 A. Rossani , A. M. Scarfone

Electrostatic interactions make a large contribution to solvation free energy in ionic fluids such as electrolytes and colloidal dispersions. The electrostatic contribution to solvation free energy has been ascribed to the self-energy of a…

Statistical Mechanics · Physics 2020-02-19 Hiroshi Frusawa

Effects of charge-density fluctuations on a phase behavior of the restricted primitive model (RPM) are studied within a field-theoretic formalism. We focus on a $\lambda$-line of continuous transitions between charge-ordered and…

Statistical Mechanics · Physics 2009-11-11 A. Ciach , O. Patsahan

We investigate the dynamics of thermal Casimir interactions between plates described within a living conductor model, with embedded mobile anions and cations, whose density field obeys a stochastic partial differential equation which can be…

Statistical Mechanics · Physics 2015-06-18 David S. Dean , Rudolf Podgornik

We derive an equation capable of treating both the electrostatic and non-electrostatic interactions in the charged liquids. The equation derived is a complex version of the Poisson-Boltzmann equation, in which the non-electrostatic…

Soft Condensed Matter · Physics 2025-02-12 Li Wan

We apply general variational techniques to the problem of the counterion distribution around highly charged objects where strong condensation of counterions takes place. Within a field-theoretic formulation using a fluctuating electrostatic…

Soft Condensed Matter · Physics 2009-11-07 Roland R. Netz , Henri Orland

We study two-particle systems in a model quantum field theory, in which scalar particles and spinor particles interact via a mediating scalar field. The Lagrangian of the model is reformulated by using covariant Green's functions to solve…

Nuclear Theory · Physics 2016-09-08 Volodymyr Shpytko , Jurij Darewych

The Poisson-Boltzmann (PB) theory is widely used to depict ionic systems. As a mean-field theory, the PB theory neglects the correlation effect in the ionic atmosphere and leads to deviations from experimental results as the concentration…

Soft Condensed Matter · Physics 2019-06-25 Mao Su , Zhijie Xu , Yanting Wang

Exploiting the results of the exact solution for the ground state of the one-dimensional spinless quantum gas of Fermions and impenetrable Bosons with the mu/x_{ij}^2 particle-particle interaction, the Hellmann-Feynman theorem yields…

Strongly Correlated Electrons · Physics 2009-10-31 Rudolf A. Roemer , Paul Ziesche

Electrostatic correlations and fluctuations in ionic systems can be described within an extended Poisson-Boltzmann theory using a Gaussian variational form. The resulting equations are challenging to solve because they require the solution…

Computational Physics · Physics 2015-06-17 Zhenli Xu , A. C. Maggs

We consider an overall neutral system consisting of two similarly charged plates and their oppositely charged counterions and analyze the electrostatic interaction between the two surfaces beyond the mean-field Poisson-Boltzmann…

Soft Condensed Matter · Physics 2016-08-31 A. W. C. Lau , P. Pincus

To explore charge regulation (CR) in physicochemical and biophysical systems, we present a model of colloidal particles with sticky adsorption sites which account for the formation of covalent bonds between the hydronium ions and the…

Soft Condensed Matter · Physics 2019-12-12 Amin Bakhshandeh , Derek Frydel , Alexandre Diehl , Yan Levin