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Based on temperature dependent far infrared transmission spectra of YMn2O5 and TbMn2O5 single crystals, we report the observation of electric dipole-active magnetic excitations, or electromagnons, in these multiferroics. Electromagnons are…

Strongly Correlated Electrons · Physics 2013-05-29 A. B. Sushkov , R. Valdes Aguilar , S. Park , S-W. Cheong , H. D. Drew

We present a large magnetodielectric (MD) effect of 65 % at 100 kHz with 5 T field in B-site ordered La2CoMnO6 (LCMO) polycrystalline sample. Frequency and temperature dependent impedance and dielectric studies under magnetic field divulge…

Materials Science · Physics 2014-11-11 J. Krishna Murthya , K. Devi Chandrasekhar S. Murugavel , A. Venimadhav

The electric polarization and its magnetic origins in multiferroic RMn2O5, where R is rare-earth ion, are still issues under debate. In this work, the temperature-dependent electric polarization of DyMn2O5, the most attractive member of…

Materials Science · Physics 2014-02-06 Z. Y. Zhao , M. F. Liu , X. Li , L. Lin , Z. B. Yan , S. Dong , J. -M. Liu

Cross-correlation between magnetic and dielectric properties has been attracting renewed interest because of the fundamental as well as technological importance of controlling the electric (magnetic) polarization by an external magnetic…

Strongly Correlated Electrons · Physics 2007-05-23 D. Higashiyama , N. Kida , S. Miyasaka , T. Arima , Y. Tokura

The magnetoelectric coupling, i.e., cross-correlation between electric and magnetic orders, is a very desirable property to combine functionalities of materials for next-generation switchable devices. Multiferroics with spin-driven…

Strongly Correlated Electrons · Physics 2019-01-07 Ian Aupiais , Masahito Mochizuki , Hideaki Sakata , Romain Grasset , Yann Gallais , Alain Sacuto , Maximilien Cazayous

We present a unique example of giant magnetoelectric effect in a conventional multiferroic HoMnO3, where polarization is very large (~56 mC/m2) and the ferroelectric transition temperature is higher than the magnetic ordering temperature by…

Strongly Correlated Electrons · Physics 2015-05-13 N. Hur , I. K. Jeong , M. F. Hundley , S. B. Kim , S. -W. Cheong

We report the dielectric dispersion of the giant magnetocapacitance (GMC) in multiferroic DyMnO$_{3}$ over a wide frequency range. The GMC is found to be attributable not to the softened electromagnon but to the electric-field-driven motion…

Strongly Correlated Electrons · Physics 2009-11-13 F. Kagawa , M. Mochizuki , Y. Onose , H. Murakawa , Y. Kaneko , N. Furukawa , Y. Tokura

Using first principles calculations, we study the microscopic origin of ferroelectricity (FE) induced by magnetic order in the orthorhombic HoMnO3. We obtain the largest ferroelectric polarization observed in the whole class of improper…

Materials Science · Physics 2009-11-13 Silvia Picozzi , Kunihiko Yamauchi , Biplab Sanyal , Ivan A. Sergienko , Elbio Dagotto

Magnetic order and excitations in multiferroic DyMnO3 were studied by neutron scattering experiments using a single crystal prepared with enriched 162Dy isotope. The ordering of Mn moments exhibits pronounced hysteresis arising from the…

Strongly Correlated Electrons · Physics 2015-06-23 T. Finger , K. Binder , Y. Sidis , A. Maljuk , D. N. Argyriou , M. Braden

Magnetodielectric materials are characterized by a strong coupling of magnetic and dielectric properties and in rare cases simultaneously exhibit both, magnetic and polar order. Among other multiferroics, TbMnO3 and GdMnO3 reveal a strong…

Strongly Correlated Electrons · Physics 2015-06-25 A. Pimenov , A. A. Mukhin , V. Yu. Ivanov , V. D. Travkin , A. M. Balbashov , A. Loidl

The magnetoelastic coupling in multiferroic $DyMn_2O_5$ is investigated by magnetostriction measurements along the three crystallographic orientations. Strong lattice anomalies as a function of the magnetic field are detected at the low…

Strongly Correlated Electrons · Physics 2007-05-23 C. R. dela Cruz , B. Lorenz , Y. Y. Sun , C. W. Chu , S. Park , S. -W. Cheong

Low energy excitations in the multiferroic material TbMnO3 have been investigated by Raman spectroscopy. Our observations reveal the existence of two peaks at 30 cm-1 and 60 cm-1. They are observed in the cycloidal phase below the Curie…

Strongly Correlated Electrons · Physics 2010-10-12 P. Rovillain , M. Cazayous , Y. Gallais , A. Sacuto , M-A. Measson , H. Sakata

Temperature (5--250 K) and magnetic field (0--70 kOe) variations of the low-energy (1--10 meV) electrodynamics of spin excitations have been investigated for a complete set of light-polarization configurations for a ferroelectric magnet…

Materials Science · Physics 2009-11-13 N. Kida , Y. Ikebe , Y. Takahashi , J. P. He , Y. Kaneko , Y. Yamasaki , R. Shimano , T. Arima , N. Nagaosa , Y. Tokura

Electromagnon is the spin wave in multiferroic materials and is known to accompany electric polarization due to the cross correlation between the charge and spin. Here, we theoretically show that the electromagnons also induce dc current…

Strongly Correlated Electrons · Physics 2019-12-30 Takahiro Morimoto , Naoto Nagaosa

The honeycomb antiferromagnet Co4Nb2O9 is known to exhibit an interesting magnetoelectric effect that the electric polarization rotates at the twice speed in the opposite direction relative to the rotation of the external magnetic field…

Strongly Correlated Electrons · Physics 2020-04-22 Masashige Matsumoto , Mikito Koga

The coupling between magnetic order and ferroelectricity has been under intense investigation in a wide range of transition-metal oxides. The strongest coupling is obtained in so-called magnetically-induced multiferroics where…

Materials Science · Physics 2015-05-13 V. S. Zapf , M. Kenzelmann , F. Wolff-Fabris , F. Balakirev , Y. Chen

We have investigated the magnetic and dielectric properties of Ca$_2$CoSi$_2$O$_7$ crystal. The dielectricity and magnetism of Ca$_2$CoSi$_2$O$_7$ are strongly coupled below a canted antiferromagnetic transition temperature ($T_{\rm N}$):…

Strongly Correlated Electrons · Physics 2009-05-29 M. Akaki , J. Tozawa , D. Akahoshi , H. Kuwahara

In this article the mechanism of the linear magnetoelectric (ME) effect in the rhombohedral multiferroic BiFeO$_3$ is considered. The study is based on the symmetry approach of the GinzburgLandau type, in which polarization,…

Materials Science · Physics 2016-04-06 A. F. Popkov , M. D. Davydova , K. A. Zvezdin , S. V. Solov'yov , A. K. Zvezdin

A recent experiment on the multiferroic BiMn$_2$O$_5$ compound under a strong applied magnetic field revealed a rich phase diagram driven by the coupling of magnetic and charge (dipolar) degrees of freedom. Based on the exchange-striction…

Materials Science · Physics 2009-04-01 Gun Sang Jeon , Jin-Hong Park , Kee Hoon Kim , Jung Hoon Han

The magnetic and dielectric properties under high magnetic fields are studied in the single crystal of Cu3Mo2O9. This multiferroic compound has distorted tetrahedral spin chains. The effects of the quasi-one dimensionality and the…

Strongly Correlated Electrons · Physics 2013-11-13 H. Kuroe , K. Aoki , R. Kino , T. Sato , H. Kuwahara , T. Sekine , T Kihara , M. Akaki , Y. Kohama , M. Tokunaga , A. Matsuo , K. Kindo , M. Hase , K. Takehana , H. Kitazawa , K. Oka , T. Ito , H. Eisaki
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