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The time-dependent Schr\"{o}dinger equation for the hydrogen atom and its interaction with coherent intense high-frequency short laser pulses is solved numerically exactly by propagating the single-electron wave packets. Thereby, the…

Atomic Physics · Physics 2013-09-11 Philipp V. Demekhin , David Hochstuhl , Lorenz S. Cederbaum

We report optical absorption imaging of ultracold neutral plasmas.Images are used to measure the ion absorption spectrum, which is Doppler-broadened. Through the spectral width, we monitor ion equilibration in the first 250ns after plasma…

Atomic Physics · Physics 2009-11-10 C. E. Simien , Y. C. Chen , P. Gupta , S. Laha , Y. N. Martinez , P. G. Mickelson , S. B. Nagel , T. C. Killian

Laser-triggered ionization injection is a promising way of generating controllable high-quality electrons in plasma-based acceleration. We show that ionization injection of electrons into a fully nonlinear plasma wave wake using a laser…

Plasma Physics · Physics 2022-02-02 Xinlu Xu , Jorge Vieira , Mark Hogan , Chan Joshi , Warren Mori

We show that the complete photoemission dynamics in situations of electron-ion entanglement can be retrieved from photoelectron spectral measurements without information on the ion. To this end, we develop an energy-time analysis of the…

We present measurements of the pulse length of ultracold electron bunches generated by near-threshold two-photon photoionization of a laser-cooled gas. The pulse length has been measured using a resonant $3$ GHz deflecting cavity in…

Atomic Physics · Physics 2017-03-24 J. G. H. Franssen , T. L. I. Frankort , E. J. D. Vredenbregt , O. J. Luiten

The balance of the linear photon momentum in multiphoton ionization is studied experimentally. In the experiment argon and neon atoms are singly ionized by circularly polarized laser pulses with a wavelength of 800 nm and 1400 nm in the…

Optics · Physics 2011-06-01 C Smeenk , L Arissian , B Zhou , A Mysyrowicz , D M Villeneuve , A Staudte , P B Corkum

We theoretically study the photoelectron angular distributions (PADs) from two-color two-photon near-threshold ionization of hydrogen and noble gas (He, Ne, and Ar) atoms by a combined action of femtosecond extreme ultraviolet (EUV) and…

Atomic Physics · Physics 2015-06-22 Kenichi L. Ishikawa , A. K. Kazansky , N. M. Kabachnik , Kiyoshi Ueda

Ionization by relativistically intense laser pulses of finite duration is considered in the framework of strong-field quantum electrodynamics. Our main focus is on the formation of ionization supercontinua. More specifically, when studying…

Atomic Physics · Physics 2016-07-13 K. Krajewska , J. Z. Kamiński

We explore the laser-induced ionization dynamics of N2 and CO2 molecules subjected to a few-cycle, linearly polarized, 800\,nm laser pulse using effective two-dimensional single active electron time-dependent quantum simulations. We show…

Atomic Physics · Physics 2012-10-02 Michel Peters , Tung Nguyen-Dang , Eric Charron , Arne Keller , Osman Atabek

We explore photo-electron spectra (PES) and photo-electron angular distributions (PAD) of C$_{60}$ with time-dependent density functional theory (TDDFT) in real time. To simulate experiments in gas phase, we consider isotropic ensembles of…

Atomic and Molecular Clusters · Physics 2014-12-12 C. -Z. Gao , P. Wopperer , P. M. Dinh , E. Suraud , P. -G. Reinhard

Methods for experimental reconstruction of molecular frame (MF) photoionization dynamics, and related properties - specifically MF photoelectron angular distributions (PADs) and continuum density matrices - are outlined and discussed.…

Chemical Physics · Physics 2024-06-06 Paul Hockett , Varun Makhija

We present a combined experimental and theoretical study on the photodissociation dynamics of ion-pair formation in O$_2$ following resonant two-photon absorption of a 9.3 eV femtosecond pulse, where the resulting O$^+$ ions are detected…

Chemical Physics · Physics 2020-08-28 Kirk A. Larsen , Robert R. Lucchese , Daniel S. Slaughter , Thorsten Weber

Laser induced plasmas have found numerous applications including plasma-assisted combustion, combustion diagnostics, laser induced breakdown spectroscopy, light detection and ranging techniques (LIDAR), microwave guiding, reconfigurable…

Plasma Physics · Physics 2017-10-11 A. Sharma , M. N. Slipchenko , M. N. Shneider , X. Wang , K. A. Rahman , A. Shashurin

Photoelectron spectroscopy is a powerful method that provides insight into the quantum mechanical properties of a wide range of systems. The ionized electron wavefunction carries information on the structure of the bound orbital, the ionic…

Strong-field ionization of polar molecules contains rich dynamical processes such as tunneling, excitation, and Stark shift. These processes occur on a sub-cycle time scale and are difficult to distinguish in ultrafast measurements. Here,…

Atomic Physics · Physics 2021-12-15 Jia-Yin Che , Chao Chen , Shang Wang , Guo-Guo Xin , Yan-Jun Chen

3D photoelectron angular distributions (PADs) are measured from an atomic target ionized by ultrafast, elliptical fields of opposite handedness. Comparing these PADs to one another and to numeric simulations, a difficult to avoid systematic…

Coherent light has revolutionized scientific research, spanning biology, chemistry, and physics. To delve into ultrafast phenomena, the development of high-energy, high-tunable light sources is instrumental. Here, the photo-electric effect…

Atomic Physics · Physics 2023-11-29 Camilo Granados , Enrique G. Neyra , Lorena Rebón , Marcelo F. Ciappina

Atoms ionization by the simultaneous absorption of multiple photons has found applications in fiber optics, where it leads to unique nonlinear phenomena. To date, studies of the ionization regime have been limited to gas-filled hollow-core…

Coherence among rotational ion channels during photoionization is exploited to control the anisotropy of the resulting photoelectron angular distributions at specific photoelectron energies. The strategy refers to a robust and single…

Chemical Physics · Physics 2019-09-11 R. Chamakhi , M. Telmini , O. Atabek , E. Charron

Recent experimental work on the photorecombination and the photoionization of astrophysically relevant atomic ions employing the merged-beams technique at heavy-ion storage-rings and synchrotron-light sources, respectively, is summarized.…

Astrophysics · Physics 2011-01-06 Stefan Schippers