Related papers: Symmetry selective third harmonic generation from …
We propose and experimentally demonstrate a scheme allowing to reach noncollinear phase-matching of high harmonic generation in solids, which may potentially lead to an enhancement of the generation efficiency. The principle is based on…
Classical nonlocality in conducting nanostructures has been shown to dramatically alter the linear optical response, by placing a fundamental limit on the maximum field enhancement that can be achieved. This limit directly extends to all…
We prescribe a novel approach for continuously tailoring the local phase of the nonlinear polarizability which can lead to an arbitrary phase profile for harmonic generations. The introduced phase of the nonlinear polarizability is…
By numerically integrating the three-dimensional Maxwell equations in the time domain with reference to a dispersive quadratically nonlinear material, we study second harmonic generation in planar photonic crystal microresonators. The…
We present a study of the second-order nonlinear optical properties of metal-based metamaterials. A hydrodynamic model for electronic response is used, in which nonlinear surface contributions are expressed in terms of the bulk…
Plasmonic metasurfaces have emerged as a promising platform for enhancing a range of nonlinear optical processes, offering compact geometry and flexibility in light manipulation. Second order nonlinear processes, like second harmonic…
A nonlinear electromagnetic scattering problem is studied in the presence of bound states in the radiation continuum. It is shown that the solution is not analytic in the nonlinear susceptibility and the conventional perturbation theory…
Optical phase-matching involves establishing a proper phase relationship between the fundamental and generated waves to enable efficient optical parametric processes. It is typically achieved through either birefringence or periodically…
To understand the photophysics of molecular aggregates, exciton model of J- and H-aggregate has been extensively utilized. However, it lacks consideration of crystal symmetry. Although discrete molecules may lack symmetry, their aggregates…
High-harmonic generation (HHG) in solids has rapidly emerged as a promising platform for creating compact attosecond sources and probing ultrafast electron dynamics. Resonant metasurfaces are essential for enhancement of the otherwise small…
Two conditions on symmetries are identified as necessary for a linear scattering system to be able to rotate the linear polarisation of light: Lack of at least one mirror plane of symmetry and electromagnetic duality symmetry. Duality…
The effective nonlinear response of films of random composites consisting of a binary composite with nonlinear particles randomly embedded in a linear host is theoretically and numerically studied. A theoretical expression for the effective…
We put forward a technique to unveil to which symmetry group a nonlinear crystal belongs, making use of nonlinear optics with structured light. We consider as example the process of spontaneous parametric down-conversion. The crystal, which…
Strong light-matter coupling within electromagnetic environments provides a promising path to modify and control chemical and physical processes. The origin of the enhancement of nonlinear optical processes such as second-harmonic and…
High quality factor optical nanostructures provide great opportunity to enhance nonlinear optical processes such as third harmonic generation. However, the field enhancement in these high quality factor structures is typically accompanied…
We show that nonlinear multipolar interference allows achieving not only unidirectional, but also non-reciprocal nonlinear generation from a nanoelement, with the direction of the nonlinearly produced light decoupled from that of at least…
The use of bichromatic counter-rotating laser field is known to generate high-order harmonics with non-zero ellipticity. By combining such laser field with a plasmonic-enhanced spatially inhomogeneous field, we propose a way to influence…
We examined the chirality dependent optical selection rules in two-dimensional monolayer materials with the honeycomb lattice, and based on symmetry argument, we generalized these rules to multi-photon transitions of arbitrary orders. We…
We aim to clarify the role that absorption plays in nonlinear optical processes in a variety of metallic nanostructures and show how it relates to emission and conversion efficiency. We define a figure of merit that establishes the…
We use ultrafast laser pulses to experimentally demonstrate that the second-order optical response of bulk single crystals of the topological insulator Bi$_2$Se$_3$ is sensitive to its surface electrons. By performing surface doping…