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Wetting of a charged substrate by an electrolyte solution is investigated by means of classical density functional theory applied to a lattice model. Within the present model the pure, i.e., salt-free solvent, for which all interactions are…

Soft Condensed Matter · Physics 2013-06-06 Ingrid Ibagon , Markus Bier , S. Dietrich

The wetting of a charged wedge-like wall by an electrolyte solution is investigated by means of classical density functional theory. As in other studies on wedge wetting, this geometry is considered as the most simple deviation from a…

Soft Condensed Matter · Physics 2018-05-25 Maximilian Mußotter , Markus Bier

We use microscopic density functional theory to study filling transitions in systems with long-ranged wall-fluid and short-ranged fluid-fluid forces occurring in a right-angle wedge. By changing the strength of the wall-fluid interaction we…

Statistical Mechanics · Physics 2016-05-04 Alexandr Malijevský , Andrew O. Parry

We present numerical studies of first-order and continuous filling transitions, in wedges of arbitrary opening angle $\psi$, using a microscopic fundamental measure density functional model with short-ranged fluid-fluid forces and…

Statistical Mechanics · Physics 2015-06-11 Alexandr Malijevský , Andrew O. Parry

In this communication we demonstrate the existence of a first-order prewetting transition of a supracritical model polymer solution adjacent to an attractive surface. The model fluid we use mimics (qualitatively) an aqueous polyethylene…

Soft Condensed Matter · Physics 2024-10-28 Jan Forsman , Clifford E. Woodward

Wetting transitions have been predicted and observed to occur for various combinations of fluids and surfaces. This paper describes the origin of such transitions, for liquid films on solid surfaces, in terms of the gas-surface interaction…

Materials Science · Physics 2015-05-13 Silvina M. Gatica , Milton W. Cole

Four on-lattice and six off-lattice models for active matter are studied numerically, showing that in contact with a wall, they display universal wetting transitions between three distinctive phases. The particles, which interact via…

Statistical Mechanics · Physics 2018-12-05 Néstor Sepúlveda , Rodrigo Soto

A lattice model for active matter is studied numerically, showing that it displays wettings transitions between three distinctive phases when in contact with an impenetrable wall. The particles in the model move persistently, tumbling with…

Soft Condensed Matter · Physics 2017-09-13 Néstor Sepúlveda , Rodrigo Soto

We look at the wetting of a pure fluid in contact with a charged flat surface. In the bulk, the fluid is a classical van der Waals fluid containing dissociated ions. The presence of wall and ions leads to strong dielectrophoretic and…

Statistical Mechanics · Physics 2021-11-16 Yoav Tsori

Using density functional theory we calculate the density profiles of a binary solvent adsorbed around a pair of big solute particles. All species interact via repulsive Gaussian potentials. The solvent exhibits fluid-fluid phase separation…

Soft Condensed Matter · Physics 2007-05-23 A. J. Archer , R. Evans , R. Roth , M. Oettel

The influence of a chemically or electrically heterogeneous distribution of interaction sites at a planar substrate on the number density of an adjacent fluid is studied by means of classical density functional theory (DFT). In the case of…

Soft Condensed Matter · Physics 2018-05-25 Maximilian Mußotter , Markus Bier , S. Dietrich

We calculate the ion and composition distributions around colloid particles in an aqueous mixture, accounting for preferential adsorption, electrostatic interaction, selective solvation among ions and polar molecules, and…

Soft Condensed Matter · Physics 2011-11-04 Ryuichi Okamoto , Akira Onuki

Alkanes of medium chain length show an unusual wetting behavior on (salt) water, exhibiting a sequence of two changes in the wetting state. When deposited on the water surface at low temperatures, the liquid alkane forms discrete droplets…

Statistical Mechanics · Physics 2007-05-23 Volker C. Weiss , Joseph O. Indekeu

In recent experiments, a sequence of changes in the wetting state (`wetting transitions') has been observed upon increasing the temperature in systems consisting of pentane on pure water and of hexane on brine. This sequence of two…

Statistical Mechanics · Physics 2009-11-10 Volker C. Weiss , Joseph O. Indekeu

We report a theoretical and simulation study of the drying and wetting phase transitions of a truncated Lennard-Jones fluid at a flat structureless wall. Binding potential calculations predict that the nature of these transitions depends on…

Statistical Mechanics · Physics 2017-09-13 Robert Evans , Maria C. Stewart , Nigel B. Wilding

Understanding the wetting properties of premelting films requires knowledge of the film's equation of state, which is not usually available. Here we calculate the disjoining pressure curve of premelting films, and perform a detailed…

Soft Condensed Matter · Physics 2020-09-09 Pablo Llombart , Eva G. Noya , David N. Sibley , Andrew J. Archer , Luis G. MacDowell

We present numerical studies of complete, first-order and critical wedge filling transitions, at a right angle corner, using a microscopic fundamental measure density functional theory. We consider systems with short-ranged, cut-off…

Statistical Mechanics · Physics 2015-06-16 Alexandr Malijevsky , Andrew O Parry

We calculate various thermodynamic quantities of vortex liquids in a layered superconductor by using the nonperturbative parquet approximation method, which was previously used to study the effect of thermal fluctuations in two-dimensional…

Superconductivity · Physics 2009-10-31 Joonhyun Yeo , M. A. Moore

Recent analyses of wetting in the semi-infinite two dimensional Ising model, extended to include both a surface coupling enhancement and a surface field, have shown that the wetting transition may be effectively first-order and that…

Statistical Mechanics · Physics 2016-07-20 Andrew O. Parry , Alexandr Malijevský

Using fundamental-measure density functional theory we investigate entropic wetting in an asymmetric binary mixture of hard spheres with positive non-additivity. We consider a general planar hard wall, where preferential adsorption is…

Soft Condensed Matter · Physics 2015-05-28 Paul Hopkins , Matthias Schmidt
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