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Related papers: A new spin-anisotropic harmonic honeycomb iridate

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Iridate oxides on a honeycomb lattice are considered promising candidates for realization of quantum spin liquid states. We investigate the magnetic couplings in a structural model for a honeycomb iridate K$_2$IrO$_3$, with $C_3$ point…

Strongly Correlated Electrons · Physics 2019-10-23 Ravi Yadav , Satoshi Nishimoto , Manuel Richter , Jeroen van den Brink , Rajyavardhan Ray

We have investigated the thermodynamic and local magnetic properties of the Mott insulating system Ag$_{3}$LiRu$_{2}$O$_{6}$ containing Ru$^{4+}$ (4$d$$^{4}$) for novel magnetism. The material crystallizes in a monoclinic $C2/m$ structure…

We study the interplay of strong electron correlations and intra-triangle spin exchange at two-thirds filling of the single-orbital Hubbard model on the decorated honeycomb lattice using rotationally invariant slave bosons. We find that the…

Strongly Correlated Electrons · Physics 2021-08-06 H. L. Nourse , Ross H. McKenzie , B. J. Powell

We study roles of electron correlations on topological insulators on the honeycomb lattice with the spin-orbit interaction. Accurate variational Monte Carlo calculations show that the increasing on-site Coulomb interactions cause a strong…

Strongly Correlated Electrons · Physics 2011-05-24 Youhei Yamaji , Masatoshi Imada

A new honeycomb lattice iridate (La,Na)IrO$_3$ ($\approx$ LaNaIr$_2$O$_6$) is successfully synthesized from the spin-orbit coupled Mott insulator Na$_2$IrO$_3$ by replacing the interlayer Na$^+$ ions with La$^{3+}$ ions. (La,Na)IrO$_3$…

Strongly Correlated Electrons · Physics 2024-06-06 Yuya Haraguchi , Hiroko Aruga Katori

The layered honeycomb magnet $\alpha$-Li$_2$IrO$_3$ has been theoretically proposed as a candidate to display novel magnetic behaviour associated with Kitaev interactions between spin-orbit entangled $j_{\rm eff}=1/2$ magnetic moments on a…

Strongly Correlated Electrons · Physics 2017-02-17 S. C. Williams , R. D. Johnson , F. Freund , Sungkyun Choi , A. Jesche , I. Kimchi , S. Manni , A. Bombardi , P. Manuel , P. Gegenwart , R. Coldea

We report discovery of a new iridate family K$_x$Ir$_y$O$_2$ with depleted triangular lattice planes made up of edge sharing IrO$_6$ octahedra separated by K planes. Such a material interpolates between the triangular and honeycomb lattices…

Strongly Correlated Electrons · Physics 2019-08-23 Kavita Mehlawat , Yogesh Singh

We propose a theoretical model for a gapless spin liquid phase that may have been observed in a recent experiment on $\mathrm{H_3Li Ir_2 O_6}$. Despite the insulating and non-magnetic nature of the material, the specific heat coefficient…

Strongly Correlated Electrons · Physics 2018-03-29 Kevin Slagle , Wonjune Choi , Li Ern Chern , Yong Baek Kim

Through a combination of crystal symmetry analysis and density functional theory calculations we unveil a possible microscopic origin of the unexpected insulating behavior reported in the honeycomb Kitaev material Cu$_2$IrO$_3$. Our study…

Strongly Correlated Electrons · Physics 2024-12-03 Ying Li , Roger D. Johnson , Yogesh Singh , Radu Coldea , Roser Valentí

A bond-directional anisotropic exchange interaction, called the Kitaev interaction, is a promising route to realize quantum spin liquids. The Kitaev interactions were found in Mott insulators with the strong spin-orbit coupling, in the…

Strongly Correlated Electrons · Physics 2020-04-08 Yusuke Sugita , Yasuyuki Kato , Yukitoshi Motome

A burning question in the emerging field of spin-orbit driven insulating iridates, such as Na2IrO3 and Li2IrO3 is whether the observed insulating state should be classified as a Mott-Hubbard insulator derived from a half-filled relativistic…

Strongly Correlated Electrons · Physics 2014-01-31 I. I. Mazin , S. Manni , K. Foyevtsova , Harald O. Jeschke , P. Gegenwart , Roser Valenti

We revisit the theory of magnetic Raman scattering in Mott insulators with strong spin-orbit coupling, with a major focus on Kitaev materials. We show that Kitaev materials with bond-anisotropic interactions are generally expected to show…

Strongly Correlated Electrons · Physics 2021-10-27 Yang Yang , Mengqun Li , Ioannis Rousochatzakis , Natalia B. Perkins

The electronic ground state in many iridate materials is described by a complex wave-function in which spin and orbital angular momenta are entangled due to relativistic spin-orbit coupling (SOC). Such a localized electronic state carries…

The Kitaev spin liquid, a ground state of the bond-dependent Kitaev model in a honeycomb lattice has been a centre of attraction, since a microscopic theory to realize such an interaction in solid-state materials was discovered. A challenge…

Strongly Correlated Electrons · Physics 2022-05-20 Jiefu Cen , Hae-Young Kee

Recently, the effects of spin-orbit coupling (SOC) in correlated materials have become one of the most actively studied subjects in condensed matter physics, as correlations and SOC together can lead to the discovery of new phases. Among…

Strongly Correlated Electrons · Physics 2016-03-17 Jeffrey G. Rau , Eric Kin-Ho Lee , Hae-Young Kee

Effects of spin-orbit interactions in condensed matter are an important and rapidly evolving topic. Strong competition between spin-orbit, on-site Coulomb and crystalline electric field interactions in iridates drives exotic quantum states…

Strongly Correlated Electrons · Physics 2018-02-27 Gang Cao , Pedro Schlottmann

With large spin-orbit coupling, the $t_{2g}^5$ electron configuration in $d$-metal oxides is prone to highly anisotropic exchange interactions and exotic magnetic properties. In $5d^5$ iridates, given the existing variety of crystal…

Strongly Correlated Electrons · Physics 2015-11-30 Vamshi M. Katukuri , Satoshi Nishimoto , Ioannis Rousochatzakis , Hermann Stoll , Jeroen van den Brink , Liviu Hozoi

The magnetic field response of the Mott-insulating honeycomb iridate Na$_{2}$IrO$_{3}$ is investigated using torque magnetometry measurements in magnetic fields up to 60 tesla. A peak-dip structure is observed in the torque response at…

The quest for Kitaev quantum spin liquids has led to great interest in honeycomb quantum magnets with strong spin-orbit coupling. It has been recently proposed that even Mott insulators with $3d$ transition metal ions, having nominally weak…

Strongly Correlated Electrons · Physics 2021-11-25 Shreya Das , Sreekar Voleti , Tanusri Saha-Dasgupta , Arun Paramekanti

The Kitaev interaction in a honeycomb lattice with higher-spin $S$ has been one of the central attractions, as it may offer quantum spin liquids. A microscopic theory showed that when the Hund's coupling at the transition metal generates…

Strongly Correlated Electrons · Physics 2024-01-23 Jiefu Cen , Hae-Young Kee