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Soft X-rays (90-173 eV) from the 3rd generation Canadian Light Source have been used in conjunction with a multi coincidence time and position sensitive detection apparatus to observe the dissociative ionization of OCS. By varying the X-ray…

We devise an ab initio formalism for the quantum dynamics of Auger decay by laser-dressed atoms which are inner-shell ionized by extreme ultraviolet (XUV) light. The optical dressing laser is assumed to be sufficiently weak such that…

Atomic Physics · Physics 2009-11-06 Christian Buth , Kenneth J. Schafer

We predict that attosecond spectroscopy could be used to observe time delay for electron emission {in the C$^{1+}$ ion} from a few step processes {that include electron impact excitation}. The results reveal that the photon energy…

Atomic Physics · Physics 2018-10-01 Valdas Jonauskas , Šarūnas Masys

We discuss the possibility of non-exponential tunneling ionization of atoms irradiated by intense laser field. This effect can occur at times, which are greater than the lifetime of a system under consideration. The mechanism for…

Atomic Physics · Physics 2015-03-02 A. M. Ishkhanyan , V. P. Krainov

We investigate neutralization processes (especially thermal surface neutralization), which are required for the magneto-optical trapping of radioactive atoms. A variety of neutralization methods are first summarized: neutral beam injection…

Instrumentation and Detectors · Physics 2019-08-29 H. Kawamura , T. Aoki , K. Harada , T. Inoue , S. Ito , K. Kato , L. Koehler , K. Sakamoto , A. Uchiyama , Y. Sakemi

Photodetachment of the outer-most electrons in few- and many-electron atomic systems is studied in the non-relativistic dipole approximation. Such a photodetachment is analyzed for the neutral atoms and positively charged atomic ions. We…

Atomic Physics · Physics 2021-11-04 Alexei M. Frolov

Molecules show a much increased multiple ionization rate in a strong laser field as compared to atoms of similar ionization energy. A widely accepted model attributes this to the action of the joint fields of the adjacent ionic core and the…

Atomic Physics · Physics 2013-05-16 J. Wu , M. Meckel , L. Ph. H. Schmidt , M. Kunitski , S. Voss , H. Sann , H. Kim , T. Jahnke , A. Czasch , R. Dörner

Based on a semi-empirical generalized Anderson-Newns model we construct a pseudo-particle description for electron emission due to de-excitation of metastable molecules at surfaces. The pseudo-particle approach allows us to treat resonant…

Strongly Correlated Electrons · Physics 2015-06-05 Johannes Marbach , Franz Xaver Bronold , Holger Fehske

Photoionization of an atom in the presence of a neighboring atom of different species is studied. The latter first undergoes resonant photoexcitation, leading to an autoionizing state of the diatomic system. Afterwards, the excitation…

Atomic Physics · Physics 2020-08-11 F. Grüll , A. B. Voitkiv , C. Müller

A unitary model describing the electronic transitions in an atom subject to a strong high frequency laser pulse is proposed. The model fully accounts for the initial state coupling with the continuum spectrum. Continuum-continuum as well as…

Atomic Physics · Physics 2016-05-10 M. G. Bustamante , V. D. Rodríguez

Oxygen, the third most abundant element in the universe, plays a key role in the chemistry of condensed matter and biological systems. Here, we report evidence for a hitherto unexplored Auger transition in oxides, where a valence band…

We study excitation and ionization in the 1.5 MeV/amu O$^{8+}$-Li collision system, which was the subject of a recent reaction-microscope-type experiment [Fischer \textit{et al.}, Phys. Rev. Lett. \textbf{109}, 113202 (2012)]. Starting from…

Atomic Physics · Physics 2015-01-19 T. Kirchner , N. Khazai , L. Gulyás

The absorption of a photon and the emission of an electron is not a simple, two-particle process. The complicated many-electron features observed during core photo-ionization can therefore reveal many of the hidden secrets about the ground…

Strongly Correlated Electrons · Physics 2018-07-04 J. C. Woicik , J. M. Ablett , N. F. Quackenbush , A. K. Rumaiz , C. Weiland , T. C. Droubay , S. A. Chambers

In this paper we have tried to establish a theory for angular correlation between the photo- and Auger electrons in the two-step double photoionization of a rare gas atom. The basic finding of this paper is that a general theoretical…

Atomic Physics · Physics 2007-05-23 Chiranjib Sur , Dipankar Chattarji

We explore the laser-induced ionization dynamics of N2 and CO2 molecules subjected to a few-cycle, linearly polarized, 800\,nm laser pulse using effective two-dimensional single active electron time-dependent quantum simulations. We show…

Atomic Physics · Physics 2012-10-02 Michel Peters , Tung Nguyen-Dang , Eric Charron , Arne Keller , Osman Atabek

The process of ionization of a hydrogen atom by a short infrared laser pulse is studied in the regime of very large pulse intensity, in the dipole approximation. Let $A$ denote the integral of the electric field of the pulse over time at…

Mathematical Physics · Physics 2015-05-18 Juerg Froehlich , Alessandro Pizzo , Benjamin Schlein

An alternative method to the density matrix formalism for the derivation of general expressions of the interaction of polarized atoms with polarized photons and electrons is presented. The expression for the cross-section describing the…

Quantum Physics · Physics 2015-06-26 A. Kupliauskiene

With an eye on plasma walls we investigate, within an effective model for the two active electrons involved in the process, secondary electron emission due to Auger de-excitation of metastable nitrogen $N_2(^3\sigma^+_u)$ molecules at…

Other Condensed Matter · Physics 2011-09-07 J. Marbach , F. X. Bronold , H. Fehske

We consider photo ionization of an atom which, due to passing through a diffraction grating, is prepared in a multi-site state possessing a periodic space structure with alternating maxima and minima. It has been found that this process…

Atomic Physics · Physics 2020-08-07 S. F. Zhang , B. Najjari , X. Ma , A. B. Voitkiv

The computational treatment of many-electron systems capable of exchanging {electrons and nuclei} with the environment represents one of the outermost frontiers in simulation methodology. The exchanging process occurs in a large variety of…

Chemical Physics · Physics 2019-02-21 Luigi Delle Site