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The drying of a colloidal dispersion can result in a gel phase defined as a porous matrix saturated in solvent. During the drying process, high mechanical stresses are generated. When these stresses exceed the strength of the material, they…

Soft Condensed Matter · Physics 2013-02-15 François Boulogne , Frédérique Giorgiutti-Dauphiné , Ludovic Pauchard

Charged colloidal dispersions make up the basis of a broad range of industrial and commercial products, from paints to coatings and additives in cosmetics. During drying, an initially liquid dispersion of such particles is slowly…

Soft Condensed Matter · Physics 2019-01-07 Lucas Goehring , Joaquim Li , Pree-Cha Kiatkirakajorn

We study the stress developed during the drying of a colloidal drop of silica nanoparticles. In particular, we use the wrinkling instability of a thin floating sheet to measure the net stress applied by the deposit on the substrate and we…

Soft Condensed Matter · Physics 2016-06-15 François Boulogne , Yong Lin Kong , Janine K. Nunes , Howard A. Stone

The process of colloidal drying gives way to particle self-assembly in numerous elds including photonics or biotechnology. Yet, the mechanisms and conditions driving the nal particle arrangement in dry colloidal layers remain elusive. Here,…

The drying of colloidal suspensions leads to complex deposition patterns, accompanied by instabilities such as cracking and delamination. In this study, we experimentally investigate the coupled influence of particle surface charge and…

Soft Condensed Matter · Physics 2026-01-27 A. Madhav Sai Kumar , A. Hari Govindha , Ranajit Mondal , Kirti Chandra Sahu

Drying of colloidal dispersion and their consolidation into a particulate deposit is a common phenomenon. This process involves various physical processes such as diffusion of liquid molecules into the ambient atmosphere and advection of…

Soft Condensed Matter · Physics 2020-12-01 Hisay Lama , Ranajit Mondal

In simulations and experiments, we study the drying of films containing mixtures of large and small colloidal particles in water. During drying, the mixture stratifies into a layer of the larger particles at the bottom with a layer of the…

Thin films made of deformable micro- and nano-units, such as biological membranes, polymer interfaces, and particle-laden liquid surfaces, exhibit a complex behavior during drying, with consequences for various applications like wound…

-- A scientific hurdle in manufacturing solid films by drying colloidal layers is preventing them from fracturing. This paper examines how the drying rate of colloidal liquids influences the particle packing at the nanoscale in correlation…

Soft Condensed Matter · Physics 2016-02-29 Keyvan Piroird , Véronique Lazarus , Georges Gauthier , Arnaud Lesaine , Daniel Bonamy , Cindy Rountree

We consider a carpet of self-propelled particles at the liquid-gas interface of a liquid film on a solid substrate. The particles excert an excess pressure on the interface and also move along the interface while the swimming direction…

Soft Condensed Matter · Physics 2015-06-22 Andrey Pototsky , Uwe Thiele , Holger Stark

Some of our recent studies of the structure and mechanical properties of a special type of nanocomposite are reviewed here. In silica-latex systems, a latex film with silica inclusions is formed from a colloidal solution of both components.…

Soft Condensed Matter · Physics 2007-05-23 Julian Oberdisse

During drying of colloidal suspensions, colloidal particles can form concentrated particle layers beneath the receding free surface. The drying rate can gradually decrease with the growth of the particle layers. We construct a model to…

Soft Condensed Matter · Physics 2023-06-22 Rei Tatsumi , Osamu Koike , Yukio Yamaguchi , Yoshiko Tsuji

The ordering of particles in the drying process of a colloidal suspension is crucial in determining the properties of the resulting film. For example, microscopic inhomogeneities can lead to the formation of cracks and defects that can…

Soft Condensed Matter · Physics 2021-10-04 Maarten Wouters , Othmane Aouane , Marcello Sega , Jens Harting

Drying a droplet of colloidal dispersion can result in complex pattern formation due to both development and deformation of a skin at the drop surface. The present study focus on the drying process of droplets of colloidal dispersions in a…

Soft Condensed Matter · Physics 2012-11-08 François Boulogne , Frédérique Giorgiutti-Dauphiné , Ludovic Pauchard

Substrate wettability alteration induced control over crack formation process in thin colloidal films has been addressed in the present study. Colloidal nanosuspension (53nm, mean particle diameter) droplets have been subjected to natural…

The formation of periodic wrinkles in soft layered materials due to mechanical instabilities is prevalent in nature and has been proposed for use in multiple applications. However, such phenomena have been explored predominantly in…

We develop a dynamical density functional theory based model for the drying of colloidal films on planar surfaces. We consider mixtures of two different sizes of hard-sphere colloids. Depending on the solvent evaporation rate and the…

Soft Condensed Matter · Physics 2021-01-28 Boshen He , Ignacio Martin-Fabiani , Roland Roth , Gyula I. Tóth , Andrew J. Archer

We use molecular dynamics computer simulations to study the equilibrium properties of the surface of amorphous silica. Two types of geometries are investigated: i) clusters with different diameters (13.5\AA, 19\AA, and 26.5\AA) and ii) a…

Statistical Mechanics · Physics 2009-10-31 Alexandra Roder , Walter Kob , Kurt Binder

We report an experimental study of the crack pattern formed during the drying of a colloidal suspension. A horizontal fiber, which provides a one dimensional, boundary-free substrate, is coated by a film of micronic thickness. The geometry…

Soft Condensed Matter · Physics 2014-09-30 François Boulogne , Ludovic Pauchard , Frédérique Giorgiutti-Dauphiné

Wrinkling patterns at the metallized surface of thin polymer films are shown to be sensitive to the sticky or slippery character of the polymer/substrate interface (titanium coating, polystyrene film and coated silicon substrate). Selective…

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