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We theoretically study the electrolyte Seebeck effect in the vicinity of a heated metal nanostructure, such as the cap of an active Janus colloid in an electrolyte, or gold- coated interfaces in optofluidic devices. The thermocharge…

Soft Condensed Matter · Physics 2018-02-27 Aboubakry Ly , Arghya Majee , Alois Würger

We discuss the thermoelectric properties of a locally heated micron-size volume in an electrolyte solution. We find that such a hot spot carries a net charge Q which, for an excess temperature of 10 K, may attain hundreds of elementary…

Soft Condensed Matter · Physics 2014-01-30 Arghya Majee , Alois Wüurger

Thermally driven colloidal transport is, to a large extent, due to the thermoelectric or Seebeck effect of the charged solution.We show that, contrary to the generally adopted single-particle picture, the transport coefficient depends on…

Soft Condensed Matter · Physics 2014-01-30 Arghya Majee , Alois Würger

We report on the direct observation of the thermoelectric transport in a nondegenerate correlated electron system formed on the surface of liquid helium. We find that the microwave-induced excitation of the vertical transitions of electrons…

Other Condensed Matter · Physics 2021-11-10 Ivan Kostylev , A. A. Zadorozhko , M. Hatifi , Denis Konstantinov

When two electrolyte-immersed electrodes have different temperatures, a voltage $\Delta \psi$ can be measured between them. This electrolyte Seebeck effect is usually explained by cations and anions flowing differently in thermal gradients.…

Chemical Physics · Physics 2023-09-15 Ole Nickel , Ludwig J. V. Ahrens-Iwers , Robert H. Meißner , Mathijs Janssen

We discuss the peculiarities of the Seebeck effect in stabilized electrolytes containing the colloidal particles. Its unusual feature is the two-stage character, with the linear increase of differential thermopower as the function of…

Soft Condensed Matter · Physics 2021-02-24 Ioulia Chikina , Sawako Nakamae , Valeriy Shikin , Andrey Varlamov

The Seebeck effect describes the generation of an electric potential in a conducting solid exposed to a temperature gradient. Besides fundamental relevance in solid state physics, it serves as a key quantity to determine the performance of…

Single-ion Soret coefficients $\alpha_{i}$ characterize the tendency of ions in an electrolyte solution to move in a thermal gradient. When these coefficients differ between cations and anions, an electric field can be generated. For this…

Chemical Physics · Physics 2021-05-03 André Luiz Sehnem , Mathijs Janssen

Ionic thermoelectricity in nanochannels has received increasing attention because of its advantages such as high Seebeck coefficient and low cost. However, most studies have focused on dilute simple electrolytes that neglect the effects of…

Soft Condensed Matter · Physics 2023-08-17 Wenyao Zhang , Xinxi Liu , Kai Jiao , Qiuwang Wang , Chun Yang , Cunlu Zhao

The Seebeck and Soret coefficients of ionically stabilized suspension of maghemite nanoparticles in dimethyl sulfoxide are experimentally studied as a function of nanoparticle volume fraction. In the presence of a temperature gradient, the…

Ionic Seebeck effect of electrolytes has shown promising applications in harvesting energy from low-grade waste-heat sources with small temperature difference from the environment, which can power sensors and Internet-of-Things devices.…

Soft Condensed Matter · Physics 2022-02-03 Xin Qian , Te-Huan Liu , Ronggui Yang

We develop an electrokinetic technique that continuously manipulates colloidal particles to concentrate into patterned particulate groups in an energy efficient way, by exclusive harnessing of the intrinsic Joule heating effects. Our…

Applied Physics · Physics 2019-04-17 Golak Kunti , Jayabrata Dhar , Anandaroop Bhattacharya , Suman Chakraborty

A systematic theoretical study of thermoelectric effect and temperature-gradient-driven electrokinetic flow of electrolyte solutions in charged nanocapillaries is presented. The study is based on a semianalytical model developed by…

Fluid Dynamics · Physics 2023-09-14 Wenyao Zhang , Qiuwang Wang , Min Zeng , Cunlu Zhao

The application of a temperature gradient to an extended system generates an electromotive force that induces an electric current in conductors and a macroscopic polarization in insulators. The ratio of the electromotive force to the…

Materials Science · Physics 2024-02-01 Enrico Drigo , Stefano Baroni

Colloids with patchy metal coating under laser irradiation could act as local sources of heat due to the absorption of light. While for asymmetric colloids this could induce self-propulsion, it also leads to the generation of a slowly…

Soft Condensed Matter · Physics 2015-05-30 Ramin Golestanian

We investigate nonequilibrium effects in the transport of interacting electrons in quantum conductors, proposing the nonlocal thermoelectric response as a direct indicator of the presence of interactions, nonthermal states and the effect of…

Mesoscale and Nanoscale Physics · Physics 2024-05-10 Alessandro Braggio , Matteo Carrega , Björn Sothmann , Rafael Sánchez

We study the Soret effect of charged polystyrene particles as a function of temperature and electrolyte composition. As a main result we find that the Soret coefficient is determined by charge effects, and that non-ionic contributions are…

Soft Condensed Matter · Physics 2014-02-28 Kyriakos A. Eslahian , Arghya Majee , Michael Maskos , Alois Würger

The atomic variations of electronic wavefunctions at the surface and electron scattering near a defect have been detected unprecedentedly by tracing thermoelectric voltages given a temperature bias [Cho et al., Nature Mater. 12, 913…

Mesoscale and Nanoscale Physics · Physics 2014-04-02 Eui-Sup Lee , Sanghee Cho , Ho-Ki Lyeo , Yong-Hyun Kim

The non-equilibrium distribution of colloids in a polymer solution under a temperature gradient is studied experimentally. A slight increase of local temperature by a focused laser drives the colloids towards the hot region, resulting in…

Soft Condensed Matter · Physics 2015-05-13 Hong-Ren Jiang , Hirofumi Wada , Natsuhiko Yoshinaga , Masaki Sano

We study the thermal diffusion coefficient DT of a charged colloid in a temperature gradient, and find that it is to a large extent determined by the thermoelectric response of the electrolyte solution. The thermally induced salinity…

Soft Condensed Matter · Physics 2014-01-30 Alois Würger
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