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We report measurements of energy-dependent attosecond photoionization delays between the two outer-most valence shells of N$_2$O and H$_2$O. The combination of single-shot signal referencing with the use of different metal foils to filter…

Atomic Physics · Physics 2016-09-21 Martin Huppert , Inga Jordan , Denitsa Baykusheva , Aaron von Conta , Hans Jakob Wörner

Photon exchange due to nuclear bremsstrahlung during nuclear collisions can cause Coulomb excitation in the projectile and the target nuclei. The corresponding process originated in nuclear timescales can also be observed in atomic…

Attosecond photoionisation time delays reveal information about the potential energy landscape an outgoing electron wavepacket probes upon ionisation. In this study we experimentally quantify, for the first time, the dependence of the time…

We calculate the transient absorption of an isolated attosecond pulse by helium atoms subject to a delayed infrared (\ir) laser pulse. With the central frequency of the broad attosecond spectrum near the ionization threshold, the absorption…

Atomic Physics · Physics 2015-06-12 Shaohao Chen , Mengxi Wu , Mette B. Gaarde , Kenneth J. Schafer

We study laser-assisted photodetachment time delays by attosecond pulse trains from the closed-shell negative ions F- and Cl-. We investigate the separability of the delay into two contributions: (i) the Wigner-like delay associated with…

Atomic Physics · Physics 2017-09-13 Eva Lindroth , Jan Marcus Dahlström

We describe in detail how attosecond delays in laser-assisted photoionization can be computed using perturbation theory based on two-photon matrix elements. Special emphasis is laid on above-threshold ionization, where the electron…

Atomic Physics · Physics 2015-06-19 J. M. Dahlström , E. Lindroth

We investigate the behavior of light pulse propagation in a 4-level double Lambda atomic system under condition of electromagnetically induced transparency. The Fano type interference effect and spectral hole burning appears in the the…

Optics · Physics 2013-11-28 Bakhtt A Bacha , Fazal Ghafoor , Iftikhar Ahmad

This tutorial presents an introduction to the interaction of light and matter on the attosecond timescale. Our aim is to detail the theoretical description of ultra-short time-delays, and to relate these to the phase of extreme ultraviolet…

Atomic Physics · Physics 2012-07-20 J. M. Dahlström , A. L'Huillier , A. Maquet

The photoelectric effect is not truly instantaneous, but exhibits attosecond delays that can reveal complex molecular dynamics. Sub-femtosecond duration light pulses provide the requisite tools to resolve the dynamics of photoionization.…

Recently the time delay in the attosecond photoemission was observed (Science,2010). In this paper we propose the description of that time delay in the framework of hyperbolic heat transport equation. We argue that the observed time delay…

General Physics · Physics 2013-02-20 J. Marciak-Kozlowska , M. Kozlowski

The development of attosecond technology has enabled the real-time observation of coherent electron motion in atoms, molecules and condensed phases. Experimentally, it is now possible to generate laser pulses of durations of only a few tens…

Chemical Physics · Physics 2017-05-18 David Ayuso

In the interaction of laser pulses of extreme intensity ($>10^{23}~{\rm W cm}^{-2}$) with high-density, thick plasma targets, simulations show significant radiation friction losses, in contrast to thin targets for which such losses are…

Plasma Physics · Physics 2019-03-27 S. V. Popruzhenko , T. V. Liseykina , A. Macchi

An analytic study is presented of the efficient multiphoton excitation and strong harmonic generation in three-level systems specified by a pair of nearly degenerate, strongly dipole-coupled excited states. Such systems are physically…

Quantum Physics · Physics 2015-05-19 Michal Berent , Ryszard Parzyński

Numerous X-ray bursts show strong oscillations in their flux at several hundred Hz as revealed by RXTE. Analyzing one such oscillation from the X-ray binary Aql X-1, I find that low energy photons (3.5-5.7 keV) lag high energy photons (>5.7…

Astrophysics · Physics 2009-10-31 Eric C. Ford

We show that if the laser is intense enough, it may always ionize an atom or induce transitions between discrete energy levels of the atom, no matter what is its frequency. It means in the quantum transition of an atom interacting with an…

Quantum Physics · Physics 2007-05-23 Qi-Ren Zhang

It is shown that the effect of hole-burning under conditions of coherent population oscillations as well as the light pulse delay in a saturable absorber (a modification of the "slow light" effect) can be interpreted, in a comprehensive…

Optics · Physics 2009-11-13 V. S. Zapasskii , G. G. Kozlov

A technique for measuring photoionization time delays with attosecond precision is combined with calculations of photoionization matrix elements to demonstrate how multi-electron dynamics affect photoionization time delays in carbon…

We study photoionization of argon atoms excited by attosecond pulses using an interferometric measurement technique. We measure the difference in time delays between electrons emitted from the $3s^2$ and from the $3p^6$ shell, at different…

When an atom or molecule absorbs a high-energy photon, an electron is emitted with a well-defined energy and a highly-symmetric angular distribution, ruled by energy quantization and parity conservation. These rules seemingly break down…

With the development of laser technology, pulse length enters the optical cycle regime and hence the interaction time between laser pulse and atoms becomes prominent. We investigate this problem in this Letter through the photoelectron…

Optics · Physics 2010-04-13 Yang Xiang , Yueping Niu , Yihong Qi , Shangqing Gong
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