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In the last decade, there has been a proliferation of laser sources for time- and angle-resolved photoemission spectroscopy (TR-ARPES), building on the proven capability of this technique to tackle important scientific questions. In this…

Optics · Physics 2023-10-26 MengXing Na , Arthur K. Mills , David J. Jones

We describe a setup of time-, spin-, and angle-resolved photoemission spectroscopy (tr-SARPES) employing a 10.7-eV ($\lambda$=115.6 nm) pulse laser at 1-MHz repetition rate as a probe photon source. This equipment effectively combines…

A synchrotron radiation beamline in the photon energy range of 18 - 240 eV and an electron spectroscopy end station have been constructed at the 3 GeV Diamond Light Source storage ring. The instrument features a variable polarisation…

We demonstrate a versatile technique for generating continuously wavelength-tunable laser waveforms, with mJ pulse energies and ultrashort pulse durations down to few-cycle in the ultraviolet C and visible spectral ranges. Using the…

The paper describes a time- and angle-resolved photoemission apparatus consisting of a hemispherical analyzer and a pulsed laser source. We demonstrate 1.48-eV pump and 5.90-eV probe measurements at the >10.5-meV and >240-fs resolutions by…

Materials Science · Physics 2016-12-16 Y. Ishida , T. Togashi , K. Yamamoto , M. Tanaka , T. Kiss , T. Otsu , Y. Kobayashi , S. Shin

We have developed a state-of-the-art apparatus for laser-based spin- and angle-resolved photoemission spectroscopy with micrometer spatial resolution (micro-SARPES). This equipment is achieved through the combination of a high-resolution…

We present the development of a time- and angle-resolved photoemission spectroscopy based on a Yb-based femtosecond laser and a hemispherical electron analyzer. The energy of the pump photon is tunable between 1.4 and 1.9 eV, and the pulse…

Strongly Correlated Electrons · Physics 2020-03-03 Yuanyuan Yang , Tianwei Tang , Shaofeng Duan , Chaocheng Zhou , Duxing Hao , Wentao Zhang

The quest for mapping the femtosecond dynamics of the electronic band structure of complex materials via Time- and Angle-Resolved Photoelectron Spectroscopy (TR-ARPES) over their full First Brillouin Zone is pushing the development of…

We report on the development of a high-order harmonic generation (HHG)-based ultrafast high-repetition-rate (250 kHz) monochromatic extreme ultraviolet (21.6 eV) source with polarization tunability, specifically designed for multi-modal…

Scaling femtosecond terahertz (THz) and ultraviolet (UV) sources to high repetition rates is essential for high-throughput ultrafast spectroscopy and imaging applications. Yet, their efficient generation at high average power remains…

Optics · Physics 2026-01-06 Andrey Ryabov , Kasra Amini

A VUV beamline at SSRF for ARPES measurements are designed. To increase the resolution and bulk sensitivity, the photon energy as low as 7 eV is desired. Because the reflectivity for p-polarized photons strongly decreases when the photon…

Instrumentation and Detectors · Physics 2015-02-12 Jiajia Wang , Mao Ye , Tan Shi , Rui Chang , Shan Qiao

Angle-resolved photoemission spectroscopy with sub-micrometer spatial resolution ({\mu}-ARPES), has become a powerful tool for studying quantum materials. To achieve sub-micrometer or even nanometer-scale spatial resolution, it is important…

We demonstrate a wideband-tunable Q-switched fiber laser exploiting a graphene saturable absorber. We get ~2us pulses, tunable between 1522 and 1555nm with up to~40nJ energy. This is a simple and low-cost light source for metrology,…

Mesoscale and Nanoscale Physics · Physics 2015-05-20 D. Popa , Z. Sun , T. Hasan , F. Torrisi , F. Wang , A. C. Ferrari

A solid-state organic thin-film laser with intracavity frequency doubling is reported. Tunable ultraviolet emission from 309 to 322 nm is achieved from a vertical external cavity surface-emitting organic laser, with 2 % efficiency (1 $\mu$J…

Time- and angle-resolved photoelectron spectroscopy (trARPES) is a powerful method to track the ultrafast dynamics of quasiparticles and electronic bands in energy and momentum space. We present a setup for trARPES with 22.3 eV…

In order to meet requirements of the synchrotron radiation users, a fully coherent VUV free electron laser (FEL) has been preliminarily designed. One important goal of this design is that the radiation wavelength can be easily tuned in a…

Accelerator Physics · Physics 2013-06-24 Li He-Ting , Jia Qi-Ka

The significant progress in angle-resolved photoemission spectroscopy (ARPES) in last three decades has elevated it from a traditional band mapping tool to a precise probe of many-body interactions and dynamics of quasiparticles in complex…

Superconductivity · Physics 2018-04-13 Xingjiang Zhou , Shaolong He , Guodong Liu , Lin Zhao , Li Yu , Wentao Zhang

Recent progress in laser-based high-repetition rate extreme ultraviolet (EUV) lightsources and multidimensional photoelectron spectroscopy enable the build-up of a new generation of time-resolved photoemission experiments. Here, we present…

Unraveling and controlling chemical dynamics requires techniques to image structural changes of molecules with femtosecond temporal and picometer spatial resolution. Ultrashort-pulse x-ray free-electron lasers have significantly advanced…

We present a source of coherent extreme ultraviolet (XUV) radiation with a flux of 10$^{13}$ photons per second at 26.5 eV. The source is based on high-harmonic generation (HHG) in argon and pumped by a frequency-doubled 100 kHz repetition…