Related papers: Multiple Ionization under Strong XUV to X-ray Radi…
We analyze the role of shake-off and of the final state interactions in inelastic processes in the fullerene shell which follow ionization of the caged atom. We demonstrate that in the broad interval of the photon energies the process is…
We theoretically examine neon atoms in ultrashort and intense x rays from free electron lasers and compare our results with data from experiments conducted at the Linac Coherent Light Source (LCLS). For this purpose, we treat in detail the…
We present a theoretical study of atomic ionization due to an XUV pulse in the presence of an infrared laser. Within the strong field approximation and considering the periodicity and symmetry of the transition matrix we show that the…
Strong field ionization of benzene, fluorobenzene, benzonitrile and 1-chloro-2-fluorobenzene, is studied within the framework of real-space and real-time time-dependent density functional theory. Analysis of the ionization rates as function…
Multiple electron processes occur widely in atoms, molecules, clusters, and condensed matters when they are interacting with energetic particles or intense laser fields. In this work, a unified and accurate theoretical formalism is proposed…
We present a novel approach to calculating strong field ionization dynamics of multielectron molecular targets. Adopting a multielectron wavefunction ansatz based on field-free ab initio neutral and ionic multielectron states, a set of…
We study strong-field molecular ionization as a function of pulse duration. Experimental measurements of the photoelectron yield for a number of molecules reveal competition between different ionization continua (cationic states) which…
We present a theoretical description of atomic strong-field photoionization. Specifically, we consider an atom driven by a combination of two electromagnetic fields: a high-frequency field assisted by an intense, low-frequency laser. We…
We study strong field molecular ionization using few- (four to ten) cycle laser pulses. Employing a supercontinuum light source, we are able to tune the optical laser wavelength (photon energy) over a range of about $\sim$200 nm (500 meV).…
Resonant two-photon ionization in a system consisting of two spatially well-separated atoms is studied. Due to two-center electron-electron correlations, the ionization may also proceed through photo-excitation of both atoms with subsequent…
We extend the semiclassical two-step model [Phys. Rev. A 94, 013415 (2016)] to include a multielectron polarization-induced dipole potential. Using this model we investigate the imprints of multielectron effects in the momentum…
We give examples showing that two well-known versions of the S-matrix theory, which describes a nonresonant multiphoton ionization of atoms and ions in intense laser fields, lead to qualitatively different results. The latter refer not only…
Intense light with frequencies above typical atomic or molecular ionization potentials as provided by free-electron lasers couples many photons into extended targets such as clusters and biomolecules. This implies, in contrast to…
Photoionization of an atom via interatomic correlations to N neighboring atoms may be strongly enhanced due to constructive interference of quantum pathways. The ionization proceeds via resonant photoexcitation of a neighbor atom and…
Understanding the interaction of intense, femtosecond X-ray pulses with heavy atoms is crucial for gaining insights into the structure and dynamics of matter. One key aspect of nonlinear light-matter interaction was, so far, not studied…
Strong-field photoelectron momentum imaging of the prototypical biomolecule indole was disentangled in a combined experimental and computational approach. Experimentally, strong control over the molecules enabled the acquisition of…
We present a study of multiphoton dissociative ionization from molecules. By solving the time-dependent Schr\"{o}dinger equation for H$_2^+$ and projecting the solution onto double continuum scattering states, we observe the correlated…
When a strong laser pulse induces the ionization of an atom, momentum conservation dictates that the absorbed photons transfer their momentum $p_{\gamma}=E_{\gamma}/c$ to the electron and its parent ion. Even after 30 years of studying…
We present a theory illuminating the cross-over from strong-field tunnelling ionization to weak-field multiphoton ionization in the interaction of a classical laser field with a hydrogen atom. A simple formula is derived in which the…
We investigate the laser-assisted single XUV photon double ionization of ground state helium. By solving full six-dimensional time-dependent schr{\"o}dinger equation, we study the correlation and angular distribution. The discussion in…