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We perform time- and angle-resolved photoemission spectroscopy of a prototypical topological insulator Bi$_2$Se$_3$ to study the ultrafast dynamics of surface and bulk electrons after photo-excitation. By analyzing the evolution of surface…

Mesoscale and Nanoscale Physics · Physics 2015-03-20 Y. H. Wang , D. Hsieh , E. J. Sie , H. Steinberg , D. R. Gardner , Y. S. Lee , P. Jarillo-Herrero , N. Gedik

Using time-, spin- and angle-resolved photoemission, we investigate the ultrafast spin dynamics of hot electrons on the surface of the topological insulator Bi$_2$Te$_3$ following optical excitation by fs-infrared pulses. We observe two…

Mesoscale and Nanoscale Physics · Physics 2017-05-22 J. Sánchez-Barriga , M. Battiato , M. Krivenkov , E. Golias , A. Varykhalov , A. Romualdi , L. V. Yashina , J. Minár , O. Kornilov , H. Ebert , K. Held , J. Braun

Using femtosecond time- and angle- resolved photoemission spectroscopy, we investigated the nonequilibrium dynamics of the topological insulator Bi2Se3. We studied p-type Bi2Se3, in which the metallic Dirac surface state and bulk conduction…

We have studied the energy dispersion of the Dirac bands of the topological insulator Bi2Se3 at large parallel momenta using a setup for laser-based time-resolved momentum microscopy with 6 eV probe-photons. Using this setup, we can probe…

Ultrafast carrier dynamics in the topological insulator Bi2Se3 have recently been intensively studied using a variety of techniques. However, we are not aware of any successful experiments exploiting transient absorption (TA) spectroscopy…

Mesoscale and Nanoscale Physics · Physics 2021-05-31 Yuri D. Glinka , Junzi Li , Tingchao He , Xiao Wei Sun

We study ultrafast population dynamics in the topological surface state of Sb$_2$Te$_3$ in two-dimensional momentum space with time- and angle-resolved two-photon photoemission. Linear polarized mid-infrared pump pulses are used to permit a…

Mesoscale and Nanoscale Physics · Physics 2023-04-26 J. Reimann , K. Sumida , M. Kakoki , K. A. Kokh , O. E. Tereshchenko , A. Kimura , J. Güdde , U. Höfer

We discuss the ultrafast evolution of the surface electronic structure of the topological insulator Bi$_2$Te$_3$ following a femtosecond laser excitation. Using time and angle resolved photoelectron spectroscopy, we provide a direct…

We exploit time- and angle- resolved photoemission spectroscopy to determine the evolution of the out-of-equilibrium electronic structure of the topological insulator Bi2Se. The response of the Fermi-Dirac distribution to ultrashort IR…

Mesoscale and Nanoscale Physics · Physics 2012-12-17 A. Crepaldi , B. Ressel , F. Cilento , M. Zacchigna , C. Grazioli , H. Berger , Ph. Bugnon , K. Kern , M. Grioni , F. Parmigiani

Scanning tunneling microscopy and spectroscopy have been used to investigate the femtosecond dynamics of Dirac fermions in the topological insulator Bi$_2$Se$_3$ ultrathin films. At two-dimensional limit, bulk electrons becomes quantized…

Mesoscale and Nanoscale Physics · Physics 2015-05-08 Can-Li Song , Lili Wang , Ke He , Shuai-Hua Ji , Xi Chen , Xu-Cun Ma , Qi-Kun Xue

Angle-resolved photoelectron spectroscopy is used for a detailed study of the electronic structure of the topological insulator Bi2Se3. Nominally stoichiometric and calcium-doped samples were investigated. The pristine surface shows the…

Topological insulators (TIs) are a new quantum state of matter. Their surfaces and interfaces act as a topological boundary to generate massless Dirac fermions with spin-helical textures. Investigation of fermion dynamics near the Dirac…

We characterize the occupied and unoccupied electronic structure of the topological insulator Bi$_2$Se$_3$ by one-photon and two-photon angle-resolved photoemission spectroscopy and slab band structure calculations. We reveal a second,…

This article reviews experimental work on the ultrafast electron dynamics in the topological surface state (TSS) of three-dimensional (3D) topological insulators (TIs) observed with time- and angle-resolved two-photon photoemission (2PPE).…

Mesoscale and Nanoscale Physics · Physics 2021-02-03 Jens Güdde , Ulrich Höfer

The nature of the Dirac quasiparticles in topological insulators calls for a direct investigation of the electron-phonon scattering at the \emph{surface}. By comparing time-resolved ARPES measurements of the TI Bi_{2}Se_{3} with different…

Gapless surface states on topological insulators are protected from elastic scattering on non-magnetic impurities which makes them promising candidates for low-power electronic applications. However, for wide-spread applications, these…

Strongly Correlated Electrons · Physics 2013-01-09 Z. -H. Pan , A. V. Fedorov , D. Gardner , Y. S. Lee , S. Chu , T. Valla

We report time- and angle-resolved photoemission spectroscopy measurements on the topological insulator Bi2Se3. We observe oscillatory modulations of the electronic structure of both the bulk and surface states at a frequency of 2.23 THz…

We present energy-momentum mapping of surface Dirac photocurrent in the topological insulator Sb$_2$Te$_3$ by means of time- and angle-resolved two-photon photoemission spectroscopy combined with polarization-variable mid-infrared pulse…

Materials Science · Physics 2017-02-08 Kenta Kuroda , J. Reimann , K. A. Kokh , O. E. Tereshchenko , A. Kimura , J. Güdde , U. Höfer

We report on time-resolved ultrafast optical spectroscopy study of the topological insulator (TI) Bi$_2$Se$_3$. We unravel that a net spin polarization can not only be generated using circularly polarized light via interband transitions…

Materials Science · Physics 2016-01-26 M. C. Wang , S. Qiao , Z. Jiang , S. N. Luo , J. Qi

Individual relaxation dynamics of electrons and holes in optically pumped semiconductors is rarely observed due to their overlap. Here we report the individual dynamics of long-lived (~200 mks) holes observed at room temperature in a 10 nm…

Mesoscale and Nanoscale Physics · Physics 2022-12-06 Yuri D. Glinka , Tingchao He , Xiao Wei Sun

The electron dynamics of the topological surface state on Bi2Se3(111) is investigated by temperature-dependent angle-resolved photoemission. The electron-phonon coupling strength is determined in a spectral region for which only intraband…

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