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We investigated the temperature-dependent evolution of the electronic structure of the Jeff,1/2 Mott insulator Sr2IrO4 using optical spectroscopy. The optical conductivity spectra $\sigma(\omega)$ of this compound has recently been found to…

Strongly Correlated Electrons · Physics 2009-10-23 S. J. Moon , Hosub Jin , W. S. Choi , J. S. Lee , S. S. A. Seo , J. Yu , G. Cao , T. W. Noh , Y. S. Lee

We report on the optical excitation spectra in Sr$_2$VO$_4$. The phonon modes are assigned and their evolution with temperature is discussed in the frame of the different phase transitions crossed upon cooling. Besides the expected…

Strongly Correlated Electrons · Physics 2015-05-30 J. Teyssier , R. Viennois , E. Giannini , R. M. Eremina , A. G. Gunter , J. Deisenhofer , M. V. Eremin , D. van der Marel

The infrared transmission measurement was performed for a two-dimensional spin-orbit coupling induced Mott insulator Sr$_{2}$IrO$_{4}$ with a layered-perovskite structure. A phonon-assisted magnon mode was observed at around 1870 cm$^{-1}$…

Strongly Correlated Electrons · Physics 2015-06-12 Yasuyuki Hirata , Hiroyuki Tajima , Kenya Ohgushi

In indirect band gap materials, phonon-assisted processes are key mechanisms for photoluminescence (PL). Using a first-principles many-body approach, we systematically investigate the phonon-assisted PL in bilayer MoS$_2$ and its dependence…

Materials Science · Physics 2026-02-25 Gyanu P. Kafle , Zhen-Fei Liu

Raman scattering experiments on stoichiometric, Mott-insulating LaTiO$_3$ over a wide range of excitation energies reveal a broad electronic continuum which is featureless in the paramagnetic state, but develops a gap of $\sim 800$…

Strongly Correlated Electrons · Physics 2015-10-28 C. Ulrich , G. Khaliullin , M. Guennou , H. Roth , T. Lorenz , B. Keimer

We have observed the characteristic temperature dependence of the intermolecular phonon spectrum in the organic dimer Mott insulator kappa-(ET)2Cu2(CN)3 exhibiting a dielectric anomaly at 30 K. The anomalous spectral narrowing of the 55…

Strongly Correlated Electrons · Physics 2015-06-16 K. Itoh , H. Itoh , S. Saito , I. Hosako , Y. Nakamura , H. Kishida , N. Yoneyama , T. Sasaki , S. Ishihara , S. Iwai

We report a comprehensive Raman study of the phonon behaviour in PdSe$_2$ in the temperature range of 5 K to 300 K. A remarkable change in the Raman spectrum is observed at 120 K: a significant enhancement of the out-of-plane phonon…

An infrared study of the phonon spectra of ZrW2O8 as a function of temperature which includes the low energy (2-10 meV) region relevant to negative thermal expansion is reported and discussed in the context of specific heat and neutron…

Materials Science · Physics 2010-07-28 Jason N. Hancock , Chandra Turpen , Zack Schlesinger , Glen Kowach , Art Ramirez

We investigated temperature dependent optical conductivity spectra of La_{7/8}Sr_{1/8}MnO_3. Its phonon bending mode starts to be splitted near a structural phase transition temperature. With further cooling, strength of a mid-infrared…

Strongly Correlated Electrons · Physics 2009-10-31 J. H. Jung , K. H. Kim , H. J. Lee , J. S. Ahn , N. J. Hur , T. W. Noh , M. S. Kim , J. -G. Park

We investigate experimentally the ultrafast changes in the spectral response of the Mott insulator $\kappa$-(BEDT-TTF)$_2$Cu[N(CN)$_2$]Cl ($\kappa$-Cl) upon photodoping with intense excitation at 1.6 eV and probing with continuum pulses…

Strongly Correlated Electrons · Physics 2023-10-31 Konstantin Warawa , Yassine Agarmani , Harald Schubert , Martin Dressel , Michael Lang , Hartmut G. Roskos , Mark D. Thomson

We have investigated the excitation spectra of $j_{eff}$=$\frac{1}{2}$ Mott insulator Na$_2$IrO$_3$. Taking into account a relativistic multiplet structure of Ir ions, we have calculated the optical conductivity $\sigma(\omega)$ and…

Strongly Correlated Electrons · Physics 2014-02-25 Beom Hyun Kim , G. Khaliullin , B. I. Min

Applying newly developed dynamical density matrix renormalization group techniques at zero and finite temperatures to a Hubbard-Holstein model at half-filling, we examine the optical conductivity of a typical one-dimensional Mott insulator…

Strongly Correlated Electrons · Physics 2010-11-30 Shigetoshi Sota , Takami Tohyama

The infrared reflectance of the transition metal chalcogenide 1T-TaS2 has been measured at temperatures from 30K to 360K over 30-45,000cm^-1 (4meV-5.5eV). The optical conductivity was obtained by Kramers-Kronig analysis. At 360K only modest…

Condensed Matter · Physics 2013-10-31 L. V. Gasparov , K. G. Brown , A. C. Wint , D. B. Tanner , H. Berger , R. Gaal , L. Forro , G. Margaritondo

Sn-doped In$_2$O$_3$ or ITO is the most widely used transparent conducting oxide. We use first-principles calculations to investigate the limitations to its transparency due to free-carrier absorption mediated by phonons or charged defects.…

Materials Science · Physics 2019-08-27 H. Peelaers , E. Kioupakis , C. G. Van de Walle

Magnetic properties of Mott-Hubbard insulators are determined by superexchange interactions mediated by the high-spin (HS) and low-spin (LS) intersite d-d charge excitations, which can be associated with the HS- and LS-Hubbard subbands in…

Strongly Correlated Electrons · Physics 2023-10-19 N. N. Kovaleva

We have measured the intricate temperature dependence of the Co L2,3 x-ray absorption spectra (2p-3d excitations) of CoO. To allow for accurate total electron yield measurements, the material has been grown in thin film form on a metallic…

Strongly Correlated Electrons · Physics 2008-06-24 M. W. Haverkort , A. Tanaka , Z. Hu , H. H. Hsieh , H. -J. Lin , C. T. Chen , L. H. Tjeng

The isospin-phonon coupling in Sr2IrO4 is investigated by temperature dependent phonon Raman scattering. Anomalous behavior in the frequency of all studied optical phonons is observed below the magnetic transition temperature TN ~240 K. The…

Strongly Correlated Electrons · Physics 2019-04-23 Kousik Samanta , Danilo Rigitano , Pascoal Jose Giglio Pagliuso , Eduardo Granado

We develop an approximate theory of phonon-induced topological insulation in Dirac materials. In the weak coupling regime, long wavelength phonons may favor topological phases in Dirac insulators with direct and narrow bandgaps. This…

Strongly Correlated Electrons · Physics 2014-05-09 Kush Saha , Ion Garate

We propose phonon spectroscopy by electric measurements of the low-temperature conductance of coupled-quantum dots, specifically employing dephasing of the quantum electronic transport by the phonons. The setup we consider consists of a…

Mesoscale and Nanoscale Physics · Physics 2013-05-29 A. Ueda , O. Entin-Wohlman , M. Eto , A. Aharony

We investigate ultrafast dynamics from photoinduced reflectivity of Sr2RhO4 by using femtosecond near-infrared pulses. We observe a clear temperature-dependent anomaly in its electronic dynamics which slows down below 160 K. In addition,…

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