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UKRmol+ is a new implementation of the UK R-matrix electron-molecule scattering code. Key features of the implementation are the use of quantum chemistry codes such as Molpro to provide target molecular orbitals; the optional use of mixed…

Computational Physics · Physics 2020-02-19 Zdeněk Mašín , Jakub Benda , Jimena D. Gorfinkiel , Alex G. Harvey , Jonathan Tennyson

We formulate a computationally efficient time-independent method based on the multi-electron molecular R-matrix formalism. This method is used to calculate transition matrix elements for the multi-photon ionization of atoms and molecules…

Atomic Physics · Physics 2022-05-10 Jakub Benda , Zdeněk Mašín

Spatially-structured laser beams, eventually carrying orbital angular momentum, affect electronic transitions of atoms and their motional states in a complex way. We present a general framework, based on the spherical tensor decomposition…

The study of electronic transitions within a molecule connected to the absorption or emission of light is a common task in the process of the design of new materials. The transitions are complex quantum mechanical processes and a detailed…

Human-Computer Interaction · Computer Science 2021-06-03 Talha Bin Masood , Signe Sidwall Thygesen , Mathieu Linares , Alexei I. Abrikosov , Vijay Natarajan , Ingrid Hotz

We present a new extension of the UKRmol electron-molecule scattering code suite, which allows one to compute ab initio photoionization and photorecombination amplitudes for complex molecules, resolved both on the molecular alignment…

Chemical Physics · Physics 2014-02-18 Alex G Harvey , Danilo S Brambila , Felipe Morales , Olga Smirnova

Molecular hydrogen ions are of metrological relevance due to the possibility of precise theoretical evaluation of their spectrum and of external-field-induced shifts. In homonuclear molecular ions the electric dipole $E1$ transitions are…

Atomic Physics · Physics 2021-01-20 P. Danev , D. Bakalov , V. I. Korobov , S. Schiller

Non-radiative energy transfer between a Rydberg atom and a polar molecule can be controlled by a DC electric field. Here we show how to exploit this control for state-resolved, non-destructive detection and spectroscopy of the molecules…

Atomic Physics · Physics 2023-11-28 Sabrina Patsch , Martin Zeppenfeld , Christiane P. Koch

Implementation of Effective Core Potentials (ECPs) into the molecular scattering suite UKRmol+ is presented together with a set of calculations for a range of targets relevant for plasma modeling. Continuum description in scattering and…

Electronic transitions in molecules due to absorption or emission of light is a complex quantum mechanical process. Their study plays an important role in the design of novel materials. A common yet challenging task in the study is to…

Electronic transitions in molecules due to the absorption or emission of light is a complex quantum mechanical process. Their study plays an important role in the design of novel materials. A common yet challenging task in the study is to…

Human-Computer Interaction · Computer Science 2023-02-02 Mohit Sharma , Talha Bin Masood , Signe S. Thygesen , Mathieu Linares , Ingrid Hotz , Vijay Natarajan

The R-matrix method has been used for theoretical calculation of electron collision with atoms and molecules for long years. The method was also formulated to treat photoionization process, however, its application has been mostly limited…

Chemical Physics · Physics 2010-04-08 Motomichi Tashiro

Electron injection from an adsorbed molecule to the substrate (heterogeneous electron transfer) is studied. One reaction coordinate is used to model this process. The surface phonons and/or the electron-hole pairs together with the internal…

Chemical Physics · Physics 2009-11-07 Michael Schreiber , Ivan Kondov , Ulrich Kleinekathoefer

Electron-atom collisions in warm dense plasmas are crucial for astrophysics and controlled fusion research, where calculating short-range scattering matrices under screening plasma potentials is essential. While electron-neutral atom…

Atomic Physics · Physics 2026-01-28 Chao Wu , Wen Hao Xia , Yong Wu , Jun Yan , Ming Li , Jian Guo Wang , Xiang Gao

For a molecule, the two-center interference and the molecular scattering phase of the electron are important for almost all the processes that may occur in a laser field. In this study, we investigate their effects in the transfer of linear…

Atomic Physics · Physics 2018-12-19 Hao Liang , Mu-Xue Wang , Xiang-Ru Xiao , Qihuang Gong , Liang-You Peng

Detecting the internal state of polar molecules is a substantial challenge when standard techniques such as resonance-enhanced multi photon ionization (REMPI) or laser-induced fluorescense (LIF) do not work. As this is the case for most…

Atomic Physics · Physics 2014-12-01 Rosa Glöckner , Alexander Prehn , Gerhard Rempe , Martin Zeppenfeld

Coherent transition radiation (CTR) from relativistic electron beam interaction with an overdense plasma foil is investigated by making use of two-dimensional particle-in-cell simulations. Well-defined single electron beam either of uniform…

Plasma Physics · Physics 2019-02-14 W. J. Ding , F. Y. Li , S. M. Weng , P. Bai , Z. M. Sheng

Our computation effort is primarily concentrated on support of current and future measurements being carried out at various synchrotron radiation facilities around the globe, and photodissociation computations for astrophysical…

Atomic Physics · Physics 2017-01-17 B M McLaughlin , C P Ballance , M S Pindzola , P C Stancil , S Schippers , A Müller

With the flourishing development of nanophotonics, Cherenkov radiation pattern can be designed to achieve superior performance in particle detection by fine-tuning the properties of metamaterials such as photonic crystals (PCs) surrounding…

Optics · Physics 2023-03-22 Xiaoke Gao , Xiaoyu Zhao , Ruoyu Huang , Siyuan Ma , Xikui Ma , Tianyu Dong

Pi-conjugated segments - chromophores - constitute the electronically active units of polymer materials used in organic electronics. To elucidate the effect of bending of these linear moieties on elementary electronic properties such as…

FERM3D is a three-dimensional finite element program, for the elastic scattering of a low energy electron from a general polyatomic molecule, which is converted to a potential scattering problem. The code is based on tricubic polynomials in…

Chemical Physics · Physics 2009-11-13 Stefano Tonzani
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