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We report observation of strong and anisotropic third harmonic generation (THG) in monolayer and multilayer ReS$_2$. The third-order nonlinear optical susceptibility of monolayer ReS$_2$, $\left| \chi^{(3)} \right|$ is on the order of…

Materials Science · Physics 2017-04-12 Qiannan Cui , Rodrigo A. Muniz , J. E. Sipe , Hui Zhao

To add the detailed information to the existed knowledge of nonlinear optics field, the nonlinear optical processes of the second and third order have been discussed in their respective susceptibility tensors in the presence of degenerate…

Optics · Physics 2018-01-29 A Srinivasa Rao

We report experiments on the generation of third and fifth harmonics of millijoule-level, tightly focused, femtosecond laser pulses at 2.2 {\mu}m wavelength in air. The measured ratio of yields of the third and fifth harmonics in our setup…

Optics · Physics 2015-05-28 Gombojav O. Ariunbold , Pavel Polynkin , Jerome V. Moloney

The plasmon-enhanced second harmonic generation in the subwavelength neutral metal cubic nanoparticles is calculated for the first time in the hydrodynamic and cold plasma approximations. The theory is developed that takes into account all…

Mesoscale and Nanoscale Physics · Physics 2016-02-15 S. V. Fomichev , A. M. Bratkovsky

We report the observation of strong third harmonic generation from a macroscopic array of aligned ultralong single-wall carbon nanotubes (SWCNTs) with intense midinfrared radiation. Through power-dependent experiments, we determined the…

Mesoscale and Nanoscale Physics · Physics 2013-04-22 D. T. Morris , C. L. Pint , R. S. Arvidson , A. Luttge , R. H. Hauge , A. A. Belyanin , G. L. Woods , J. Kono

Second-harmonic generation is of paramount importance in several fields of science and technology, including frequency conversion, self-referencing of frequency combs, nonlinear spectroscopy and pulse characterization. Advanced…

We demonstrate the simultaneous generation of second, third, and fourth harmonic from a single dielectric Bismuth Ferrite nanoparticle excited by a telecom fiber laser at 1560 nm. We first characterize the signals associated with different…

We use ultrafast laser pulses to experimentally demonstrate that the second-order optical response of bulk single crystals of the topological insulator Bi$_2$Se$_3$ is sensitive to its surface electrons. By performing surface doping…

Materials Science · Physics 2011-02-02 D. Hsieh , J. W. McIver , D. H. Torchinsky , D. R. Gardner , Y. S. Lee , N. Gedik

We experimentally demonstrate efficient third harmonic generation from an indium tin oxide (ITO) nanofilm (lambda/42 thick) on a glass substrate for a pump wavelength of 1.4 um. A conversion efficiency of 3.3x10^-6 is achieved by exploiting…

The dynamics of an electron-hole plasma governed by strong Coulomb interaction is a challenging many-body problem.We report on experimental realization of electron-hole many-body states in the picosecond time scale, with tunable densities…

Strongly Correlated Electrons · Physics 2025-05-16 Changqing Zhu , Anneke Reinold , Patrick Pilch , Sergey Kovalev , Julian Heckötter , Doris Reiter , Manfred Bayer , Marc Assmann , Zhe Wang

High-harmonic generation (HHG) provides short-wavelength light that is useful for precision spectroscopy and probing ultrafast dynamics. We report efficient, phase-coherent harmonic generation up to 9th-order (333 nm) in chirped…

Second-order nonlinear optical processes do not manifest in the bulk of centrosymmetric materials, but may occur in the angstroms-thick layer at surfaces. At such length-scales, quantum mechanical effects come into play which could be…

Optics · Physics 2021-05-11 Muhammad Khalid , Cristian Ciracì

Second harmonic generation is a powerful tool directly connected to the symmetry of materials. Phase transitions, lattice rotations or electromagnetic coupling in multiferroic compounds can be revealed by using second harmonic…

Optics · Physics 2010-01-11 Pablo Molina , Mariola O Ramirez , Basilio J. Garcia , Luisa E. Bausa

Second harmonic generation has been applied to study lattice, electronic and magnetic proprieties in atomically thin materials. However, inversion symmetry breaking is usually required for the materials to generate a large signal. In this…

Materials Science · Physics 2022-05-12 Zhuoliang Ni , Nan Huang , Amanda V. Haglund , David G. Mandrus , Liang Wu

The generation of harmonics of the voltage response is considered when an AC current is applied through a superconducting film above T_c. It is shown that almost at all temperatures the mechanism of the temperature oscillations created by…

Superconductivity · Physics 2009-11-07 Todor Mishonov , Nicolas Chéenne , Didier Robbes , Joseph Indekeu

The generation of high-order harmonics in finite, hexagonal nanoribbons is simulated. Ribbons with armchair and zig-zag edges are investigated by using a tight-binding approach with only nearest neighbor hopping. By turning an alternating…

Mesoscale and Nanoscale Physics · Physics 2024-03-12 Hannah Jürß , Dieter Bauer

Ever since the advent of high-order harmonic generation, one of the main goals has been to maximize the high harmonic yield. This is due to the wide range of applications in multidisciplinary research fields, including nonlinear XUV optics…

Material systems with lone-pair electrons have long been a treasure trove in the search for large second harmonic generation effects. Revealing the origin of second harmonic generation in nonlinear optical materials can provide theoretical…

Materials Science · Physics 2025-05-13 Fuming Li , Shilie Pan , Zhihua Yang

Recent progresses in femtosecond ytterbium-doped fiber laser technology areopening new perspectives in strong field physics and attosecond science. Highorder harmonic generation from these systems is particularly interesting because it…

We report a set of experimental data on local third-harmonic generation at microwave frequencies (0.5 GHz) in $YBa_2Cu_3O_7$ and Nb films. For local investigations of the nonlinear response a probe with inductive coupling was elaborated.…

Superconductivity · Physics 2007-05-23 Evgeny E. Pestov , Yury N. Nozdrin , Vladislav V. Kurin